Abstract

Water evaporation systems driven by solar energy delivers great potential for seawater desalination and sustainable energy generation, which is of great significance to relieve the worldwide shortage of fresh-water and energy. However, the achievement of well-designed materials and configuration for water evaporation systems remains a great challenge, hindering the realization of high evaporation rates and stable energy output. Herein, conductive coal-based nanocarbon material was creatively fabricated to assemble a novel multifunctional membrane based evaporation system for simultaneous solar thermal desalination of seawater and power generation. The coal-based multifunctional membrane (CBMM) possesses a permanently asymmetric wetting structure, which can ensure high photothermal evaporation efficiency and stable energy output. The constructed device unit demonstrate a long and stable operation in seawater under one sun irradiance for 100 h, achieving a high evaporation rate of 1.81 kg m−2 h−1 and a large voltage output of 410 mV. Especially, multiple units of the devices can be easily connected in series or parallel to power small electronic devices. This work provides a cost-effective and large scale method for the fabrication of coal-based nanomaterials and the creative application in high-perforamnce water evaporation systems for seawater desalination and sustainable energy generation.

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