Abstract
A thorough understanding of the thermal stability and potential reshaping of anisotropic gold nanostars is required for various potential applications. Combination of a tomographic heating holder with fast tilt series acquisition has been used to monitor temperature-induced morphological changes of Au nanostars. The outcome of our 3D investigations can be used as an input for boundary element method simulations, enabling us to investigate the influence of reshaping on the nanostars' plasmonic properties. Our work leads to a better understanding of the mechanism behind thermal reshaping. In addition, the approach presented here is generic and can hence be applied to a wide variety of nanoparticles made of different materials and with arbitrary morphology.
Highlights
Gold nanoparticles (Au NPs) have shown enormous potential for applications in various fields, ranging from biology and medicine to chemistry and physics
We implemented a novel methodology to perform fast electron tomography, which allowed us to observe the morphological evolution of Au NSs heated at 200 °C, 300 °C and 400 °C, at different time steps up to 1200 s
We show that the major part of the morphological evolution occurs within the first minute of heating, regardless of temperature
Summary
Gold nanoparticles (Au NPs) have shown enormous potential for applications in various fields, ranging from biology and medicine to chemistry and physics.
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