Abstract
Towards a new family of ligands: The synthesis of the ligand HLT (depicted left) is described. Although HLT appears to be a simple chelating diphosphane, the tiazole proton can be removed with a base to produce an anionic diphosphane. Thus HLT can chelate in two modes: as a neutral rigid diphosphane, or as an anionic rigid diphosphane. Furthermore, HLT reacts in an unprecedented fashion with Me3SiN3 to give LT-N (depicted right).
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