Abstract

This work deals with a comprehensive theoretical and numerical framework that allows the modeling of finite strain magnetorheological elastomers (MREs) comprising mechanically soft nonlinear elastic–viscoelastic polymer phases and magnetically hard (i.e. dissipative) or soft (i.e. purely energetic) magnetic phases. The framework is presented in a general manner and is implemented using the finite element method. Two software implementations are developed, one using FEniCS and the other in Abaqus. A detailed analysis of the numerical schemes used to model the surrounding air is made and their pros and cons are discussed. The proposed framework is used to simulate two model geometries that are directly relevant to recent applications of MREs. The first two-dimensional example simulates a mechanically soft beam consisting of a single wavy-chain of hard or soft magnetic particles. The beam is subjected to transverse magnetic actuation loads that induce important vertical deflections. Despite the overall small local strains in the beam, a significant viscoelastic effect is observed when high-rate magnetic fields are applied. A torque model for the particles is also used to analyze the beam geometry and is found to be in relatively good agreement with the rest of the approaches for small actuation fields. The second example discusses the rotation of a three-dimensional ellipsoid embedded in a cubic elastomer domain, while the ensemble lies inside a larger cubic air domain. Non-monotonic uniaxial and rotating magnetic fields are applied leading to complex, non-monotonic rotations of the ellipsoidal particle. The hard and soft magnetic cases exhibit significant differences, whereas viscoelasticity is found to induce strong coupling with the magnetization rotation but not with the dissipative magnetization amplitude. Extensive supplementary material provides all details of our implementations as well as animated visualization of results.

Highlights

  • Magnetorheological elastomers (MREs) or magnetoactive polymers (MAEs) are most often designed as composites comprising a soft elastomer matrix carrying micron-sized magnetic inclusions

  • For that purpose we present a thermodynamically consistent computational framework based on the formalism of generalized standard materials [51,52] accounting for viscoelasticity and ferromagnetic hysteresis inspired by Miehe et al [53] and Kumar and Lopez-Pamies [54]

  • We begin with the fundamentals of magnetomechanics at finite strains before presenting the magnetomechanical initial boundary value problem (IBVP) considered in this work

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Summary

Introduction

Magnetorheological elastomers (MREs) or magnetoactive polymers (MAEs) are most often designed as composites comprising a soft elastomer matrix carrying micron-sized magnetic inclusions. Keip and Sridhar [43] addressed the point of dissipative ferromagnetism at the particle level with the framework of micromagnetics [44] While this approach provides great insight into the fine-scale details of domain wall motion, its computational cost renders it prohibitive for the simulation of macroscopic MREs. We mention the recent contributions considering already magnetized elastic [45,46,47] and viscoelastic [48] bodies. These examples demonstrate the effect of viscosity and ferromagnetic hysteresis compared with purely elastic and magnetically non-hysteretic responses.

Theory
Fundamentals of magnetomechanics
The abstract magnetomechanical initial boundary value problem
Specialization to a particle–matrix system
Air domain
Discretization and numerics
Time discretization
Deformation in free space
Non-local mesh-coupling
Auxiliary energy density of free space
Effect of the modeling of free space
Hard versus soft magnetic particles
Rotating magnetic field
Conclusion
Full Text
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