Abstract

A global climatology of absorbing carbonaceous aerosols (ACA) for the period 2005–2015 is obtained by using satellite MODIS (Moderate Resolution Imaging Spectroradiometer)-Aqua and OMI (Ozone Monitoring Instrument)-Aura aerosol optical properties and by applying an algorithm. The algorithm determines the frequency of presence of ACA (black and brown carbon) over the globe at 1° × 1° pixel level and on a daily basis. The results of the algorithm indicate high frequencies of ACA (up to 19 days/month) over world regions with extended biomass burning, such as the tropical forests of southern and central Africa, South America and equatorial Asia, over savannas, cropland areas or boreal forests, as well as over urban and rural areas with intense anthropogenic activities, such as the eastern coast of China or the Indo-Gangetic plain. A clear seasonality of the frequency of occurrence of ACA is evident, with increased values during June–October over southern Africa, during July–November over South America, August–November over Indonesia, November–March over central Africa and November–April over southeastern Asia. The estimated seasonality of ACA is in line with the known annual patterns of worldwide biomass-burning emissions, while other features such as the export of carbonaceous aerosols from southern Africa to the southeastern Atlantic Ocean are also successfully reproduced by the algorithm. The results indicate a noticeable interannual variability and tendencies of ACA over specific world regions during 2005–2015, such as statistically significant increasing frequency of occurrence over southern Africa and eastern Asia.

Highlights

  • Atmospheric aerosols can cause an overall planetary cooling, partly counterbalancing the global warming caused by greenhouse gases [1]

  • The combination of daily 1◦ ×1◦ gridded MODIS and OMI data, which are indicative of aerosol load (AOD), size and absorptivity (AI), enable the identification/characterization of absorbing carbonaceous aerosols (ACA)

  • The algorithm ran on a daily basis and for each year of the study period (2005–2015)

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Summary

Introduction

Atmospheric aerosols can cause an overall planetary cooling, partly counterbalancing the global warming caused by greenhouse gases [1]. In spite of the overall aerosol cooling, absorbing. Atmosphere 2019, 10, 671 carbonaceous aerosols (ACA) including black carbon (BC) and brown organic carbon (BrOC) warm the planet. The BC aerosols dominated by soot-like elemental carbon (EC) are stronger absorbers of solar radiation than brown (BrOC), being referred as brown carbon (BrC) aerosols, which mainly absorb at visible to ultraviolet wavelengths [3]. Both are primarily consisted of fine particles mostly less than

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