A CFD study of ignition of lean propane-air mixtures in a heat recirculating U-bend catalytic microreactor

Abstract

Heat recirculating (HR) geometries have been studied in the literature for their use in energy generation applications. This work investigates the ignition and cold-start behavior of lean propane-air combustion in a U-bend catalytic microreactor through computational fluid dynamics (CFD) study. Although several studies have focused on stability and combustion behavior, the role of heat recirculation on catalytic and homogeneous ignition from the cold-start conditions has not been analyzed so far. The U-bend microreactor is a typical example of HR geometry, where the hot exhaust gases in the recirculation channel transfer heat to the cold incoming fluid. Significance of heat recirculation across the dividing wall on the ignition temperature, as well as transient evolution of temperature, propane conversion and reaction are presented. Ignition temperature is found to be 20K lower in the U-bend microreactor than straight channel microreactor. However, transient ignition study revealed that at nominal conditions, U-bend microreactor takes about 35s longer than straight channel for ignition and to reach steady state, owing to heat distribution internally within the U-bend microreactor. The effect of flowrate is analyzed, which shows that at higher flowrates, the ignition and steady-state times are also lower for the U-bend microreactor. Finally, the effect of solid wall material is investigated, which shows that lower conductivity material (such as ceramic) showed faster ignition with low thermal inputs.