As is generally known, the broadband near-infrared supercontinuum (SC) is significant for applications such as pump-probe spectroscopy, nonlinear spectroscopy, frequency combs and nonlinear optical parametric amplification. We present the first detailed demonstration of approximate near-infrared, octave-spanning SC generation in an all-normal dispersion CS2 single-hole liquid core optical fiber (LCOF). By solving the generalized nonlinear Schrödinger equation, the SC can be calculated at different parameters. The influence of important parameters—including but not limited to the fiber core diameter, pump wavelength, pump power and pulse width—on the supercontinuum generation (SCG) of a CS2-infiltrated LCOF can be analyzed for the optimization of near-infrared SCG. The results show that at low pump power (such as P0 = 4 kW), the SC generated by using two pump wavelengths (1.55 μm and 1.95 μm) has spectral flatness, good coherence and is octave-spanning. However, the bandwidth is severely affected by the large pulse duration T0, and the coherence is seriously influenced by the pulse duration T0 > 1200 fs at the pump wavelength of 1.55 μm. The effect of pulse duration on the first-order coherence is greater at short pump wavelengths (1.55 μm) than long wavelengths (1.95 μm). Under high power conditions (such as P0 = 20 kW), the coherence of the SC generated remains good at the two-pump wavelength. This study explores an optimized scheme for obtaining a broadband SC with high coherence and fine spectral flatness suitable for specific applications.
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