Abstract
The reaction of 1-aroyl-2-aryl-3a,6a-diazapentalenes with acetylene-dicarboxylates affords surprisingly unusual anti-Bredt's adducts having 4,10-diazabicyclo[5.2.1]deca-1,3,5,8-tetraene structure. The structure was elucidated by making full uses of new MMR spectroscopies and finally an X-Ray crystallographic analysis. The plausible mechanism for the formation of the present compounds is described.
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