Aircraft cloud seeding refers to the use of equipment on aircraft to release chemicals into clouds, changing their physical and chemical properties to increase rainfall or snowfall. The purpose of precipitation enhancement is to alleviate drought and water scarcity issues. Due to the complexity of the technology, the precise control of factors such as cloud characteristics and chemical release amounts is necessary. Therefore, a scientific evaluation of the potential of aircraft cloud seeding can help to improve the effectiveness of the process, and is currently a technical challenge in weather modification. This study used the mesoscale numerical model WRF coupled with a catalytic process to simulate and evaluate the seven aircraft cloud seeding operations conducted in Hunan Province in 2021. The results show that WRF can effectively evaluate the effectiveness of cloud seeding. When the water vapor conditions are suitable, the airborne dispersion of silver iodide (AgI) can significantly increase the content of large particles of high-altitude ice crystals, snow, and graupel, resulting in an increase in low-level rainwater content and, correspondingly, an increase in ground precipitation. When the water vapor conditions are insufficient, the dispersion of AgI does not trigger effective precipitation, consistent with the results of station observations and actual flight evaluations. This study provides an effective method for scientifically evaluating the potential and effectiveness of aircraft cloud seeding operations.