Abstract
We present a Lagrangian stochastic model of vertical dispersion in the convective boundary layer (CBL). This model is based on a generalized Langevin equation that uses the simplifying assumption that the skewed vertical velocity probability distribution is spatially homogeneous. This approach has been shown to account for two key properties of CBL turbulence associated with large-scale coherent turbulent structures: skewed vertical velocity distributions and long velocity correlation time. A 'linear-skewed' form of the generalized Langevin equation is used, which has a linear (in velocity) deterministic acceleration and a skewed random acceleration. 'Reflection' boundary conditions for selecting a new velocity for a particle that encounters a boundary were investigated, including alternatives to the standard assumption that the magnitudes of the particle incident and reflected velocities are positively correlated. Model simulations were tested using cases for which exact, analytic statistical properties of particle velocity and position are known, i.e., well-mixed spatial and velocity distributions. Simulations of laboratory experiments of CBL dispersion show that (1) the homogeneous linear-skewed Langevin equation model (as well as an alternative 'nonlinear-Gaussian' Langevin equation model) can simulate the important aspects of dispersion in the CBL, and (2) a negatively-correlated-speed reflection boundary condition simulates the observed dispersion of material near the surface in the CBL significantly better than alternative reflection boundary conditions. The homogeneous linear-skewed Langevin equation model has the advantage that it is computationally more efficient than the homogeneous nonlinear-Gaussian Langevin equation model, and considerably more efficient than inhomogeneous Langevin equation models.
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