X-ray Facilities Research Articles

Orbital Decay in an Accreting and Eclipsing 13.7 Minute Orbital Period Binary with a Luminous Donor

We report the discovery of ZTF J0127+5258, a compact mass-transferring binary with an orbital period of 13.7 minutes. The system contains a white dwarf accretor, which likely originated as a post–common envelope carbon–oxygen (CO) white dwarf, and a warm donor (T eff,donor = 16,400 ± 1000 K). The donor probably formed during a common envelope phase between the CO white dwarf and an evolving giant that left behind a helium star or white dwarf in a close orbit with the CO white dwarf. We measure gravitational wave–driven orbital inspiral with ∼51σ significance, which yields a joint constraint on the component masses and mass transfer rate. While the accretion disk in the system is dominated by ionized helium emission, the donor exhibits a mixture of hydrogen and helium absorption lines. Phase-resolved spectroscopy yields a donor radial velocity semiamplitude of 771 ± 27 km s−1, and high-speed photometry reveals that the system is eclipsing. We detect a Chandra X-ray counterpart with L X ∼ 3 × 1031 erg s−1. Depending on the mass transfer rate, the system will likely either evolve into a stably mass-transferring helium cataclysmic variable, merge to become an R CrB star, or explode as a Type Ia supernova in the next million years. We predict that the Laser Space Interferometer Antenna (LISA) will detect the source with a signal-to-noise ratio of 24 ± 6 after 4 yr of observations. The system is the first LISA-loud mass-transferring binary with an intrinsically luminous donor, a class of sources that provide the opportunity to leverage the synergy between optical and infrared time domain surveys, X-ray facilities, and gravitational-wave observatories to probe general relativity, accretion physics, and binary evolution.

A Tight Correlation between Millimeter and X-Ray Emission in Accreting Massive Black Holes from

Recent studies have proposed that the nuclear millimeter continuum emission observed in nearby active galactic nuclei (AGNs) could be created by the same population of electrons that gives rise to the X-ray emission that is ubiquitously observed in accreting black holes. We present the results of a dedicated high-spatial-resolution (∼60–100 mas) Atacama Large Millimeter/submillimeter Array (ALMA) campaign on a volume-limited (<50 Mpc) sample of 26 hard X-ray (>10 keV) selected radio-quiet AGNs. We find an extremely high detection rate (25/26 or ), which shows that nuclear emission at millimeter wavelengths is nearly ubiquitous in accreting SMBHs. Our high-resolution observations show a tight correlation between the nuclear (1–23 pc) 100 GHz and the intrinsic X-ray emission (1σ scatter of 0.22 dex). The ratio between the 100 GHz continuum and the X-ray emission does not show any correlation with column density, black hole mass, Eddington ratio, or star formation rate, which suggests that the 100 GHz emission can be used as a proxy of SMBH accretion over a very broad range of these parameters. The strong correlation between 100 GHz and X-ray emission in radio-quiet AGNs could be used to estimate the column density based on the ratio between the observed 2–10 keV () and 100 GHz (F 100 GHz) fluxes. Specifically, a ratio strongly suggests that a source is heavily obscured (). Our work shows the potential of ALMA continuum observations to detect heavily obscured AGNs (up to an optical depth of one at 100 GHz, i.e., N H ≃ 1027 cm−2), and to identify binary SMBHs with separations <100 pc, which cannot be probed by current X-ray facilities.

Synchrotron science for sustainability: life cycle of metals in the environment.

The movement of metals through the environment links together a wide range of scientific fields: from earth sciences and geology as weathering releases minerals; to environmental sciences as metals are mobilized and transformed, cycling through soil and water; to biology as living things take up metals from their surroundings. Studies of these fundamental processes all require quantitative analysis of metal concentrations, locations, and chemical states. Synchrotron X-ray tools can address these requirements with high sensitivity, high spatial resolution, and minimal sample preparation. This perspective describes the state of fundamental scientific questions in the lifecycle of metals, from rocks to ecosystems, from soils to plants, and from environment to animals. Key X-ray capabilities and facility infrastructure for future synchrotron-based analytical resources serving these areas are summarized, and potential opportunities for future experiments are explored.

Mock X-Ray Observations of Hot Gas with L-Galaxies Semi-analytic Models of Galaxy Formation

We create mock X-ray observations of hot gas in galaxy clusters with a new extension of the L-Galaxies semi-analytic model of galaxy formation, which includes the radial distribution of hot gas in each halo. Based on the model outputs, we first build some mock light cones, then generate mock spectra with the SOXS package and derive the mock images in the light cones. Using the mock data, we simulate mock X-ray spectra for the ROSAT all-sky survey, and compare the mock spectra with the observational results. Then, we consider the design parameters of the HUBS mission and simulate the observation of the halo hot gas for HUBS as an important application of our mock work. We find: (1) our mock data match the observations by current X-ray telescopes. (2) The survey of hot baryons in resolved clusters by HUBS is effective below redshift 0.5, and the observations of the emission lines in point-like sources at z > 0.5 by HUBS help us understand the hot baryons in the early universe. (3) By taking advantage of the large simulation box and flexibility in semi-analytic models, our mock X-ray observations provide the opportunity to select targets and observation strategies for forthcoming X-ray facilities.

Selected advances in small-angle scattering and applications they serve in manufacturing, energy and climate change.

Innovations in small-angle X-ray and neutron scattering (SAXS and SANS) at major X-ray and neutron facilities offer new characterization tools for researching materials phenomena relevant to advanced applications. For SAXS, the new generation of diffraction-limited storage rings, incorporating multi-bend achromat concepts, dramatically decrease electron beam emittance and significantly increase X-ray brilliance over previous third-generation sources. This results in intense X-ray incident beams that are more compact in the horizontal plane, allowing significantly improved spatial resolution, better time resolution, and a new era for coherent-beam SAXS methods such as X-ray photon correlation spectroscopy. Elsewhere, X-ray free-electron laser sources provide extremely bright, fully coherent, X-ray pulses of <100 fs and can support SAXS studies of material processes where entire SAXS data sets are collected in a single pulse train. Meanwhile, SANS at both steady-state reactor and pulsed spallation neutron sources has significantly evolved. Developments in neutron optics and multiple detector carriages now enable data collection in a few minutes for materials characterization over nanometre-to-micrometre scale ranges, opening up real-time studies of multi-scale materials phenomena. SANS at pulsed neutron sources is becoming more integrated with neutron diffraction methods for simultaneous structure characterization of complex materials. In this paper, selected developments are highlighted and some recent state-of-the-art studies discussed, relevant to hard matter applications in advanced manufacturing, energy and climate change.

A sensitive high repetition rate arrival time monitor for X-ray free electron lasers

X-ray free-electron laser sources enable time-resolved X-ray studies with unmatched temporal resolution. To fully exploit ultrashort X-ray pulses, timing tools are essential. However, new high repetition rate X-ray facilities present challenges for currently used timing tool schemes. Here we address this issue by demonstrating a sensitive timing tool scheme to enhance experimental time resolution in pump-probe experiments at very high pulse repetition rates. Our method employs a self-referenced detection scheme using a time-sheared chirped optical pulse traversing an X-ray stimulated diamond plate. By formulating an effective medium theory, we confirm subtle refractive index changes, induced by sub-milli-Joule intense X-ray pulses, that are measured in our experiment. The system utilizes a Common-Path-Interferometer to detect X-ray-induced phase shifts of the optical probe pulse transmitted through the diamond sample. Owing to the thermal stability of diamond, our approach is well-suited for MHz pulse repetition rates in superconducting linear accelerator-based free-electron lasers.

Assessment of staff of radiology department annual effective doses during bone scans

Background: The most frequent imaging techniques used by NM departments are skeletal scintigraphy and bone scans. To assess the protective measures and the anticipated radiation hazards, it is crucial to evaluate the patient's doses for the NMC staff. Objectives: Current research intended to evaluate the annual effective doses of radiology department’s staff during bone scans and their health hazards due to radiation. Methods: The study was executed at Nuclear Medical Center, in October 2022 and annual effective dose of radiologists were measured implying the two techniques including 99mTc-MDP TLDs, carrying two dose quantities of Hp (10) and Hp (0.07) and GR-200A TLDs (LiF: Mg, Cu, P). Results: Effective dose of operators was evaluated using 99mTc-MDP TLDs, was found that the mean personal equivalent dosimetry of HP 10 was 0.43 (0.12-0.74) and HP 0.07 was 0.52 (0.11-0.76). Relative strength of residual signal for successive readouts of LiF: Mg, Cu, P chips made had mean GR-200A and Ref. 10 of 0.54+0.23 and 3.10+1.12, respectively. Conclusion: The radiographers in all of the X-ray facilities were well aware of radiation safety and the staff's occupational dosages of HP(0.07) and HP (10) were within the recommended limits.

Design and performance of the camera of the Micro-channel X-ray Telescope on-board the SVOM mission

The Microchannel X-ray Telescope (MXT) is part of the scientific payload of the SVOM Sino-French space mission to observe the early afterglow of gamma-ray bursts in the 0.2–10 keV energy range and localize them within 2 arcmin. For a total mass of 42 kg and a total power of 60 W, this instrument is composed of an optical system, a structural carbon fiber tube, a radiator, a camera and a data processing unit. The camera consists of a focal plane assembly with a detector ceramic board and thermoelectric coolers, a front-end electronics, a calibration wheel and a support structure. Spectral characterization tests of the focal plane assembly based on a 256 × 256 pixel pnCCD spectroscopic imager were performed in the laboratory, at the Metrology beamline of the SOLEIL synchrotron and at the PANTER X-ray facility. Energy resolution of 79 eV FWHM at 1.5 keV was demonstrated in the nominal flight configuration (−65 °C, real time event selection by the camera). The paper presents the design, the realization and the performance of the flight camera of MXT. It focuses on the technical challenges, the original implemented solutions and the custom-made setups for the validation tests.

Shielding Adequacy of Conventional X-ray Facilities in Kano Metropolis, Nigeria using RadShield Software

Over time x-ray department gains more patient throughput compared to when it was established, this may lead to changes in room usage, workload and occupancy factor. Therefore, it becomes imperative to re-evaluate the shielding adequacy of the facilities to ensure the appropriate shielding design goal is accomplished. The study was aimed at assessing the shielding adequacy of conventional x-ray rooms in ten radio diagnostic centres in Kano Metropolis using RADSHIELD software. This was a prospective, cross-sectional study. RadShield software version 1.1 was used in the study, parameters such as distances of each wall from a radiation source (D), the average number of patients per week (N), occupancy factor (T), and use factor (U) were inserted into the software together with the shielding design goal (P). Once the result was generated, the design and shielding variables were saved in .xml format. The data were analyzed using Excel 2016. Ten facilities were studied involving 14 x-ray rooms. Room III had the largest room size of 49.2 m2 while room X had the least room size of 12.8 m2. Room II had the longest source image distance (SOD) of 180cm while room IV had the shortest (120cm). The design barrier thickness was thickest (47 cm) in room II and thinnest (1.5 cm) in barrier 5 of room III. All the x-ray rooms had the ideal room size except facilities G and H. The design barrier thickness in the radiology department of all the conventional x-ray rooms involved in the study was adequate.

Sensitivity, Specificity and Predictive Values of Chest Indrawing in the Diagnosis of Severe Pneumonia

Background: Pneumonia is a recognized leading killer disease in under 5 children not only in Bangladesh but also in all developing countries. The presence of lower chest indrawing means that the child has severe pneumonia. This study aimed to determine the sensitivity, specificity and predictive values of chest indrawing in the diagnosis of severe pneumonia. Methods: This analytical study was conducted in the department of pediatrics, Sher-e-Bangla Medical College Hospital, Barisal, from January 2015 to December 2015. A total of 100 cases of severe pneumonia aged from 2 months to 5 years and similar numbers of suitably matched controls who fulfilled inclusion criteria were enrolled in this study. A detailed history was taken, a thorough physical examination was done, data were recorded in a preformed questionnaire and were analyzed using a scientific calculator. Results: Out of 100 cases, 80 (80%) and 100 controls, 72 (72%) were in the age group of 2 months to 1 year. Fast breathing was present in 98 (98%) cases and 88 (88%) controls. Chest indrawing was present in 56 (56%) cases and 42 (42%) controls. Roentgenographically, 44 (44%) cases revealed labor/segmental consolidation, and bilateral patchy consolidation was present in 56 (56%) cases. Among the control group, 28 (28%) patients had hyperlucency of peripheral lung fields in their chest X-rays. In this study, it was found that sensitivity, specificity, positive predictive value (PPV) and negative predictive value (NPV) of chest indrawing in the diagnosis of severe pneumonia was 56%, 58%, 57.1% and 56.8% respectively. Conclusion: Chest indrawing alone is not a highly sensitive tool to predict severe pneumonia but in rural areas where X-ray facilities are not available, chest indrawing may play an important role in identifying children with possible severe pneumonia. Mediscope 2022;9(2): 54-59

Novel fabrication tools for dynamic compression targets with engineered voids using photolithography methods

Mesoscale imperfections, such as pores and voids, can strongly modify the properties and the mechanical response of materials under extreme conditions. Tracking the material response and microstructure evolution during void collapse is crucial for understanding its performance. In particular, imperfections in the ablator materials, such as voids, can limit the efficiency of the fusion reaction and ultimately hinder ignition. To characterize how voids influence the response of materials during dynamic loading and seed hydrodynamic instabilities, we have developed a tailored fabrication procedure for designer targets with voids at specific locations. Our procedure uses SU-8 as a proxy for the ablator materials and hollow silica microspheres as a proxy for voids and pores. By using photolithography to design the targets' geometry, we demonstrate precise and highly reproducible placement of a single void within the sample, which is key for a detailed understanding of its behavior under shock compression. This fabrication technique will benefit high-repetition rate experiments at x-ray and laser facilities. Insight from shock compression experiments will provide benchmarks for the next generation of microphysics modeling.

Leveraging Advanced X-ray Imaging for Sustainable Battery Design

With the growing demand for sustainable battery technologies, state-of-the-art characterization techniques become more and more critical for optimizing battery materials and uncovering their operation mechanisms. In this Review, we mainly focus on X-ray imaging techniques and the associated applications in obtaining insights into the physicochemical properties and quantitative changes of battery materials. Given the high-energy nature of X-rays, operando/in situ imaging studies have emerged as a unique method to enable researchers to investigate a variety of battery chemistries during battery cycling. Such a cutting-edge characterization tool is expected to advance the understanding of electrochemically driven heterogeneous reactions, involving the structure, chemistry, and morphology, as well as the interface. Mechanistic explanations are comprehensively provided to understand the close relationship between battery failure and electro-chemo-mechanical degradation in the electrode. We expect that the use of large-scale X-ray facilities can lead to major developments in sustainable batteries and benefit the whole materials science community.

First light of BEaTriX, the new testing facility for the modular X-ray optics of the ATHENA mission

Aims. The Beam Expander Testing X-ray facility (BEaTriX) is a unique X-ray apparatus now operated at the Istituto Nazionale di Astrofisica (INAF), Osservatorio Astronomico di Brera (OAB), in Merate, Italy. It has been specifically designed to measure the point spread function (PSF) and the effective area (EA) of the X-ray mirror modules (MMs) of the Advanced Telescope for High-ENergy Astrophysics (ATHENA), based on silicon pore optics (SPO) technology, for verification before integration into the mirror assembly. To this end, BEaTriX generates a broad, uniform, monochromatic, and collimated X-ray beam at 4.51 keV. The beam collimation is better than a few arcseconds, ensuring reliable tests of the ATHENA MMs, in their focus at a 12 m distance. Methods. In BEaTriX, a micro-focus X-ray source with a titanium anode is placed in the focus of a paraboloidal mirror, which generates a parallel beam. A crystal monochromator selects the 4.51 keV line, which is expanded to the final size by a crystal asymmetrically cut with respect to the crystalline planes. An in-house-built Hartmann plate was used to characterize the X-ray beam divergence, observing the deviation of X-ray beams from the nominal positions, on a 12-m-distant CCD camera. After characterization, the BEaTriX beam has the nominal dimensions of 170 mm × 60 mm, with a vertical divergence of 1.65 arcsec and a horizontal divergence varying between 2.7 and 3.45 arcsec, depending on the monochromator setting: either high collimation or high intensity. The flux per area unit varies from 10 to 50 photons s−1 cm−2 from one configuration to the other. Results. The BEaTriX beam performance was tested using an SPO MM, whose entrance pupil was fully illuminated by the expanded beam, and its focus was directly imaged onto the camera. The first light test returned a PSF and an EA in full agreement with expectations. As of today, the 4.51 keV beamline of BEaTriX is operational and can characterize modular X-ray optics, measuring their PSF and EA with a typical exposure of 30 min. Another beamline at 1.49 keV is under development and will be integrated into the current equipment. We expect BEaTriX to be a crucial facility for the functional test of modular X-ray optics, such as the SPO MMs for ATHENA.

Patient-reported outcomes after initial conservative fracture treatment in primary healthcare – a survey study

BackgroundPrimary healthcare in Norway has first-line responsibility for medical emergencies, including traumas and fractures. Normally, patients with suspected fractures are referred to specialist care. However, some municipalities have X-ray facilities and handle minor fractures locally. We investigated patient-reported outcome measures after initial treatment of radiologically diagnosed fractures of the wrist, collarbone, and ankle at a primary healthcare centre in a rural municipality with a large ski resort. The patients’ general satisfaction with the treatment was also investigated.MethodsValidated questionnaires were sent to patients with fractures of the wrist or collarbone (Quick DASH—Disability of Arm, Shoulder and Hand) or the ankle (FAOS -The Foot and Ankle Outcome Score). Patients with wrist and collarbone fractures also answered the Quality-of-life questions that are a subscale of the FAOS questionnaire for ankle fractures. Patient satisfaction was measured for all fracture groups. The Quick DASH scale ranges from 0 (no disability at all) to 100 (great disability), while for FAOS a score of 100 indicates no symptoms and 0 indicates extreme disabilities.ResultsA total of 148 of 238 patients answered the questionnaire (62% response rate). Patients with distal radius fractures had a mean Quick DASH score of 5.1 (median 0, range 0–77), and scores were significantly lower for males (p = 0.013) and increased with age (p = 0.024). Patients with collarbone fractures had a mean Quick DASH score of 2.1 (median 0, range 0–32) with no significant age or gender differences. Patients with ankle fractures had the following mean subscale-scores: Pain, 93.8; Symptoms, 71.4; Activities of daily living, 97.4; Sport, 90.0; and Quality of life, 92.1. The scores did not differ significantly by specialization of the physician. A total of 88% of the patients were highly or very highly satisfied with the handling of their fracture.ConclusionsThe patients reported low rates of functional disability and high rates of satisfaction after initial radiological diagnosis and treatment of their fracture at the primary healthcare centre. Specialisation of the treating physician was not associated with the outcome in any of the fracture types.

Assessment of Diagnostic Radiology Facilities Technical Radiation Protection Requirements in KSA

The national regulatory body in the state regulates the source of ionizing radiation such as diagnostic radiology to minimize exposure to the operators and the patients. The Saudi Food and Drug Authority (KSA-SFDA) cover all medical regulatory aspects of ionizing radiation such as diagnostic X-ray facilities for all practices and intervention requirements. The study presents an assessment and analysis of the level of technical radiation protection requirements and the status of applying the national regulatory standards for different diagnostic facilities in KSA. Based on the online scientific recent database published in the field of radiation protection regulations and dose assessment for diagnostic radiology in KSA, and from the data published by the KSA-SFDA report in 2015. About 109 diagnostic X-ray facilities were selected from 35 governorates distributed in the kingdom. More than 95% of the examined facilities were in good condition concerning the national radiological protection technical regulation. About 11.9% of the facilities had a radiation leakage or cracks in the wall of the X-ray room/entrance door of the room. 16.5% of the facilities did not have a radiation warning sign written in Arabic/English languages. About 21.9% of the operators did not use any personal radiation dosimeter such as TLD or OSL. More than 40.7% of those facilities do not keep a record of the personal dosimeter reading at their facilities. Only 11.1% of the examined facilities do not have any personal protective tools such as a lead apron or thyroid shield. About 38.2% of the examined facilities do not carry out the annual periodic maintenance for the used X-ray machines at those facilities. From the obtained results, it was concluded that the majority of the radiation protection, radiation safety requirements and physical security measures undertaken in these facilities were in good implementation of the national and international technical regulations. The study suggests a need to apply for a quality control test procedures program regularly at those facilities.

Feasibility Analysis of Sapphire Compound Refractive Lenses for Advanced X-Ray Light Sources

The compound refractive lens (CRL) is a commonly used X-ray optical component for photon beam conditioning and focusing on the beamlines of the X-ray facilities. The normal preparation materials are beryllium, aluminum, silicon of current lenses, and they all suffered from high heat load fatigue and short pulse damage risks. Hard materials based CRL is engaged attention for the advanced X-ray application. Sapphire crystal has the advantages of high density, high melting point, low thermal expansion coefficient. In this paper, properties of the refraction and absorption ratio of Sapphire and parameters of Sapphire lenses of effective aperture, transmittance, resolution, number of lenses needed for a certain focus, are taken into account for the CRL design, comparing with those of several common materials as well. The calculation results show that the performance of the sapphire lens is better than that of the aluminum lens and silicon lens, and inferior to that of the beryllium lens and diamond lens, but the number of lenses used is less. In the meantime, performances of sapphire lenses focusing are simulated and thermal effects on lenses are analyzed. Analysis and discussion are carried out under the same conditions as the metal Aluminum ones. The focusing simulation shows that the sapphire lenses can obtain a smaller spot with more intensity. The thermal analysis indicates that the temperature during use of the sapphire lens is much lower than the melting point of sapphire, and the thermal deformation is negligible.

Harnessing interpretable and unsupervised machine learning to address big data from modern X-ray diffraction

The information content of crystalline materials becomes astronomical when collective electronic behavior and their fluctuations are taken into account. In the past decade, improvements in source brightness and detector technology at modern X-ray facilities have allowed a dramatically increased fraction of this information to be captured. Now, the primary challenge is to understand and discover scientific principles from big datasets when a comprehensive analysis is beyond human reach. We report the development of an unsupervised machine learning approach, X-ray diffraction (XRD) temperature clustering (X-TEC), that can automatically extract charge density wave order parameters and detect intraunit cell ordering and its fluctuations from a series of high-volume X-ray diffraction measurements taken at multiple temperatures. We benchmark X-TEC with diffraction data on a quasi-skutterudite family of materials, (CaxSr[Formula: see text])3Rh4Sn13, where a quantum critical point is observed as a function of Ca concentration. We apply X-TEC to XRD data on the pyrochlore metal, Cd2Re2O7, to investigate its two much-debated structural phase transitions and uncover the Goldstone mode accompanying them. We demonstrate how unprecedented atomic-scale knowledge can be gained when human researchers connect the X-TEC results to physical principles. Specifically, we extract from the X-TEC-revealed selection rules that the Cd and Re displacements are approximately equal in amplitude but out of phase. This discovery reveals a previously unknown involvement of [Formula: see text] Re, supporting the idea of an electronic origin to the structural order. Our approach can radically transform XRD experiments by allowing in operando data analysis and enabling researchers to refine experiments by discovering interesting regions of phase space on the fly.

Коррекция аппаратурного спектра CdTe-детектора в области рентгеновского излучения с граничной энергией до 150 кэВ

The article devotes to algorithm for the instrumental spectrum correction of a CdTe detector in the low-energy X-ray region with a cutoff energy &lt; 150 keV. By minimizing the influence of the detector’s response function, the algorithm allows the instrumental spectrum to be reconstructed, approaching its shape closer to the true one. Particular attention is paid to the low-energy region with the boundary energy up to 100 keV. For a given region, the algorithm makes it possible to correct the spectrum taking into account the difference between the theoretical efficiency curve and the modeled efficiency curve. The main goal of developing an improved algorithm is to determine the characteristics of the radiation quality of an X-ray facility.

Temperature dependence of luminescence characteristics of LYSO:Ce scintillator under x-ray excitation

Temperature dependence of the luminescence characteristics of Lu1.84Y0.16SiO5:Ce (LYSO:Ce) scintillator was investigated under x-ray excitation. The luminescence decay time, light yield, radioluminescence (RL) spectra, spatial resolution, and luminescence homogeneity from 300 to 550 K are experimentally examined with multiple x-ray facilities. The results show that the decay time and light output of the LYSO:Ce scintillator will decrease from 42 to 1.89 ns and from 32 000 to 1120 photons/MeV with a temperature increase from 300 to 550 K, respectively. The RL spectrum experiments demonstrate that the spectrum peak will move from 414 to 426 nm when adjusting the temperature from 300 to 550 K. The spatial resolution experiments show that the spatial resolution is hardly affected and can reach as high as 2.5 lp/mm when increasing the temperature from 300 to 550 K, and the luminescence homogeneity remains unchanged with increase in temperature. The experimental results provide important information for the radiation imaging application of the LYSO:Ce scintillator.

Development of an operando characterization stage for multi-modal synchrotron x-ray experiments.

It is widely accepted that micro- and nanoscale inhomogeneities govern the performance of many thin-film solar cell absorbers. These inhomogeneities yield material properties (e.g., composition, structure, and charge collection) that are challenging to correlate across length scales and measurement modalities. The challenge is compounded if a correlation is sought during device operation or in conditions that mimic aging under particular stressors (e.g., heat and electrical bias). Correlative approaches, particularly those based on synchrotron x-ray sources, are powerful since they can access several material properties in different modes (e.g., fluorescence, diffraction, and absorption) with minimal sample preparation. Small-scale laboratory x-ray instruments have begun to offer multi-modality but are typically limited by low x-ray photon flux, low spatial resolution, or specific sample sizes. To overcome these limitations, a characterization stage was developed to enable multi-scale, multi-modal operando measurements of industrially relevant photovoltaic devices. The stage offers compatibility across synchrotron x-ray facilities, enabling correlation between nanoscale x-ray fluorescence microscopy, microscale x-ray diffraction microscopy, and x-ray beam induced current microscopy, among others. The stage can accommodate device sizes up to 25 × 25mm2, offering access to multiple regions of interest and increasing the statistical significance of correlated properties. The stage materials can sustain humid and non-oxidizing atmospheres, and temperature ranges encountered by photovoltaic devices in operational environments (e.g., from 25 to 100 °C). As a case study, we discuss the functionality of the stage by studying Se-alloyed CdTe photovoltaic devices aged in the stage between 25 and 100 °C.