An experimental study was performed to measure the size and number density distributions of soot particles produced in turbulent, stratified (high spatial equivalence ratio gradient), swirled (rotating flow) premixed ethylene-air flames at atmospheric pressure. Soot particle size and number density measurements are initially performed using a Scanning Mobility Particle Sizer (SMPS). For this purpose, two-stage sampling and dilution device designed for hot gas analysis was used. The dilution rate of the sampling apparatus was evaluated to ensure a most representative probing. In a second step, the ex-situ measurements were replaced by single-shot measurements recorded with a high cadency planar multi-angle light scattering (2D-MALS) laser diagnostic technique, based on the relationship between aggregate size and light scattering angle. In a third step, results obtained by the SMPS as well as by the optical diagnostic were compared. Because a direct confrontation of the obtained results obtained is not feasible due to difference in nature of both techniques, a two-step post-processing methodology as developed. For this purpose, the median electric mobility diameters measured by SMPS were converted into diameters of gyration by means of a semi-empirical conversion tool. Moreover, a time average data processing was applied to the soot size distributions recorded by 2D-MALS, considering that SMPS measurements performed over a relatively large acquisition time converge to a single value. Results obtained in stratified swirled premixed flames by SMPS exhibit an overall good agreement with the optical measurements. This good similarity between the results provides a remarkably high degree of confidence in the quality of the measurements for both measurement systems investigated. Furthermore, the results suggest that a comparison of soot aggregate size and number density measurements between a sampling probe and a light scattering technique is still possible in turbulent flames at atmospheric pressure. While the current work has focused on the performances of SMPS and the 2D-MALS approach on a one-to-one basis, future work will also address the application of these diagnostics to high-pressure two-phase flames for which measurements are made in confined environments.
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