Abstract
HighlightsUltra-thin asymmetric composite solid-state electrolytes with ultralight areal density were designed for solid-state lithium metal batteries, achieving interfacial stability to Li metal and high-voltage cathode.The improved mechanical properties of the electrolyte contribute to the inhibition of Li dendrite growth was demonstrated by both experimental and theoretical simulations.The assembled pouch cell exhibited a high gravimetric/volume energy density of 344.0 Wh kg−1/773.1 Wh L−1.
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