Yields Of Fragments Research Articles

Simultaneous analysis of the elastic scattering and breakup channel for the reactionLi11+Pb208at energies near the Coulomb barrier

We present a detailed analysis of the elastic scattering and breakup channel for the reaction of Li-11 on Pb-208 at incident laboratory energies of 24.3 and 29.8 MeV, measured at the radioactive ion beam facility of TRIUMF, in Vancouver, Canada. A large yield of Li-9 fragments was detected by four charged particle telescopes in a wide angular range. The experimental angular and energy distributions of these Li-9 fragments have been compared to coupled-reaction-channel and continuum-discretized coupled-channel calculations. The large production of Li-9 fragments at small angles can be explained by considering a direct breakup mechanism, while at medium-large angles a competition between direct breakup and neutron transfer to the continuum of the Pb-208 target was observed.

γ-ray spectroscopy of fission fragments produced inPb208(O18,f)

Prompt gamma-ray spectroscopy of fission fragments produced in the heavy-ion induced fusion-fission reaction $^{208}\mathrm{Pb}(^{18}\mathrm{O},f)$ at $E=90$ MeV has been performed. The relative isotopic yields of the fission fragments and the fragment mass distribution have been studied. Structures in the mass distribution have been discussed in the light of earlier results. Relative yields of several odd-$A$ isotopes of Mo, Ru, Pd, and Cd and the odd-$A$ isotones with $N=62$ and 64 have been studied along with the yields of the neighboring even-$Z$, even-$N$ fragments and correlated to nuclear structural effects. The average total neutron multiplicity during fission has been measured to be $5.48\ifmmode\pm\else\textpm\fi{}0.59$. The level schemes of the two neutron-rich nuclei $^{110}\mathrm{Pd}$ and $^{116}\mathrm{Cd}$ have been studied from $\ensuremath{\gamma}$-ray triple coincidence data. A large number of transitions, previously reported only from $\ensuremath{\beta}$-decay studies, have been observed in $^{110}\mathrm{Pd}$ for the first time. The yrast band in $^{116}\mathrm{Cd}$ has been extended up to spin $({16}^{+})$. In addition, a rotational sequence built upon an excited ${5}^{\ensuremath{-}}$ state in $^{116}\mathrm{Cd}$ has been observed up to $({13}^{\ensuremath{-}})$. The level schemes have been discussed in the context of existing results, both experimental and theoretical, in the literature.

Novel technique to extract experimental symmetry free energy information for nuclear matter

A new method of accessing information on the symmetry free energy from yields of fragments produced in Fermi-energy heavy-ion collisions is proposed. Furthermore, by means of quantum fluctuation analysis techniques, correlations between extracted symmetry free energy coefficients with temperature and density were studied. The obtained results are consistent with those of commonly used isoscaling techniques.

Real-time fragmentation dynamics of clusters ionized by intense extreme-ultraviolet pulses

We investigate the fragmentation dynamics of atomic clusters ionized by intense extreme-ultraviolet pulses from a high-order harmonic generation source. It is demonstrated that the transient modification of the trimer fragment yield induced by a weak near-infrared (NIR) probe pulse provides valuable information on the cluster disintegration process. For medium-sized Ar clusters and delays of around 5 ps, we observe a transition from a collective response, where efficient absorption of the NIR laser energy takes place, to a state where the interaction of the probe laser pulse with individual fragments dominates. The cluster disintegration is faster for smaller clusters, in agreement with a simple physical picture taking into account the measured expansion speeds of excited and ionic fragments. For Xe clusters, we find a significantly increased fragmentation time of about 40 ps, attributed to the larger atomic mass and to more efficient electron–ion recombination processes.

Fission fragment mass distributions via prompt γ-ray spectroscopy

The distribution of fragment masses formed in nuclear fission is one of the most striking features of the process. Such measurements are very important to understand the shape evolution of the nucleus from ground state to scission through intermediate saddle points. The fission fragment mass distributions, generally obtained via conventional methods (i.e., by measuring the energy and/or the velocity of the correlated fission fragments) are limited to a mass resolution of 4–5 units. On the other hand, by employing the γ-ray spectroscopy, it is possible to estimate the yield of individual fission fragments. In this work, determination of the fission fragment mass distribution by employing prompt γ-ray spectroscopy is described along with the recent results on 238U(18O, f) and 238U(32S, f) systems.

Charge transfer and formation of complexes in the He+ collisions with the furan molecules

SynopsisCharge transfer and formation of the collision complexes have been studied experimentally in fragmentation of the furan molecules in collisions with He+ cations. The excited atomic and diatomic fragments of furan have been identified using collision-induced luminescence spectroscopy. Charge transfer ionization of the furan molecules has been observed in production of helium atoms in the excited 1s4d 1D2, 3D1,2,3 states. The fragmentation yields of the excited fragments have been measured as a function of the projectile energies (velocities) in the range 5-1000 eV. Enhancement of the fragmentation yields occurring at lower velocities may indicate formation of the [He-C4H4O]+ collision complexes prior to dissociation.

Fragmentation of tryptophan molecule by low-energy electron-impact

SynopsisThe fragmentation of a gas-phase tryptophan molecule by a low-energy (<70 eV) electron impact was studied both experimentally and theoretically. Various positively charged fragments have been observed and analyzed. A special attention is paid to the energy characteristics of the ionic fragment yield.

Modeling radiation-induced cell death: role of different levels of DNA damage clustering.

Some open questions on the mechanisms underlying radiation-induced cell death were addressed by a biophysical model, focusing on DNA damage clustering and its consequences. DNA "cluster lesions" (CLs) were assumed to produce independent chromosome fragments that, if created within a micrometer-scale threshold distance (d), can lead to chromosome aberrations following mis-rejoining; in turn, certain aberrations (dicentrics, rings and large deletions) were assumed to lead to clonogenic cell death. The CL yield and d were the only adjustable parameters. The model, implemented as a Monte Carlo code called BIophysical ANalysis of Cell death and chromosome Aberrations(BIANCA), provided simulated survival curves that were directly compared with experimental data on human and hamster cells exposed to photons, protons, α-particles and heavier ions including carbon and iron. d=5μm, independent of radiation quality, and CL yields in the range ~2-20CLsGy(-1)cell(-1), depending on particle type and energy, led to good agreement between simulations and data. This supports the hypothesis of a pivotal role of DNA cluster damage at sub-micrometric scale, modulated by chromosome fragment mis-rejoining at micrometric scale. To investigate the features of such critical damage, the CL yields were compared with experimental or theoretical yields of DNA fragments of different sizes, focusing on the base-pair scale (related to the so-called local clustering), the kbp scale ("regional clustering") and the Mbp scale, corresponding to chromatin loops. Interestingly, the CL yields showed better agreement with kbp fragments rather than bp fragments or Mbp fragments; this suggests that also regional clustering, in addition to other clustering levels, may play an important role, possibly due to its relationship with nucleosome organization in the chromatin fiber.

Energy dependence of the complexity of DNA damage induced by carbon ions.

To assess the complexity of DNA damage induced by carbon ions as a function of their energy and LET, 2-Gy irradiations by 100 keV u(-1)-400 MeV u(-1) carbon ions were investigated using the PARTRAC code. The total number of fragments and the yield of fragments of <30 bp were calculated. The authors found a particularly important contribution of DNA fragmentation in the range of <1 kbp for specific energies of <6 MeV u(-1). They also considered the effect of different specific energies with the same LET, i.e. before and after the Bragg peak. As a first step towards a full characterisation of secondary particle production from carbon ions interacting with tissue, a comparison between DNA-damage induction by primary carbon ions and alpha particles resulting from carbon break-up is presented, for specific energies of >1 MeV u(-1).

Yield estimation of neutron-rich rare isotopes induced by 200 MeV/u 132Sn beams by using GEANT4

A so-called “two-step reaction scheme”, in which neutron-rich rare isotopes obtained from ISOL are post-accelerated and bombarded on a second target, is employed to estimate the production yields of exotic rare isotopes. The production yields of neutron-rich rare isotope fragments induced by 200MeV/u 132Sn beams bombarded on a 9Be target are estimated with Monte Carlo code, GEANT4. To substantiate the use of GEANT4 for this study, benchmark calculations are done for 80MeV/u 59Co, 95MeV/u 72Zn, 500MeV/u 92Mo, and 950MeV/u 132Sn beams on the 9Be target. It is found that 132Sn beams can produce neutron-rich rare isotopes with 45⩽Z⩽50 more effectively than 238U beams at the same energy per nucleon.

Improvements and innovations in endoscopic ultrasound guided fine needle aspiration.

Keywords: Algorithm; Core histology needle; Cytology; Endoscopic ultrasound guided fine needle aspiration fine needle biopsy; Histology

Fragmentation of tetrahydrofuran molecules by H(+), C(+), and O(+) collisions at the incident energy range of 25-1000 eV.

We have studied fragmentation processes of the gas-phase tetrahydrofuran (THF) molecules in collisions with the H(+), C(+), and O(+) cations. The collision energies have been varied between 25 and 1000 eV and thus covered a velocity range from 10 to 440 km/s. The following excited neutral fragments of THF have been observed: the atomic hydrogen H(n), n = 4-9, carbon atoms in the 2p3s (1)P1, 2p4p (1)D2, and 2p4p (3)P states and vibrationally and rotationally excited diatomic CH fragments in the A(2)Δ and B(2)Σ(-) states. Fragmentation yields of these excited fragments have been measured as functions of the projectile energy (velocity). Our results show that the fragmentation mechanism depends on the projectile cations and is dominated by electron transfer from tetrahydrofuran molecules to cations. It has been additionally hypothesized that in the C(+)+THF collisions a [C-C4H8O](+) complex is formed prior to dissociation. The possible reaction channels involved in fragmentation of THF under the H(+), C(+), and O(+) cations impact are also discussed.

Dynamics of the A-band ultraviolet photodissociation of methyl iodide and ethyl iodide via velocity-map imaging with 'universal' detection.

We report data from a comprehensive investigation into the photodissociation dynamics of methyl iodide and ethyl iodide at several wavelengths in the range 236-266 nm, within their respective A-bands. The use of non-resonant single-photon ionization at 118.2 nm allows detection and velocity-map imaging of all fragments, regardless of their vibrotational or electronic state. The resulting photofragment kinetic energy and angular distributions and the quantum yields of ground-state and spin-orbit excited iodine fragments are in good agreement with previous studies employing state-selective detection via REMPI. The data are readily rationalised in terms of three competing dissociation mechanisms. The dominant excitation at all wavelengths studied is via a parallel transition to the (3)Q0 state, which either dissociates directly to give an alkyl radical partnered by spin-orbit excited iodine, or undergoes radiationless transfer to the (1)Q1 potential surface, where it dissociates to an alkyl radical partnered by iodine in its electronic ground state. Ground state iodine atoms can also be formed by direct dissociation from the (1)Q1 or (3)Q1 excited states following perpendicular excitation at the shorter and longer wavelength region, respectively, in the current range of interest. The extent of internal excitation of the alkyl fragment varies with dissociation mechanism, and is considerably higher for ethyl fragments from ethyl iodide photolysis than for methyl fragments from methyl iodide photolysis. We discuss the relative advantages and disadvantages of single-photon vacuum-ultraviolet ionization relative to the more widely used REMPI detection schemes, and conclude, in agreement with others, that single-photon ionization is a viable detection method for photofragment imaging studies, particularly when studying large molecules possessing multiple fragmentation channels.

Some Dynamical Features of Molecular Fragmentation by Electrons and Swift Ions

To date, the large majority of studies on molecular fragmentation by swift charged particles have been carried out using simple molecules, for which reliable Potential Energy Curves are available to interpret the measured fragmentation yields. For complex molecules the scenario is quite different and such guidance is not available, obscuring even a simple organization of the data which are currently obtained for a large variety of molecules of biological or technological interest. In this work we show that a general and relatively simple methodology can be used to obtain a broader picture of the fragmentation pattern of an arbitrary molecule. The electronic ionization or excitation cross section of a given molecular orbital, which is the first part of the fragmentation process, can be well scaled by a simple and general procedure at high projectile velocities. The fragmentation fractions arising from each molecular orbital can then be achieved by matching the calculated ionization with the measured fragmentation cross sections. Examples for Oxygen, Chlorodifluoromethane and Pyrimidine molecules are presented.

Electron-impact-induced tryptophan molecule fragmentation

The fragmentation of a gas-phase tryptophan molecule by a low-energy (<70 eV) electron impact was studied both experimentally and theoretically. Various positively charged fragments were observed and analyzed. A special attention was paid to the energy characteristics of the ionic fragment yield. The geometrical parameters of the initial molecule rearrangement were also analyzed. The fragmentation observed was due to either a simple bond cleavage or more complex reactions involving molecular rearrangements.

Systematic study of neutron-rich rare isotope production in peripheral heavy-ion collisions below the Fermi energy

Detailed calculations of the yields of projectilelike fragments (with focus on the neutron-rich isotopes) are presented for the interaction of $^{86}\mathrm{Kr}$ (15 MeV/nucleon) with $^{64}\mathrm{Ni}$, $^{58}\mathrm{Ni}$, and $^{124}\mathrm{Sn}$, $^{112}\mathrm{Sn}$, as well as $^{86}\mathrm{Kr}$ (25 MeV/nucleon) with $^{124}\mathrm{Sn}$ and compared with our recently published experimental data for these reactions. The calculations are based on a two-step approach: the dynamical stage of the collision was described with the microscopic constrained molecular dynamics (CoMD) model, as well as the phenomenological deep-inelastic transfer (DIT) model and its modified (DITm) version. The deexcitation of the hot projectile fragments was performed with the statistical multifragmentation model (SMM) and the binary-decay model gemini, which provided nearly similar results for the neutron-rich products from the reactions studied. An overall good agreement of the calculations with the experimental results, especially for near-projectile isotopes was observed using both the CoMD model and the DITm model for the dynamical stage. The successful description of the production of neutron-rich isotopes with the CoMD model is of particular importance, due to the predictive power of the microscopic approach that essentially does not depend on the reaction dynamics. Our studies to date suggest that peripheral heavy-ion collisions at this energy range (i.e., well above the Coulomb barrier, but below the Fermi energy), if induced by neutron-rich rare-isotope beams of adequate intensity may offer a unique route to access extremely neutron-rich rare isotopes toward the astrophysical $r$-process path and the presently uncharted neutron drip line.

Assessment of optimal control mechanism complexity by experimental landscape Hessian analysis: fragmentation of CH2BrI

Optimally shaped femtosecond laser pulses can often be effectively identified in adaptive feedback quantum control experiments, but elucidating the underlying control mechanism can be a difficult task requiring significant additional analysis. We introduce landscape Hessian analysis (LHA) as a practical experimental tool to aid in elucidating control mechanism insights. This technique is applied to the dissociative ionization of CH2BrI using shaped fs laser pulses for optimization of the absolute yields of ionic fragments as well as their ratios for the competing processes of breaking the C–Br and C–I bonds. The experimental results suggest that these nominally complex problems can be reduced to a low-dimensional control space with insights into the control mechanisms. While the optimal yield for some fragments is dominated by a non-resonant intensity-driven process, the optimal generation of other fragments maa difficult task requiring significant additionaly be explained by a non-resonant process coupled to few level resonant dynamics. Theoretical analysis and modeling is consistent with the experimental observations.

Status and prospects of investigations into the collinear cluster decay of heavy nuclei

Basic experimental results confirming the existence a new cluster-decay type called collinear cluster tripartition (CCT) are presented. Decays of this type manifest themselves, in particular, as a two-dimensional region of a locally enhanced yield of fragments (bump) that corresponds to specific missing-mass values in the mass-mass distribution of fission fragments. One of the decay modes that contribute to the bump can be treated as a cluster-decay type that is new in relation to the well-known heavy-ion or lead radioactivity. The conclusions drawn from an analysis of correlation mass distributions are confirmed by the results obtained from neutron-gated data, measurements of the nuclear charge for CCT events, and the direct detection of new-decay products.

Xylan hydrolysis in Populus trichocarpa × P. deltoides and model substrates during hydrothermal pretreatment

Previous studies defined easy and difficult to hydrolyze fractions of hemicellulose that may result from bonds among cellulose, hemicellulose, and lignin. To understand how such bonds affect hydrolysis, Populus trichocarpa×Populus deltoides, holocellulose isolated from P.trichocarpa×P. deltoides and birchwood xylan were subjected to hydrothermal flow-through pretreatment. Samples were characterized by glycome profiling, HPLC, and UPLC–MS. Glycome profiling revealed steady fragmentation and removal of glycans from solids during hydrolysis. The extent of polysaccharide fragmentation, hydrolysis rate, and total xylose yield were lowest for P.trichocarpa×P. deltoides and greatest for birchwood xylan. Comparison of results from P.trichocarpa×P. deltoides and holocellulose suggested that lignin–carbohydrate complexes reduce hydrolysis rates and limit release of large xylooligomers. Smaller differences between results with holocellulose and birchwood xylan suggest xylan–cellulose hydrogen bonds limited hydrolysis, but to a lesser extent. These findings imply cell wall structure strongly influences hydrolysis.

Carbon ion fragmentation effects on the nanometric level behind the Bragg peak depth

In this study, fragmentation yields of carbon therapy beams are estimated using the Geant4 simulation toolkit version 9.5. Simulations are carried out in a step-by-step mode using the Geant4-DNA processes for each of the major contributing fragments. The energy of the initial beam is taken 400 MeV amu−1 as this is the highest energy, which is used for medical accelerators and this would show the integral role of secondary contributions in radiotherapy irradiations. The obtained results showed that 64% of the global dose deposition is initiated by carbon ions, while up to 36% is initiated by the produced fragments including all their isotopes. The energy deposition clustering yields of each of the simulated fragments are then estimated using the DBSCAN clustering algorithm and they are compared to the yields of the incident primary beam.