Abstract
The Cs3d3/2-core regions of atomic Cs and molecular CsCl have been compared. In atomic cesium, two satellites with a combined intensity of 18% of the 3d3/2 peak have been observed at 5.3 and 7.7 eV higher binding energy. Dirac–Fock calculations suggest that they are mostly due to 6s → 7s and 6s → 8s excitation accompanying core ionization. In contrast, no intense satellites have been observed in CsCl, since the Cs6s electron has been partially transferred to the chlorine.
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