63Ni, its half-life and standardization: Revisited

Abstract

Recent liquid scintillation (LS) measurements at the National Institute of Standards and Technology (NIST) and at the Laboratoire National Henri Becquerel (LNHB) on a standardized 63Ni solution that has been tracked for nearly 40 years have resulted in several important findings: (i) a 63Ni half-life value of 101.2±1.5 a has been determined with the present decay data. This value is consistent with a previous specific activity determination and with an earlier value from decay measurements; and it appears to be more satisfactory than a recent data evaluator's recommended value of 98.7 a. (ii) All solution standards of 63Ni as disseminated by NIST for the past 38 + years are internally consistent with past and recent standardizations. (iii) Primary LS standardizations of 63Ni by the triple-to-double coincidence ratio (TDCR) method and by CIEMAT/NIST 3H-standard efficiency tracing (CNET) appear to be comparable, although the latter methodology is believed to be inherently inferior. (iv) There is excellent measurement agreement between NIST and LNHB for 63Ni primary standardizations.