A coupled watershed-biogeochemical model to simulate dissolved and particulate 137Cs discharge from a forested catchment affected by the Fukushima accident

Abstract

<p>Dissolved <sup>137</sup>Cs discharge represents approximately 30% of the total <sup>137</sup>Cs discharge from the forested upstream catchment of the Ohta River in Fukushima, Japan [1]. It is thought that a major source of the dissolved <sup>137</sup>Cs entering the river water may be leaching from forest litter [1]. A watershed simulation based on the distribution coefficient (K<sub>d</sub>) that modelled water, sediment, and particulate and dissolved <sup>137</sup>Cs transport could not reproduce the seasonal variability of the base flow dissolved <sup>137</sup>Cs concentrations, nor the peaks in concentration that occurred during storms [2].</p><p>We developed a combined watershed-biogeochemistry model for simulating dissolved and particulate <sup>137</sup>Cs discharge from forest catchments to describe the two phenomenon as mentioned above. A compartment model for the forest ecosystem was appended to the General-purpose Terrestrial fluid-Flow Simulator (GETFLOWS) watershed code. The compartment model included compartments for undecomposed and decomposed litter, with transfer from the former into the latter depending on temperature. A pathway for dissolved <sup>137</sup>Cs input to forest streams was linked from the decomposed litter compartment.</p><p>The results from a simulation with the new simulation model reproduced the seasonal variability of dissolved <sup>137</sup>Cs concentrations and the peaks occurring during storms. Therefore the new modelling results add weight to the theory that leaching from decomposed litter can input dissolved <sup>137</sup>Cs concentrations in river water in Fukushima Prefecture. The developed model is expected to be useful for further explorations into factors affecting dissolved <sup>137</sup>Cs input to river water in forested catchments.</p><p> </p><p>[1]Tsuji et al., 2016. J. Geophys. Res. Biogeosci. 121, 2588-2599.</p><p>[2]Sakuma et al., 2018. J. Environ. Radioact. 184-185, 53-62.</p>