As shield tunnels increase, managing shield muck strains construction and the environment. To mitigate this problem, shield muck replaced bentonite in silty clay to improve synchronous grouting slurry. Initially, the physical attributes and microstructural composition of shield muck were obtained, alongside an analysis of the effects of the muck content, particle size, and general influencing factors on the slurry properties through standardized tests and regression models. Subsequently, leveraging three-dimensional response surface methodology, admixture interactions and multiple factor impacts on the slurry were explored. Finally, utilizing the SQP optimization technique, an optimal slurry blend ratio tailored for actual project needs was derived for improved muck slurry. The findings reveal with the decreasing bleeding rates as the muck content rises, the particle size diminishes. An inverse relationship exists between the muck content and slurry fluidity. At soil–binder ratios below 0.6, a decrease in the soil–binder ratio intensifies the influence of the water–binder ratio on the slurry density, bleeding rate, and setting time. The fly flash–cement ratio inversely correlates with the slurry bleeding rate, while the ratio greater than 0.6 is positively correlated. For muck particle sizes under 0.2 mm, the fly flash–cement ratio inversely impacts the density, while over 0.2 mm, it correlates positively. The optimal proportion for silty clay stratum synchronous grouting slurry, substituting muck for bentonite, includes a water–binder ratio of 0.559, binder–sand ratio of 0.684, fly flash–cement ratio of 2.080, soil–binder ratio of 0.253, particle size under 0.075 mm, and water-reducing admixture of 0.06.
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