A comprehensive reappraisal of long-term aerosol characteristics, trends, and variability in Asia

Abstract

Abstract. Changes in aerosol loadings and properties are important for the understanding of atmospheric environment and climate change. This study investigates the characteristics and long-term trends of aerosols of different sizes and types in Asia from 2000 to 2020 by considering multi-source aerosol data and novel analysis methods and perspectives, all of which provides the groundwork for promoting the acquisition of new discoveries that are different from the past. The geometric mean aggregation method is applied, and serial autocorrelation is considered to avoid the overestimation of trend significance. Among regions in Asia, high values of aerosol optical depth (AOD) are mainly concentrated in East Asia (EA) and South Asia (SA) and are closely related to the population density. The AOD in EA showed the most significant negative trend, with a value of -5.28×10-4 per year, mainly owing to decreases in organic carbon (OC), black carbon (BC), and dust aerosols. It is also worth noting that this observed large-scale decrease in OC and BC is a unique and significant phenomenon to region of EA and mainly around China. In contrast, the aerosol concentrations in SA generally show a positive trend, with an increased value of AOD of 1.25 × 10−3 per year. This increase is mainly due to large emissions of fine-mode aerosols, such as OC and sulfate aerosol. Additionally, the high aerosol loading in northern SA has a lower AOD variability when compared with that of East China Plain, revealing a relatively more persistent air pollution situation. Over the whole region of Asia, the characteristics of the percentage changes in different types of AOD are seen in the increases in BC (6.23 %) and OC (17.09 %) AOD, together with a decrease in dust (−5.51 %), sulfate (−3.07 %), and sea salt (−9.80 %) AOD. Except for anthropogenic emissions, the large increase in the percentage of OC is also due to wildfires found in northern Asia in the summer, whereas the differently sized AOD only shows slight changes in Asia in that small-sized AOD decreases (−3.34 %) and that the total AOD did not show a significant change. This suggests that, from a trend perspective, decreases in aerosol in recent years have mostly been offsetting earlier increases in the anthropogenic emissions over Asia. To summarize, the above findings analyse the comprehensive characteristics of aerosol distributions and reappraise the long-term trends of different aerosol parameters, which will greatly enhance the understanding of regional and global aerosol environment and climatology, in addition to filling the gaps and breaking through the limitations of past knowledge.