Abstract
Improvements in a 16-μm radiation source based upon the combined effects of stimulated rotational Raman scattering and resonantly enhanced four-wave mixing in parahydrogen gas are described. For this source, the input waves of which are provided by temporally and spatially coincident pulsed beams from a ruby and CO <inf xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</inf> TEA laser, it was found that cooling the parahydrogen gas from 300 K to <100 K, at constant molecular density, increased the output at 16 μm by roughly a factor 4. The maximum output was measured to be <tex xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">\sim 40 \mu</tex> J/pulse, which is near the theoretical limit for the 2.5 MW CO <inf xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</inf> laser intensities that were applied.
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