A digitally generated ultrafine optical frequency comb for spectral measurements with 0.01-pm resolution and 0.7-µs response time

Abstract

Optical spectral measurements are crucial for optical sensors and many other applications, but the prevailing methods, such as optical spectrum analysis and tunable laser spectroscopy, often have to make compromises among resolution, speed, and accuracy. Optical frequency combs are widely used for metrology of discrete atomic and molecular spectral lines. However, they are usually generated by optical methods and have large comb spacing, which limits the resolution for direct sampling of continuous spectra. To overcome these problems, this paper presents an original method to digitally generate an ultrafine optical frequency comb (UFOFC) as the frequency ruler for spectral measurements. Each comb line provides one sampling point, and the full spectrum can be captured at the same time using coherent detection. For an experimental demonstration, we adopted the inverse fast Fourier transform to generate a UFOFC with a comb spacing of 1.46 MHz over a 10-GHz range and demonstrated its functions using a Mach-Zehnder refractive index sensor. The UFOFC obtains a spectral resolution of 0.01 pm and response time of 0.7 μs; both represent 100-fold improvements over the state of the art and could be further enhanced by several orders of magnitude. The UFOFC presented here could facilitate new label-free sensor applications that require both high resolution and fast speed, such as measuring binding kinetics and single-molecule dynamics. Optical frequency combs with ultrafine spacings look set to bring big improvements to spectral measurements and optical sensing. Yuan Bao and co-workers from China and the USA used custom-designed electrical wavefronts prepared by a digital signal processor to modulate the output of a narrow-linewidth laser. The result was an ultrafine optical frequency comb with a spacing as small as 1.46 MHz over a range of 10 GHz. Significantly, the digital signal processor prepared the comb in just 0.7 μS. Such a comb is ideal for fast, very high-resolution (0.01 pm) spectral measurements and far outperforms the scan speed and resolution of conventional grating-based optical spectrum analysers. The team demonstrated the benefits of their ultrafine comb in a highly sensitive Mach-Zehnder refractive index sensor.