Abstract
It is demonstrated that 50% substitution of vanadium for molybdenum in the pyrochlore lattice of the complex oxide Y2(V x Mo1 − x )2O7 results in a transition from the spin-glass ground state (at x = 0) to the ferromagnetic state in Y2VMoO7 (a = 10.1645(2) Å, T C = 55 K). The Gd2V0.67Mo1.33O7 compound (a = 10.2862(3) Å) is a ferromagnet with T C (84 K) exceeding that of undoped Gd2MnO2O7.
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