Abstract

We use ERA-Interim reanalysis, MLS observations, and a trajectory model to examine the chemical transport and tracers distribution in the Upper Troposphere and Lower Stratosphere (UTLS) associated with an east-west oscillation case of the anticyclone in 2016. The results show that the spatial distribution of water vapor (H2O) was more consistent with the location of the anticyclone than carbon monoxide (CO) at 100 hPa, and an independent relative high concentration center was only found in H2O field. At 215 hPa, although the anticyclone center also migrated from the Tibetan Mode (TM) to the Iranian Mode (IM), the relative high concentration centers of both tracers were always colocated with regions where upward motion was strong in the UTLS. When the anticyclone migrated from the TM, air within the anticyclone over Tibetan Plateau may transport both westward and eastward but was always within the UTLS. The relative high concentration of tropospheric tracers within the anticyclone in the IM was from the east and transported by the westward propagation of the anticyclone rather than being lifted from surface directly. Air within the relative high geopotential height centers over Western Pacific was partly from the main anticyclone and partly from lower levels.

Highlights

  • The Asian summer monsoon is an important component of global climate system and a significant system of global atmospheric circulation in boreal summer [1]

  • It plays an important role in StratosphereTroposphere Exchange (STE) because of persistent deep convections and the impact on mass transport, especially on chemical distribution in the Upper Troposphere and Lower Stratosphere (UTLS) region [9, 19, 20, 27,28,29]

  • Both carbon monoxide (CO) and H2 O variability at 100 hPa during the period indicate that mass distribution on this level migrated from Tibetan mode to Iranian mode with the

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Summary

Introduction

The Asian summer monsoon is an important component of global climate system and a significant system of global atmospheric circulation in boreal summer [1]. Asian summer monsoon anticyclone (South Asia High) is one of the dominant features of the Asian summer monsoon [1, 18,19,20,21,22,23,24,25,26] It plays an important role in STE because of persistent deep convections and the impact on mass transport, especially on chemical distribution in the Upper Troposphere and Lower Stratosphere (UTLS) region [9, 19, 20, 27,28,29]. Chemical species mixing ratio from satellite data, meteorological field from reanalysis data, and a trajectory model are combined to address the following questions: (1) How does the east-west oscillation of the Asian summer monsoon anticyclone influence chemical distribution in the UTLS? We analyze space-time variability of CO and H2 O in the UTLS to investigate the mass transport that is related to the anticyclone oscillation

Data and Model
Chemical Distribution in the UTLS
Tropospheric Upward Motion
Trajectory Analysis
Conclusions
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