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Coupling of Surface Plasmon Polaritons and Hyperbolic Phonon Polaritons on the Near-Field Radiative Heat Transfer Between Multilayer Graphene/hBN Structures

ABSTRACT Near-field radiative heat transfer (NFRHT) between multilayer graphene/hBN heterostructures has been demonstrated to exceed the blackbody limit due to the coupling mechanism of surface plasmon polaritons and hyperbolic phonon polaritons, opening the door to applications in thermal management, thermophotovoltaics, and nanoscale metrology. Recent studies have shown that adding vacuum layers within multilayer structures can effectively promote surface modes and thus enhance NFRHT. However, the influence of vacuum layers on NFRHT between multilayer graphene/hBN heterostructures has not been investigated. Moreover, the influence of vacuum layers on coupled resonance modes excited in multilayer structures is worth discussing. In this work, we study the NFRHT based on multilayer graphene/vacuum/hBN/vacuum structures. The results show that as the gap distance increases from 20 nm to 100 nm, the NFRHT of three-cell and six-cell configurations is enhanced, while that of unit-cell configuration is suppressed. The potential mechanism can be identified as the excitation of surface plasmon-phonon polaritons (SPPPs) and hyperbolic plasmon-phonon polaritons (HPPPs) in multilayer structures. The enhancement factor of the six-cell configurations is up to 4.82 when the gap distance is 80 nm. Moreover, the influences of the chemical potential of graphene and the layer thickness on the NFRHT are discussed. The interesting results in this work indicate the perspectives for future near-field research involving coupling of SPPPs and HPPPs, and shed new light on high-performance devices introducing vacuum layers based on near-field radiative heat transfer.

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Thermodynamic control the self-assembled formation of vertically aligned nanocomposite thin film

ABSTRACT Emergent exotic phenomena in the self-assembled process of vertically aligned nanocomposite (VAN) thin film remain under intensive studies. Insight exploration on the self-assembled formation from the combination of two different phases of materials is not only important to optimize the physical properties yields from those combined materials, but also open up a new avenue to discover new materials with the VAN system. In this work, the thermodynamic control of the self-assembled formation of BiFeO3-CoFe2O4 (BFO-CFO) VAN thin film has been confirmed by studying the effects of substrate temperature during the growth process by pulsed laser deposition (PLD) technique. The structural examination results on the samples, which were growing with various substrate temperatures highlight the importance of the thermodynamic factor to control the crystalline structure of BFO phase and CFO pillar size, which then affect the physical properties and further its practical applications. For instance, we can control the size of the CFO pillar using a temperature substrate to find appropriate spin magnetic switching in the CFO pillar for memory device applications. This study also sheds light on the relationship between thermodynamics and elastic strain energy on the formation of self-assembled matrix-pillars of the BFO-CFO VAN which is important for device fabrication.

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Elasto-Thermodiffusive Microtemperature Model Induced by a Mechanical Ramp-Type of Nanoscale Photoexcited Semiconductor

ABSTRACT In this study, a novel theoretical approach to describe thermo-optical elastic materials is proposed. This formulation offers insights into the relationship between plasma waves and thermomechanical waves when the microtemperature properties of semiconductor materials such as silicon are taken into account. The proposed model involves incorporating the concept of microtemperature effect according to photothermal (PT) excitation processes in nonlocal photo-thermoelasticity. The investigation of the electron-hole interaction concerning the elasto-thermodiffusion (ETD) theory in the context of thermoelastic (TD) and electronic (ED) deformation is the main focus of the work. The advanced model is utilized to analyze how the mechanical loading of ramp-like structures impacts the unrestricted nonlocality semiconductor material on a free outer plane. The Laplace transform approach in one-dimensional (1D) provides an analytical solution for main non-dimensional thermo-photo-elastic fields (the hole charge carrier field, the displacement (acoustic) wave, thermal wave, and plasma wave (carrier density). The primary fields in the Laplace domain are obtained analytically, and boundary conditions are established using a mechanical ramp type. Using a numerical inverse Laplace transform, full time domain solutions for the fundamental fields are obtained numerically according to the Riemann-sum approximation approach. The graphical representations illustrate and discuss the outcomes of the main physical fields.

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Subcooled Pool Boiling on Hierarchical Micro- and Nanostructure-Modified Copper Surfaces in HFE-7100 Dielectric Liquid

ABSTRACT Hierarchical surfaces comprised both microscale and nanoscale structures have been previously studied as a means of targeting multiple length scales to achieve superior pool boiling performance. However, preceding studies have focused almost exclusively on high surface tension working fluids, while technologically important low surface tension fluids have remained largely unexplored. Due to their significantly lower surface tension these liquids tend to push out the air trapped in surface cavities of the heating surface, resulting in fewer nucleation sites compared to the same surface in water at low to moderate superheats. Thus, developing effective surface modification techniques for pool boiling in dielectric liquids and understanding the multiphase physics behind them is a pressing need in order to overcome these performance limitations and accelerate their adoption. In this work, we utilize scalable manufacturing techniques to realize four separate surface types (planar, nanoscale-modified, microscale-modified, and hierarchical) and experimentally determine their respective pool boiling performance within the low surface tension commercial working fluid HFE-7100. A maximum heat transfer enhancement of 125% at 38 K of superheat was observed for the best performing samples, which interestingly were nanoscale-modified and not those of the hierarchical type. Visual observations via high-speed video analysis of vapor bubble behavior are utilized to explain the underlying multiphase physics as to why these samples performed so well and future directions for achieving surface optimization across multiple length scales.

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Refinement of Thermal Conduction-Based Dew Condensation Detection on Target Solid Surface by Galvanic Arrays Sensor Chip

ABSTRACT A reliable early detection of dew condensation can efficiently protect target solid surfaces from numerous negative effects such as surface fogging and corrosion. Achieving this goal beneficially requires a specially designed moisture sensor whose surface needs to be thermally identical with the target surface via a thermal conductor. However, the effect of the geometrical shape of the thermal conductor on the thermal conduction process is yet to be experimentally emphasized. In this study, we examined the potential detection of dew condensation events at our recently developed moisture sensor chip (MSC) under an effective control of its surface temperature via an attachment with Al-based thermal conductors. Precise and practical dew condensation detections were carried out in a multi-step and a one-step temperature-controlling modes, respectively. The experimental results revealed that the MSC response current (as a measure of dew condensation detection) increased when its surface temperature was dropped below the dew point. Moreover, the geometrical shape of thermal conductor attached to the backside of MSC can affect its thermal resistivity leading to a remarkable improvement in dew condensation detection. Therefore, it can be concluded that the geometrically designed thermal conductor can work effectively to minimize the temperature difference between MSC and target surface. This finding is believed to enable MSC to detect the target surface condition precisely in real time.

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Flow and Heat Transfer in Two-Phase Flow Immiscible Droplets in Microchannels

ABSTRACT The enhancement of heat transfer in microchannels without phase change is a significant area of study, primarily driven by the internal fluid recirculation in two-phase flows. This investigation focuses on a circular microchannel, 100 μm in diameter, where mineral oil droplets are introduced into a water flow. The study utilizes the conservative level set method for precise interface tracking and liquid film thickness measurement. This research introduces a modified Nusselt number, specifically tailored to describe the heat transfer characteristics of multiphase flows. The study delves into the effects of varying droplet sizes, from small spheres to a slug. The findings indicate that the most significant heat transfer enhancement occurs with droplets whose volume closely matches that of a sphere fitting within the channel. Moreover, the investigation explores the impact of parameters like inlet velocity, primary-phase slug length, and contact angle. Notably, higher inlet velocities lead to improved heat transfer, resulting in a substantial increase in the Nusselt number compared to single-phase flows. The study underscores the delicate balance between recirculation intensity and droplet heat capacity concerning slug length, as excessive variations can harm thermal performance. It also highlights the pivotal role of surface wettability, showing improved thermal performance on hydrophobic surfaces.

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MHD Mixed Convection of Developing Slip Flow in a Vertical Porous Microchannel Under Local Thermal Non–Equilibrium Conditions

ABSTRACT MHD mixed convection heat transfer of an ionized gas in a vertical microchannel filled with a porous medium is simulated and discussed in this study. The considered flow is hydrodynamically and thermally developing with Local Thermal Non – Equilibrium (LTNE) between the gas and the solid matrix. The Darcy – Brinkman – Forchheimer model is utilized to describe the flow filed in the porous medium. Moreover, both velocity – slip and temperature – jump boundary conditions are applied to the gas at the walls. The governing equations are solved by the finite – volume method. Results are presented and discussed in terms of the developed profiles of velocity and temperature of the constituents as well as the variations of the Nusselt number through the microchannel, the numerical values of the hydrodynamic and thermal entry lengths, and the fully – developed Nusselt number for different conditions. It is found that direct relations exist between the fully – developed Nusselt number and the Richardson number, the Reynolds number, the Hartmann number, the Biot number, the thermal conductivity ratio, and the Forchheimer number. With rise in the Knudsen number or the Darcy number, however, the Nusselt number deteriorates. The results indicate that the Knudsen number, the Hartmann number, the Biot number, and the thermal conductivity ratio are the most influential parameters on the fully – developed Nusselt number. It is envisaged that a tenfold increase in the Hartmann number and a hundredfold elevation in the Knudsen number are accompanied by 14% rise and 42% reduction in the fully – developed Nusselt number, respectively.

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Simultaneous Determination of Thermal Conductivity and Heat Capacity in Thin Films with Picosecond Transient Thermoreflectance and Picosecond Laser Flash

ABSTRACT Combining the picosecond transient thermoreflectance (ps-TTR) and picosecond laser flash (ps-LF) techniques, we have developed a novel method to simultaneously measure the thermal effusivity and the thermal diffusivity of metal thin films and determine the thermal conductivity () and the heat capacity () altogether. In order to validate our approach and evaluate the uncertainties, we analyzed five different metal films (Al, Cr, Ni, Pt, and Ti) with thicknesses ranging from 297 nm to 1.2 µm. Our results on thermal transport properties and heat capacity are consistent with reference values, with the uncertainties for the thermal conductivity and the heat capacity measurements below 25% and 15%, respectively. Compared with the ps-TTR technique alone, the combined approach substantially lowers the uncertainty of the thermal conductivity measurement. Uncertainty analyses on various materials show that this combined approach is capable of measuring most of the materials with a wide range of thicknesses, including those with low thermal conductivity (e.g., mica) down to thicknesses as small as 60 nm and ultrahigh thermal conductivity materials (such as cubic BAs) down to 1400 nm. Simultaneous measurement of thermal conductivity and heat capacity enables exploration of the thermal physical behavior of materials under various thermodynamic and mechanical perturbations, with potential applications in thermal management materials, solid-state phase transitions, and beyond.

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Effective Thermoelectric Switch of Hollow Weakly-Coupled Molecular Junction Based on Twist Angle Effect with Boron-Doping

ABSTRACT Rational design and adjustment of flexible thermoelectric devices are key points for sustainable and effective thermoelectric conversion, which remains a fundamental challenge due to inherent high thermal conductivity and uncontrolled carrier concentration induced by non-uniform dispersion. Under ingenious combination of weakly-coupled hollow interface and nanotube structure, thermoelectric performance of a dumbbell-like molecular junction comprised of a phenyl-terminated polyyne as central molecule and two semi-infinite 1D single-walled carbon nanotube (SWCNT) as electrodes has been investigated at certain twisted angles (θ). The results indicate that molecule twisting can be reviewed as an effective thermoelectric switch to coordinatingly control electronic and phononic transmission properties simultaneously. Resonance of molecular discrete state and electrode continuous state leads to low thermal conductance, which is sensitively affected by twist angle. Meanwhile, cyclic transformation between p-type and n-type flexible thermoelectrics can be realized by manipulating twist angle in a certain period of rotation. Thermoelectric performance of such a molecular junction can be further improved by boron atom doping at head-to-tail positions, and an excellent figure of merit (ZT = 1.75) is observed near Fermi level under 25° twisted angle. This result inspires an effective strategy to modulate and control thermoelectric conversion, which will greatly broaden applications in thermoelectric twistronics.

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An Investigation into the Roughness and Film Thickness Effects on the Interfacial Thermal Resistance

ABSTRACT The roughness and film thickness effects on the interfacial thermal resistance (ITR) are explored at two deliberately selected temperatures in use of Monte-Carlo simulation method. Particular methods are proposed to define properly the phonon emitting temperature based on the one-way deviational heat flux, and to define correctly the phonon equilibrium temperature by considering the different properties and residence times of incident, transmitted, and reflected phonons near an interface. A mixed mismatch model which allows polarization conversion is constructed and employed. The so-obtained traditional ITRs, defined based on the emitting temperature difference, and the revised ITRs, defined based on the equilibrium temperature difference, are compared with model predictions in the literature. Simulation results show that at high temperature the revised ITR decreases monotonically with increasing film thickness and at low temperature it possesses a local minimum against the interface roughness. The latter is explained by the monotonically increasing traditional ITR and monotonically decreasing ratio of the equilibrium temperature difference to emitting temperature difference with increasing roughness. Among all the studied models, only the newly proposed one can well predict the ITR for different interface roughness at low temperature. None of the models captures the monotonic decrease of ITR with film thickness at high temperature however.

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