648-Hilbert space dimensionality in biphoton frequency combs for quantum-secure communications and networks

Abstract

High-dimensional entanglement with larger Hilbert spaces enable an encoding of more bits per photon and thus promise increased communication capacities over quantum channels. Quantum frequency combs, which are intrinsically multimode in the temporal and frequency degrees of freedom within a single spatial mode, naturally facilitating the generation and measurement of high-dimensional entanglement. Current challenges include the extension of well-known methods for two qubits to high-dimensional quantum systems and their application in entanglement experiments with photons. More specifically, the major challenge is the certification of high-dimensional entanglement by a number of accessible experimental measurements. In this paper, we increase the Hilbert space dimensionality and provide versatile tools for quantifying and certifying high-dimensional entanglement in a biphoton frequency comb. We quantify the time binned Schmidt number up to 18 and certify entanglement of formation with 1.89 ebits. We have demonstrated a 648- dimensional Hilbert spaces with time-frequency entanglement in a biphoton frequency comb, enabling a computational space up to 13 photonic qubits, and 6.28 bits/photon classical information capacity. This high-dimensional time frequency multimode quantum states of biphoton frequency comb significantly boosting the photon information capacity that is critical for large-scale quantum information processing. Biphoton frequency comb has indeed demonstrated an attractive and powerful approach towards achieving this fundamental goal with applications in high-dimensional quantum information processing, time-frequency cluster-state quantum computation, high-dimensional encoding in quantum networks, and high-dimensional quantum simulations.