Abstract
An amphiphilic tetrathiafulvalene derivative, with two alkylphosphonic acid substituents, has been prepared and used to form a mixed organic/inorganic Langmuir-Blodgett (LB) film containing a TTF-based organic network and a manganese phosphonate continuous lattice inorganic network. The inorganic network is isostructural with known manganese phosphonate layered solids, and undergoes magnetic ordering to a canted antiferromagnetic ground state. A model TTF derivative containing the alkylphosphonic acids, but without hydrophobic alkyl tails, was also synthesized and a manganese phosphonate solid, isostructural with the LB film, was prepared and characterized.
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