Abstract
Electron rescattering has been well studied and simulated for cases with ponderomotive energies of the quasi-free electrons, derived from laser–gas and laser–surface interactions, lower than 50 eV. However, with advents in longer wavelengths and laser field enhancement metallic surfaces, previous simulations no longer suffice to describe more recent strong field and high yield experiments. We present a brief introduction to and some of the theoretical and empirical background of electron rescattering emissions from a metal. We set upon using the Jellium potential with a shielded atomic surface potential to model the metal. We then explore how the electron energy spectra are obtained in the quantum simulation, which is performed using a custom computationally intensive time-dependent Schrödinger equation solver via the Crank–Nicolson method. Finally, we discuss the results of the simulation and examine the effects of the incident laser’s wavelength, peak electric field strength, and field penetration on electron spectra and yields. Future simulations will investigate a more accurate density functional theory metallic model with a system of several non-interacting electrons. Eventually, we will move to a full time-dependent density functional theory approach.
Highlights
Electron rescattering from a metal is the process in which an intense ultrafast laser pulse incident on a metal frees electrons through a three step process as is described here
We performed 1D time-dependent Schrödinger equation (TDSE) simulations of an electron bound to a metal undergoing electron rescattering
We used some finite-difference time-domain (FDTD)-derived fields to look for field penetration effects
Summary
Electron rescattering from a metal is the process in which an intense ultrafast laser pulse incident on a metal frees electrons through a three step process as is described here. In order of required field intensity, the electron may multi-photon ionize [1], above-threshold ionize (ATI) [2], or quantum tunnel (strong-field ionize) [3] out of the metal It propagates in the field and either continues away from the system (direct electrons) or returns to the metal to be potentially scattered and re-emitted (rescattered electrons). This photoionization process is different from the standard photoelectric effect in that, with sufficient fields, quantum tunneling effects overpower the dimmer multiphoton and ATI contributions. These processes have been studied extensively in the atomic, or gas, regime ([4,5] for instance), and increasing interest has begun to surround metallic emitters
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