Abstract

Vehicles are major sources of air pollutant emissions, and individuals living near large roads endure high exposures and health risks associated with traffic-related air pollutants. Air pollution epidemiology, health risk, environmental justice, and transportation planning studies would all benefit from an improved understanding of the key information and metrics needed to assess exposures, as well as the strengths and limitations of alternate exposure metrics. This study develops and evaluates several metrics for characterizing exposure to traffic-related air pollutants for the 218 residential locations of participants in the NEXUS epidemiology study conducted in Detroit (MI, USA). Exposure metrics included proximity to major roads, traffic volume, vehicle mix, traffic density, vehicle exhaust emissions density, and pollutant concentrations predicted by dispersion models. Results presented for each metric include comparisons of exposure distributions, spatial variability, intraclass correlation, concordance and discordance rates, and overall strengths and limitations. While showing some agreement, the simple categorical and proximity classifications (e.g., high diesel/low diesel traffic roads and distance from major roads) do not reflect the range and overlap of exposures seen in the other metrics. Information provided by the traffic density metric, defined as the number of kilometers traveled (VKT) per day within a 300 m buffer around each home, was reasonably consistent with the more sophisticated metrics. Dispersion modeling provided spatially- and temporally-resolved concentrations, along with apportionments that separated concentrations due to traffic emissions and other sources. While several of the exposure metrics showed broad agreement, including traffic density, emissions density and modeled concentrations, these alternatives still produced exposure classifications that differed for a substantial fraction of study participants, e.g., from 20% to 50% of homes, depending on the metric, would be incorrectly classified into “low”, “medium” or “high” traffic exposure classes. These and other results suggest the potential for exposure misclassification and the need for refined and validated exposure metrics. While data and computational demands for dispersion modeling of traffic emissions are non-trivial concerns, once established, dispersion modeling systems can provide exposure information for both on- and near-road environments that would benefit future traffic-related assessments.

Highlights

  • Residential location and proximity to major roads have been widely used in analyses of exposures and adverse health effects that can result from traffic-related air pollutants, reflecting the elevated concentrations found near busy roads [1,2,3,4,5,6,7,8,9]

  • This paper explores alternate metrics for characterizing exposure to traffic-related air pollutants, including metrics based on proximity to major roads, traffic volume and density, traffic type, traffic emissions density, and pollutant concentrations from dispersion modeling

  • The evaluation of the exposure metrics presented in this paper includes a comparison of exposure distributions, spatial variability using maps coded by exposure group, intraclass correlations, and concordance rates

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Summary

Introduction

Residential location and proximity to major roads have been widely used in analyses of exposures and adverse health effects that can result from traffic-related air pollutants, reflecting the elevated concentrations found near busy roads [1,2,3,4,5,6,7,8,9]. Residence location or proximity to roads can be used as a surrogate exposure metric itself, or as an input to land use regression, dispersion, space-time (geostatistical), and hybrid models, which are designed to estimate ambient air concentrations and sometimes personal exposures [11,12,13,14,15]. Ambient air quality monitoring networks do not provide the spatial coverage needed to estimate near-road exposures [13], and personal, home or biomarker measurements rarely are feasible in large scale studies. It remains important to improve exposure estimates that are used in epidemiology, health impact, environmental justice and other studies [1,14,16,17,18]

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