Abstract

A 3He neutron spin filter (NSF) program for polarized neutron scattering was launched in 2006 as part of the National Institute of Standards and Technology (NIST) Center for Neutron Research (NCNR) Expansion Initiative. The goal of the project was to enhance the NCNR polarized neutron measurement capabilities. Benefitting from more than a decade's development of spin-exchange optical pumping (SEOP) at NIST, we planned to employ SEOP based 3He neutron spin filters for the polarized neutron scattering community. These 3He NSF devices were planned for use on different classes of polarized neutron instrumentation at the NCNR, including triple-axis spectrometers (TAS), small-angle neutron scattering instruments (SANS), reflectometers, and wide-angle polarization analysis. Among them, the BT-7 thermal TAS, NG-3 SANS, and MAGIK reflectometer have already been in the user program for routine polarized beam experiments. Wide-angle polarization analysis on Multi-Axis Crystal Spectrometer (MACS) has been developed for user experiments. We describe briefly the SEOP systems dedicated for polarized beam experiments and polarizing neutron development for each instrument class. We summarize the current status and polarized neutronic performance for each instrument. We present a 3He NSF hardware and software interface to allow for synchronization of 3He polarization inversion (neutron spin flipping) and free-induction decay (FID) nuclear magnetic resonance (NMR) measurements with neutron data collection.

Highlights

  • Polarized neutron scattering (PNS) is a powerful tool that probes magnetic structures and morphologies, magnetization density, and magnetic excitations in a wide range of magnetic materials

  • We have provided an overview of the polarized neutron development using 3He neutron spin filters (NSF) at the National Institute of Standards and Technology (NIST) Center for Neutron Research (NCNR) during the last several years

  • We have demonstrated the polarized neutronic performance is highly predictable when the proper polarized beam calibration is done

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Summary

Introduction

Polarized neutron scattering (PNS) is a powerful tool that probes magnetic structures and morphologies, magnetization density, and magnetic excitations in a wide range of magnetic materials. More extensive theoretical work on PNS was developed after Halpern and Johnson[2, 3, 4]. In 1969, Moon et al experimentally demonstrated unambiguous separation of magnetic scattering from nuclear scattering, and nuclear coherent scattering from spin-incoherent scattering using uniaxial polarization analysis on a triple axis spectrometer (TAS)[5]. The uni-axial polarization analysis technique was later expanded to the xyz polarization analysis technique for separation of nuclear, magnetic, and spin-incoherent scattering[6].

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