Abstract

First step in molybdenum isotope separation for medical purposes project, based in laser ablation followed by electromagnetic separation methods, is the characterization of ablated plasma plume. In this work, a depth profile emission spectroscopy study of laser-ablated molybdenum plasma expanding on air at atmospheric pressure was performed, considering Local Thermodynamic Equilibrium and one-dimensional uniform expanding models. Plasma temperature, electron density, electron population distribution and electron impact width parameter were evaluated along plasma expansion axis and reach average values of 15000 K,1018cm-3, 1% of electron populationat 4d45s6sstate and (0.017±0.008) nm, respectively. Furthermore, mean velocity of (5.0±0.7) km/sand the plasma lifetime that was (160± 14)ns for length equal to (1.80±0.05) mm weremeasured. So, this work includes a description of mainly plasma plume parameters, which permits a discussion for isotope separation methods related to laser ablation.

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