Abstract
The CO 2 laser-induced multiphoton dissociation (MPD) of C 3H 5X(CH 3) 3 molecules (X=C or Ge) in the gas phase was studied. Average energy absorbed by molecules with C at dissociation threshold is higher than that for Ge-containing molecules. The dependence of fragmentation probability of X(CH 3) 3, formed from MPD of C 3H 5X(CH 3) 3, on the laser fluence is different for molecules with C or Ge. The distinctions in MPD of these molecules can be attributed to the heavy-atom effect on the vibrational energy transfer over the molecule.
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