Abstract
Over the past few years there has been an active program in their laboratories on long-range intramolecular electron transfer and its dependence on energetics, solvent, distance, and stereochemistry. More recently the authors have extended this study to include positive ions, or hole transfer, and triplet energy transfer. The compounds in the three studies were the same or closely related, and the processes can be summarized and designated as in (1). D{sup {minus}}-Sp-A {yields} D-Sp-A{sup {minus}} (ET); D{sup +}-Sp-A {yields} D-Sp-A{sup +} (HT); D{prime}{sup 3}-Sp-A {yields} D-Sp-A{sup 3} (TT). In the three series A = 2-naphthyl, and D = 4-biphenylyl in the Et and HT series and 4-benzophenoyl in the TT series.
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