A fiber-shaped temperature sensor composed of chitosan/rGO with high sensitivity and ultra-fast response and recovery for real-time temperature monitoring

Abstract

Wearable sensors are the development trend in the future iteration of medical devices, in which, flexible temperature sensors with high resolution, fast response speed, and good reliability under deformations, are one of the much important devices. In this study, a nano multilayer sensing structured fiber temperature sensor is fabricated via in situ coating reduced graphene oxide (rGO) and chitosan (CS) on the surface of stretchable polyurethane fiber (PF) by a layer-by-layer self-assembly method. The introduction of CS not only enhances the temperature sensitivity (with a temperature coefficient of −1.379 %‧°C−1 in the range of 30–60 °C) of the rGO-based fiber sensors but also greatly increases the mechanical stability of the nanofibrous membrane. Most importantly, the fiber-shaped temperature sensor shows a fast response time (2.4 s) and recovery time (3.9 s) to temperature. Moreover, the sensor achieves a high temperature resolution of 0.1 °C. Made from a simple and low-cost process, the fiber-like devices can be easily integrated into items such as gloves or face masks to monitor the real-time temperature changes. The results demonstrate the great potential of rGO-based fiber sensors for applications in human healthcare monitoring.