Terahertz Quantum Cascade Laser Sources Research Articles

Phase-matching in terahertz quantum cascade laser sources based on Cherenkov difference-frequency mixing

Terahertz quantum cascade laser sources based on intra-cavity Cherenkov difference-frequency generation in dual-wavelength mid-infrared quantum cascade lasers are currently the only monolithic semiconductor laser technology that can deliver continuous-wave coherent terahertz output at room temperature. Because the Cherenkov difference-frequency generation process enables terahertz radiation generation and extraction across a wide range of frequencies, it is often assumed that phase-matching conditions for this process are automatically fulfilled. We theoretically analyze and experimentally demonstrate that phase-matching plays an important role in these devices, and significant improvements in terahertz power output can be achieved by adjusting the waveguide configuration of the quantum cascade lasers to provide better phase-matching.

Terahertz difference-frequency-generation quantum cascade lasers on silicon with wire grid current injectors.

We propose the concept and experimentally verify the operation of terahertz quantum cascade laser sources based on intra-cavity Cherenkov difference-frequency generation on a silicon substrate with the current injection layer configured as a metal wire grid. Such a current injector configuration enables high transmission of TM-polarized terahertz radiation into the silicon substrate while simultaneously providing a low-resistivity metal contact for current injection.

Broadly tunable lens-coupled nonlinear quantum cascade lasers in the sub-THz to THz frequency range

Room-temperature terahertz (THz) quantum cascade laser sources with intracavity difference-frequency nonlinear mixing are electrically pumped monolithic semiconductor laser sources operating in the 0.6–6 THz spectral range. We report widely tunable, low-frequency THz quantum cascade laser sources using a lens-coupled Cherenkov waveguide scheme. Based on a watt-class high-power, λ ∼ 13.7 μm quantum cascade laser, the monolithic THz source is strongly coupled with a high-resistivity silicon lens, which causes a major increase in the THz coupling efficiency and demonstrates significant performance improvements. A room-temperature 1.5 THz device produces a 0.2 mW peak output power with a high-quality beam pattern. Improved THz outcoupling efficiency using the lens-coupled scheme enabled the demonstration of a high-performance external-cavity semiconductor THz source that is tunable from 420 GHz to 2 THz. The external-cavity, lens-coupled device configuration can technically be assembled into a butterfly-style package for a thumb-sized, widely frequency tunable THz semiconductor source.

Direct Observation of Terahertz Frequency Comb Generation in Difference-Frequency Quantum Cascade Lasers

Terahertz quantum cascade laser sources based on intra-cavity difference frequency generation from mid-IR devices are an important asset for applications in rotational molecular spectroscopy and sensing, being the only electrically pumped device able to operate in the 0.6–6 THz range without the need of bulky and expensive liquid helium cooling. Here we present comb operation obtained by intra-cavity mixing of a distributed feedback laser at λ = 6.5 μm and a Fabry–Pérot device at around λ = 6.9 μm. The resulting ultra-broadband THz emission extends from 1.8 to 3.3 THz, with a total output power of 8 μW at 78 K. The THz emission has been characterized by multi-heterodyne detection with a primary frequency standard referenced THz comb, obtained by optical rectification of near infrared pulses. The down-converted beatnotes, simultaneously acquired, confirm an equally spaced THz emission down to 1 MHz accuracy. In the future, this setup can be used for Fourier transform based evaluation of the phase relation among the emitted THz modes, paving the way to room-temperature, compact, and field-deployable metrological grade THz frequency combs.

Temperature-Insensitive Imaging Properties of a Broadband Terahertz Nonlinear Quantum Cascade Laser

Terahertz (THz) quantum cascade laser sources based on optical nonlinearity are the only electrically pumped monolithic semiconductor sources operable at room temperature in the 0.6–6 THz range. We investigated the temperature dependence of the imaging characteristics of a broadband THz nonlinear quantum cascade laser and evaluated several important properties: the spectrum, far-field pattern and THz imaging results. Consequently, we found that the far-field patterns were single-lobed Gaussian-like, and THz images were well-resolved despite the lower operating temperature of the device. The stable temperature-performance indicates that this broadband THz source is promising for THz imaging applications.

Terahertz imaging with room-temperature terahertz difference-frequency quantum-cascade laser sources.

We demonstrate high-quality non-destructive imaging using a broadband terahertz quantum cascade laser source based on Cerenkov difference-frequency generation. The source exhibited ultra-broadband terahertz emission spectra, as well as a single-lobed Gaussian-like far-field pattern at -30 °C. These features allowed us to build a compact imaging system with a high spatial resolution, from which a nearly theoretical minimum beam spot size was obtained. As a result, we achieve well-resolved, high-contrast images of objects obscured by opaque materials. We also achieved terahertz imaging with the THz DFG-QCL operated at room temperature.

Double-metal waveguide terahertz difference-frequency generation quantum cascade lasers with surface grating outcouplers

We report terahertz quantum cascade laser (QCL) sources based on intra-cavity difference-frequency generation processed into double-metal waveguides with surface-grating outcouplers. This configuration enables high confinement of the terahertz mode in the device active region and efficient surface extraction of terahertz radiation along the entire length of the waveguide. The devices operate at room temperature at 1.9 THz and produce over 110 μW of peak power output with the mid-infrared-to-terahertz conversion of 150 μW/W2. The results represent at least a factor of 2 improvement in the performance compared to the best Cherenkov difference-frequency generation QCL devices operating below 2 THz.

Spectral purity and tunability of terahertz quantum cascade laser sources based on intracavity difference-frequency generation.

Terahertz sources based on intracavity difference-frequency generation in mid-infrared quantum cascade lasers (THz DFG-QCLs) have recently emerged as the first monolithic electrically pumped semiconductor sources capable of operating at room temperature across the 1- to 6-THz range. Despite tremendous progress in power output, which now exceeds 1 mW in pulsed and 10 μW in continuous-wave regimes at room temperature, knowledge of the major figure of merits of these devices for high-precision spectroscopy, such as spectral purity and absolute frequency tunability, is still lacking. By exploiting a metrological grade system comprising a terahertz frequency comb synthesizer, we measure, for the first time, the free-running emission linewidth (LW), the tuning characteristics, and the absolute center frequency of individual emission lines of these sources with an uncertainty of 4 × 10-10. The unveiled emission LW (400 kHz at 1-ms integration time) indicates that DFG-QCLs are well suited to operate as local oscillators and to be used for a variety of metrological, spectroscopic, communication, and imaging applications that require narrow-LW THz sources.

Terahertz difference-frequency quantum cascade laser sources on silicon

Terahertz quantum cascade laser sources based on intra-cavity frequency mixing are currently the only monolithic electrically pumped semiconductor devices that can operate in the 1–6 THz spectral range at room temperature. The introduction of the Cherenkov waveguide scheme in these devices grown on semi-insulating InP substrates enabled generation of tens of microwatts of average terahertz power output and wide spectral tunability. However, terahertz radiation outcoupling in these sources is still highly inefficient. Here we demonstrate that an application of the III–V-on-silicon hybrid laser concept to terahertz quantum cascade laser sources based on Cherenkov intra-cavity difference-frequency generation dramatically improves their output power and mid-infrared-to-terahertz conversion efficiency. The best-performing device transfer-printed on a float-zone high-resistivity silicon substrate produced 270 μW of peak power output at 3.5 THz at room temperature, a factor of 5 improvement over the best reference devices on a native semi-insulating InP substrate.

Ultra-broadband room-temperature terahertz quantum cascade laser sources based on difference frequency generation.

We present ultra-broadband room temperature monolithic terahertz quantum cascade laser (QCL) sources based on intra-cavity difference frequency generation, emitting continuously more than one octave in frequency between 1.6 and 3.8 THz, with a peak output power of ~200 μW. Broadband terahertz emission is realized by nonlinear mixing between single-mode and multi-mode spectra due to distributed feedback grating and Fabry-Perot cavity, respectively, in a mid-infrared QCL with dual-upper-state active region design. Besides, at low temperature of 150 K, the device produces a peak power of ~1.0 mW with a broadband THz emission centered at 2.5 THz, ranging from 1.5 to 3.7 THz.

Spectroscopic Study of Terahertz Generation in Mid-Infrared Quantum Cascade Lasers.

Terahertz quantum cascade laser sources based on intra-cavity difference-frequency generation are currently the only room-temperature mass-producible diode-laser-like emitters of coherent 1–6 THz radiation. Device performance has improved dramatically over the past few years to reach milliwatt-level power output and broad tuning from 1.2 to 5.9 THz, all at room-temperature. Terahertz output in these sources originates from intersubband optical nonlinearity in the laser active region. Here we report the first comprehensive spectroscopic study of the optical nonlinearity and investigate its dependence on the mid-infrared pump frequencies. Our work shows that the terahertz generation efficiency can vary by a factor of 2 or greater depending on the spectral position of the mid-infrared pumps for a fixed THz difference-frequency. We have also measured for the first time the linewidth for transitions between the lower quantum cascade laser states, which is critical for determining terahertz nonlinearity and predicting optical loss in quantum cascade laser waveguides.

The spread into terahertz radiation using FeCrAl alloys wires

FeCrAl alloys wires with different Cr contents were investigated as a broadband radiation source for the spectral region from 1100 to 100cm−1. Due to the change in temperature, the radiation intensity depends on the driven current. Compared with commercial mercury arc lamp and terahertz quantum cascade laser sources, the FeCrAl alloys wires source generates a pronounced THz broad spectrum from 400cm−1 to 100cm−1. Using FeCrAl alloys wires source, the optical phonon absorption and zone-edge two-phonon absorption were observed for typical GaAs substrate transmission. The measurement of the little absorption from 400cm−1 to 100cm−1 for polyethylene film further confirms the potential application of FeCrAl alloys wires source in terahertz field.

External cavity terahertz quantum cascade laser sources based on intra-cavity frequency mixing with 1.2–5.9 THz tuning range

We discuss the design and operation of widely-tunable terahertz sources based on Cherenkov intra-cavity difference-frequency generation in mid-infrared quantum cascade lasers. Laser chips are integrated into a Littrow-type external cavity system. Devices demonstrate continuous terahertz emission tuning at room temperature with a record tuning range from 1.2 THz to 5.9 THz and peak power output varying between 5 and 90 μW, depending on the operating frequency. Beam steering of terahertz Cherenkov emission with frequency is suppressed and mid-infrared-to-terahertz conversion efficiency is improved by bonding devices onto high-resistivity silicon substrates that have virtually no refractive index dispersion and vanishingly-small optical loss in 1–6 THz range.

Room temperature terahertz quantum cascade laser sources with 215 μW output power through epilayer-down mounting

We report room temperature terahertz (THz) quantum cascade laser sources with high power based on difference frequency generation. The device is Čerenkov phase matched and spectrally purified with an integrated dual-period distributed-feedback grating. Symmetric current injection and epilayer-down mounting of the device onto a patterned submount are used to improve the electrical uniformity and heat removal, respectively. The epilayer-down mounting also allows for THz anti-reflective coating to enhance the THz outcoupling efficiency. Single mode emission at 3.5 THz with a side-mode suppression ratio and output power up to 30 dB and 215 μW are obtained, respectively.

Broadly tunable terahertz generation in mid-infrared quantum cascade lasers

Room temperature, broadly tunable, electrically pumped semiconductor sources in the terahertz spectral range, similar in operation simplicity to diode lasers, are highly desired for applications. An emerging technology in this area are sources based on intracavity difference-frequency generation in dual-wavelength mid-infrared quantum cascade lasers. Here we report terahertz quantum cascade laser sources based on an optimized non-collinear Cherenkov difference-frequency generation scheme that demonstrates dramatic improvements in performance. Devices emitting at 4 THz display a mid-infrared-to-terahertz conversion efficiency in excess of 0.6 mW W(-2) and provide nearly 0.12 mW of peak power output. Devices emitting at 2 and 3 THz fabricated on the same chip display 0.09 and 0.4 mW W(-2) conversion efficiencies at room temperature, respectively. High terahertz-generation efficiency and relaxed phase-matching conditions offered by the Cherenkov scheme allowed us to demonstrate, for the first time, an external-cavity terahertz quantum cascade laser source tunable between 1.70 and 5.25 THz.

High performance terahertz quantum cascade laser sources based on intracavity difference frequency generation

We demonstrate high power, room temperature, single-mode THz emissions based on intracavity difference frequency generation from mid-infrared quantum cascade lasers. Dual active regions both featuring giant nonlinear susceptibilities are used to enhance the THz power and conversion efficiency. The THz frequency is lithographically tuned by integrated dual-period distributed feedback gratings with different grating periods. Single mode emissions from 3.3 to 4.6 THz with side-mode suppression ratio and output power up to 40 dB and 65 µW are obtained, with a narrow linewidth of 5 GHz.

Widely tuned room temperature terahertz quantum cascade laser sources based on difference-frequency generation

We demonstrate room temperature THz quantum cascade laser sources with a broad spectral coverage based on intracavity difference-frequency generation. Two mid-infrared active cores based on the single-phonon resonance scheme are designed with a THz nonlinearity specially optimized at the high operating fields that correspond to the highest mid-infrared output powers. A Čerenkov phase-matching scheme along with integrated dual-period distributed feedback gratings are used for efficient THz extraction and spectral purification. Single mode emissions from 1.0 to 4.6 THz with a side-mode suppression ratio and output power up to 40 dB and 32 μW are obtained, respectively.

Terahertz near-field imaging using subwavelength plasmonic apertures and a quantum cascade laser source

The first demonstration, to our knowledge, of near-field imaging using subwavelength plasmonic apertures with a terahertz quantum cascade laser source is presented. "Bull's-eye" apertures, featuring subwavelength circular apertures flanked by periodic annular corrugations were created using a novel fabrication method. A fivefold increase in intensity was observed for plasmonic apertures over plain apertures of the same diameter. Detailed studies of the transmitted beam profiles were undertaken for apertures with both planarized and corrugated exit facets, with the former producing spatially uniform intensity profiles and subwavelength spatial resolution. Finally, a proof-of-concept imaging experiment is presented, where an inhomogeneous pharmaceutical drug coating is investigated.

Terahertz sources based on intracavity frequency mixing in mid-infrared quantum cascade lasers with passive nonlinear sections

We report the design and performance of terahertz quantum cascade laser sources based on intracavity difference frequency generation in dual-wavelength mid-infrared quantum cascade lasers with a passive nonlinear section at the exit facet, designed for giant second-order nonlinear susceptibility. These devices operate in the mid-infrared at λ1=8.4 μm and λ2=9.5 μm, with terahertz output at the difference frequency, λ3≈73 μm. Terahertz output of approximately 100 nW was observed up to a heat sink temperature of 210 K.

Surface-emitting terahertz quantum cascade laser source based on intracavity difference-frequency generation

We report a surface-emitting terahertz source based on intracavity difference-frequency generation in dual-wavelength midinfrared quantum cascade lasers with integrated giant second-order nonlinear susceptibility. The terahertz light is coupled out of the waveguide by a second-order grating etched into the laser ridges. In contrast to sources where the difference-frequency radiation is extracted from the facet, this approach enables extraction of the terahertz emission from the whole length of the device even when the coherence length is small.