Abstract

Recent developments in the physics of high-index resonant dielectric nanostructures suggest alternative mechanisms for subwavelength light control driven by Mie resonances with strong magnetic response that can be employed for a design of novel optical metasurfaces. Here we demonstrate metasurfaces based on nanoimprinted perovskite films optimized by alloying the organic cation part of perovskites. We reveal that such metasurfaces can exhibit a significant enhancement of both linear and nonlinear photoluminescence (up to 70 times) combined with advanced stability. Our results suggest a cost-effective approach based on nanoimprint lithography and combined with simple chemical reactions for creating a new generation of functional metasurfaces which may pave a way towards highly efficient planar optoelectronic metadevices.

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