Abstract

Investigations of magnetic and related electronic properties of UTX compounds have revealed a variety of magnetic phenomena ranging from weak paramagnetism to various types of magnetic ordering. The observed systematics of ground-state properties is discussed with respect to the development of the electronic structure related to the expected variations of the 5f-ligand hybridization. The huge magnetic anisotropy observed in all studied materials is tentatively attributed mainly to the hybridization-mediated anisotropic two-ion interaction.

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