Abstract
AbstractSynthesis of vertical heterostructures that include atomically thin layers of materials with topologically nontrivial energy bands is desirable for exploring exotic quantum states. Here, the authors report on atomic‐layer‐by‐layer deposition of magnesium on copper(111) surface by molecular beam epitaxy, monitored in situ by low‐energy electron microscopy and diffraction, and modeled by ab initio theory. It is found that a 2D MgCu2 intermetallic compound forms during initial Mg deposition and persists till a full monolayer of Mg is formed. Deposition of additional Mg triggers a phase transition from the commensurate MgCu2 to an incommensurate Mg2Cu layer and enables growth of the second layer of Mg. Ab initio calculations indicate non‐trivial topology of the electron bands in the interfacial Mg2Cu layer and the existence of Dirac nodal lines near the Fermi level. The new 2D Mg2Cu material emerges as a promising platform to study new topological states of matter.
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