Abstract
Photocurable 3D printing of polyphenol-based gels has been limited by the catechol groups, which can scavenge free radicals generated by photoinitiators during photopolymerization. Herein, a 3D-printed gel composed of poly-acrylamide (PAM) and tannic acid (TA) is presented, fabricated by using glycerol as shielding of TA and a commercial digital light processing printer. The printed gels are based on a polymeric network interpenetrated by TA-glycerol, enabling the printed objects with various favorable properties, such as improved toughness, anti-dehydration, antioxidant and antibacterial properties, etc. The proposed strategy enables photocurable 3D printing of polyphenol-based gels with complex architecture, paving the way for future applications in various fields, ranging from soft wearable devices to tissue engineering.
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