Two-dimensional Photon Gas Research Articles

Realizing arbitrary trapping potentials for light via direct laser writing of mirror surface profiles(a)(a)Contribution to the Focus Issue Turbulent Regimes in Bose-Einstein Condensates edited by Alessandra Lanotte, Iacopo Carusotto and Alberto Bramati.

The versatility of quantum gas experiments greatly benefits from the ability to apply variable potentials. Here we describe a method which allows the preparation of potential structures for microcavity photons via spatially selective deformation of optical resonator geometries with a heat-induced mirror surface microstructuring technique. We investigate the thermalization of a two-dimensional photon gas in a dye-filled microcavity composed of the custom surface-structured mirrors at wavelength-scale separation. Specifically, we describe measurements of the spatial redistribution of thermal photons in a coupled double-ridge structure, where photons form a Bose-Einstein condensate in a spatially split ground state, as a function of different pumping geometries.

Analog curved spacetimes in the reversed dissipation regime of cavity optomechanics

In this paper, we theoretically propose an optomechanical scheme to explore the possibility of simulating the propagation of the collective excitations of the photon fluid in a curved spacetime. For this purpose, we introduce two theoretical models for two-dimensional photon gas in a planar optomechanical microcavity and a two-dimensional array of coupled optomechanical systems. In the reversed dissipation regime (RDR) of cavity optomechanics where the mechanical oscillator reaches equilibrium with its thermal reservoir much faster than the cavity modes, the mechanical degrees of freedom can adiabatically be eliminated. The adiabatic elimination of the mechanical mode provides an effective nonlinear Kerr-type photon-photon interaction. Using the nonlinear Schr\"{o}dinger equation (NLSE), we show that the phase fluctuations in the two-dimensional photon fluid obey the Klein-Gordon equation for a massless scalar field propagating in a curved spacetime. The results reveal that the photon fluid as well as the corresponding metric can be controlled by manipulating the system parameters.

First-order spatial coherence measurements in a thermalized two-dimensional photonic quantum gas

Phase transitions between different states of matter can profoundly modify the order in physical systems, with the emergence of ferromagnetic or topological order constituting important examples. Correlations allow the quantification of the degree of order and the classification of different phases. Here we report measurements of first-order spatial correlations in a harmonically trapped two-dimensional photon gas below, at and above the critical particle number for Bose–Einstein condensation, using interferometric measurements of the emission of a dye-filled optical microcavity. For the uncondensed gas, the transverse coherence decays on a length scale determined by the thermal de Broglie wavelength of the photons, which shows the expected scaling with temperature. At the onset of Bose–Einstein condensation, true long-range order emerges, and we observe quantum statistical effects as the thermal wave packets overlap. The excellent agreement with equilibrium Bose gas theory prompts microcavity photons as promising candidates for studies of critical scaling and universality in optical quantum gases.

Thermalization and Bose–Einstein condensation of a photon gas in a multimode hybrid atom-membrane optomechanical microcavity

In this paper, we theoretically propose an optomechanical scheme to thermalize a two-dimensional photon gas in a hybrid optomechanical microcavity composed of a two-level atomic ensemble and a membrane oscillator enclosed in an optical cavity. The thermalization process is based on a phonon-induced asymmetry between the emission and the absorption rates of the atoms. We show that whenever this asymmetry obeys the detailed balance condition and if the photon lifetime is high enough, the steady-state photon number distribution matches the Bose–Einstein distribution. Furthermore, in order to study the effect of the optomechanical coupling on the Bose–Einstein condensation of photons, we calculate the critical photon number as a function of the temperature. We find that the optomechanically induced nonlinearity leads to the increase of the critical photon number, which can be controlled by tuning the optomechanical parameters.

Calorimetry of a Bose-Einstein-condensed photon gas.

Phase transitions, as the condensation of a gas to a liquid, are often revealed by a discontinuous behaviour of thermodynamic quantities. For liquid helium, for example, a divergence of the specific heat signals the transition from the normal fluid to the superfluid state. Apart from liquid helium, determining the specific heat of a Bose gas has proven to be a challenging task, for example, for ultracold atomic Bose gases. Here we examine the thermodynamic behaviour of a trapped two-dimensional photon gas, a system that allows us to spectroscopically determine the specific heat and the entropy of a nearly ideal Bose gas from the classical high temperature to the Bose-condensed quantum regime. The critical behaviour at the phase transition is clearly revealed by a cusp singularity of the specific heat. Regarded as a test of quantum statistical mechanics, our results demonstrate a quantitative agreement with its predictions at the microscopic level.

Effects of dissipation on the superfluid–Mott-insulator transition of photons

We investigate the superfluid--Mott-insulator transition of a two-dimensional photon gas in a dye-filled optical microcavity and in the presence of a periodic potential. We show that in the random-phase approximation the effects of the dye molecules, which generally lead to dissipation in the photonic system, can be captured by two dimensionless parameters that only depend on dye-specific properties. Within the mean-field approximation, we demonstrate that one of these parameters decreases the size of the Mott lobes in the phase diagram. By considering also Gaussian fluctuations, we show that the coupling with the dye molecules results in a finite lifetime of the quasiparticle and quasihole excitations in the Mott lobes. Moreover, we show that there are number fluctuations in the Mott lobes even at zero temperature and therefore that the true Mott-insulating state never exists if the interactions with the dye are included.

A scheme to observe universal breathing mode and Berezinskii–Kosterlitz–Thouless phase transition in a two-dimensional photon gas

A system of two-dimensional photon gas has recently been realized experimentally. We show that this setup can be used to observe a universal breathing mode of photon gas and a modification in the experimental setup would open up a possibility of observing the Berezinskii–Kosterlitz–Thouless (BKT) phase transition in such a system. Furthermore, the universal jump in the superfluid density of light in the output channel can be used as an unambiguous signature for the experimental verification of the BKT transition.

Photon gas with hyperbolic dispersion relations

We investigate the density of states for a photon gas confined in a nonmagnetic metamaterial medium in which some components of the permittivity tensor are negative. We study the effect of the resulting hyperbolic dispersion relations on the black body spectral density. We show that for both of the possible wavevector space topologies, the spectral density vanishes at a certain frequency. We obtain the partition function and derive some thermodynamical quantities of the system. To leading order, the results resemble those of a one- or two-dimensional photon gas with an enhanced density of states.

Thermalization of a two-dimensional photon gas in a polymeric host matrix

We investigate thermodynamic properties of a two-dimensional photon gas confined by a dye-filled optical microcavity. A thermally equilibrated state of the photon gas is achieved by radiative coupling to a heat bath that is realized with dye molecules embedded in a polymer at room temperature. The chemical potential of the gas is freely adjustable. The optical microcavity consisting of two curved mirrors induces both a non-vanishing effective photon mass and a harmonic trapping potential for the photons. While previous experiments of our group have used liquid dye solutions, the measurements described here are based on dye molecules incorporated into a polymer host matrix. The solid state material allows a simplified operation of the experimental scheme. We furthermore describe studies of fluorescence properties of dye-doped polymers, and verify the applicability of Kennard–Stepanov theory in this system. In the future, dye-based solid state systems hold promise for the realization of single-mode light sources in thermal equilibrium based on Bose–Einstein condensation of photons, as well as for solar energy concentrators.

Bose–Einstein condensation of photons in an optical microcavity

Bose-Einstein condensation (BEC)-the macroscopic ground-state accumulation of particles with integer spin (bosons) at low temperature and high density-has been observed in several physical systems, including cold atomic gases and solid-state quasiparticles. However, the most omnipresent Bose gas, blackbody radiation (radiation in thermal equilibrium with the cavity walls) does not show this phase transition. In such systems photons have a vanishing chemical potential, meaning that their number is not conserved when the temperature of the photon gas is varied; at low temperatures, photons disappear in the cavity walls instead of occupying the cavity ground state. Theoretical works have considered thermalization processes that conserve photon number (a prerequisite for BEC), involving Compton scattering with a gas of thermal electrons or photon-photon scattering in a nonlinear resonator configuration. Number-conserving thermalization was experimentally observed for a two-dimensional photon gas in a dye-filled optical microcavity, which acts as a 'white-wall' box. Here we report the observation of a Bose-Einstein condensate of photons in this system. The cavity mirrors provide both a confining potential and a non-vanishing effective photon mass, making the system formally equivalent to a two-dimensional gas of trapped, massive bosons. The photons thermalize to the temperature of the dye solution (room temperature) by multiple scattering with the dye molecules. Upon increasing the photon density, we observe the following BEC signatures: the photon energies have a Bose-Einstein distribution with a massively populated ground-state mode on top of a broad thermal wing; the phase transition occurs at the expected photon density and exhibits the predicted dependence on cavity geometry; and the ground-state mode emerges even for a spatially displaced pump spot. The prospects of the observed effects include studies of extremely weakly interacting low-dimensional Bose gases and new coherent ultraviolet sources.

Thermalization of a two-dimensional photonic gas in a ‘white wall’ photon box

Bose-Einstein condensation, the macroscopic accumulation of bosonic particles in the energetic ground state below a critical temperature, has been demonstrated in several physical systems. The perhaps best known example of a bosonic gas, blackbody radiation, however exhibits no Bose-Einstein condensation at low temperatures. Instead of collectively occupying the lowest energy mode, the photons disappear in the cavity walls when the temperature is lowered - corresponding to a vanishing chemical potential. Here we report on evidence for a thermalised two-dimensional photon gas with freely adjustable chemical potential. Our experiment is based on a dye filled optical microresonator, acting as a 'white-wall' box for photons. Thermalisation is achieved in a photon number-conserving way by photon scattering off the dye-molecules, and the cavity mirrors both provide an effective photon mass and a confining potential - key prerequisites for the Bose-Einstein condensation of photons. As a striking example for the unusual system properties, we demonstrate a yet unobserved light concentration effect into the centre of the confining potential, an effect with prospects for increasing the efficiency of diffuse solar light collection.

Thermodynamics of losses in photovoltaic conversion

This letter presents a thermodynamic analysis of losses in an ideal solar cell. It is shown that the maximum voltage—corresponding to the voltage produced by a hot-carrier solar cell—is equal to the energy of the incident solar photon multiplied by the appropriate Carnot factor. Voltage generated by the usual p-n junction cell is lower on account of entropy generation through kinetic losses, photon cooling, and étendue expansion of the incident beam. Simple expressions can be obtained by an approximation where the energy and entropy changes are modeled by the corresponding expressions for a two-dimensional ideal photon gas.