Superconducting Proximity Effect Research Articles

Superconducting Proximity Effect in InAsSb Surface Quantum Wells with In Situ Al Contacts

We demonstrate robust superconducting proximity effect in InAs$_{0.5}$Sb$_{0.5}$ quantum wells grown with epitaxial Al contact, which has important implications for mesoscopic and topological superconductivity. Unlike more commonly studied InAs and InSb semiconductors, bulk InAs$_{0.5}$Sb$_{0.5}$ supports stronger spin-orbit coupling and larger $g$-factor. However, these potentially desirable properties have not been previously measured in epitaxial heterostructures with superconductors, which could serve as a platform for fault-tolerant topological quantum computing. Through structural and transport characterization we observe high-quality interfaces and strong spin-orbit coupling. We fabricate Josephson junctions based on InAs$_{0.5}$Sb$_{0.5}$ quantum wells and observe strong proximity effect. These junctions exhibit product of normal resistance and critical current, $I_{c}R_{N} = \SI{270}{\micro V}$, and excess current, $I_{ex}R_{N} = \SI{200}{\micro V}$ at contact separations of 500~nm. Both of these quantities demonstrate a robust and long-range proximity effect with highly-transparent contacts.

Investigation of point-contact Andreev reflection on magnetic Weyl semimetal Co3Sn2S2

Magnetic Weyl semimetals (WSMs) with broken time-reversal symmetry (TRS) hosting topological band structures are expected to provide an ideal platform for investigating topological superconductivity and spintronics. However, the experimental verification of magnetic WSMs is very challenging. Very recently, the kagome magnet Co3Sn2S2 was confirmed to be a magnetic WSM by both angle-resolved photoemission spectroscopy and scanning tunneling spectroscopy and consequently has become the focus of great attention. This paper reports a point-contact Andreev-reflection spectroscopy (PCARS) investigation on the (001) surface and the side surface of the Co3Sn2S2 single crystals, respectively. The measurements from the sample’s (001) and side surfaces provide experimental evidence for transport spin polarization in the Co3Sn2S2 magnetic WSM. Furthermore, the superconducting proximity effect in the Co3Sn2S2 single crystal is successfully detected. The point-contact spectra (PCS) along the in-plane direction cannot be well fitted by theoretical models based on s-wave pairing, indicating that possible triplet p-wave superconductivity may be triggered at the interface, which paves the way for the future exploration of the topological superconductivity and Majorana states in broken TRS WSMs.

Massive Suppression of Proximity Pairing in Topological (Bi_{1-x}Sb_{x})_{2}Te_{3} Films on Niobium.

Interfacing bulk conducting topological Bi_{2}Se_{3} films with s-wave superconductors initiates strong superconducting order in the nontrivial surface states. However, bulk insulating topological (Bi_{1-x}Sb_{x})_{2}Te_{3} films on bulk Nb instead exhibit a giant attenuation of surface superconductivity, even for films only two layers thick. This massive suppression of proximity pairing is evidenced by ultrahigh-resolution band mappings and by contrasting quantified superconducting gaps with those of heavily n-doped topological Bi_{2}Se_{3}/Nb. The results underscore the limitations of using superconducting proximity effects to realize topological superconductivity in nearly intrinsic systems.

Superconducting proximity effect in a Rashba-type surface state of Pb/Ge(111)

The Rashba superconductor, in which spin-splitting bands become superconducting, is fascinating as a novel superconducting system in low-dimensional systems. Here, we present the results of in-situ transport measurements on a Rashba-type surface state of the striped incommensurate (SIC) phase of a Pb atomic layer on Ge(111) surface with additional Pb islands/clusters on it. We found that two-step superconducting transitions occurred at around 7 K and 3 K. The latter superconducting transition is suggested to be induced at the non-superconducting Rashba SIC area because of the lateral proximity effect caused by the superconducting Pb clusters. Our results propose a new type of Rashba superconductor, which is a platform to understand the Rashba superconducting systems.

Superconducting proximity effect in flat band systems

We study theoretically proximity-induced superconductivity and its inverse effect in dice lattice flat band model by considering Josephson junction with an s-wave pairing in the superconducting leads. Using self-consistent tight-binding Bogoliubov–de Gennes method, we show that there is a critical value for chemical potential of the superconductors depending on paring interaction strength over which for undoped normal region the proximity effect is enhanced. Whereas if the supserconductor chemical potential is less than the critical one the proximity effect decreases regardless of normal region doping and in the meanwhile, the pairing amplitude of superconducting region increases significantly. Furthermore, we unveil that the supercurrent passing through the junction is large (vanishingly small) when the superconductor chemical potential is smaller (larger) than the critical value which increases as a function of normal region chemical potential.

Phase-controllable nonlocal spin polarization in proximitized nanowires

We study the magnetic and superconducting proximity effects in a semiconducting nanowire (NW) attached to superconducting leads and a ferromagnetic insulator (FI). We show that a sizable equilibrium spin polarization arises in the NW due to the interplay between the superconducting correlations and the exchange field in the FI. The resulting magnetization has a nonlocal contribution that spreads in the NW over the superconducting coherence length and is opposite in sign to the local spin polarization induced by the magnetic proximity effect in the normal state. For a Josephson-junction setup, we show that the nonlocal magnetization can be controlled by the superconducting phase bias across the junction. Our findings are relevant for the implementation of Majorana bound states in state-of-the-art hybrid structures.

Magnetic field enhanced single particle tunneling in MoS2–superconductor vertical Josephson junction**Project supported by the National Key Research and Development Program of China (Grant Nos. 2018YFA0703703 and 2016YFA0300802) and the National Natural Science Foundation of China (Grant Nos. 91964201, 61825401, and 11774004).

As a prototypical transition-metal dichalcogenide semiconductor, MoS2 possesses strong spin–orbit coupling, which provides an ideal platform for the realization of interesting physical phenomena. Here, we report the magnetotransport properties in NbN–MoS2–NbN sandwich junctions at low temperatures. Above the critical temperature around ∼11 K, the junction resistance shows weak temperature dependence, indicating a tunneling behavior. While below ∼11 K, nearly zero junction resistance is observed, indicating the superconducting state in the MoS2 layer induced by the superconducting proximity effect. When a perpendicular magnetic field ∼1 T is applied, such proximity effect is suppressed, accompanying with insulator-like temperature-dependence of the junction resistance. Intriguingly, when further increasing the magnetic field, the junction conductance is significantly enhanced, which is related to the enhanced single particle tunneling induced by the decrease of the superconducting energy gap with increasing magnetic fields. In addition, the possible Majorana zero mode on the surface of MoS2 can further lead to the enhancement of the junction conductance.

Unusual Superconducting Proximity Effect in Magnetically Doped Topological Josephson Junctions

The transport properties of a topological Josephson junction fabricated from a magnetically doped topological insulator (TI) were investigated. The conductance spectra of the Nb/Fe-Bi$_2$Te$_2$Se/Nb junction below 1 K showed an unusual trident-shaped zero-bias conductance peak with a tiny peak width of $\sim$ 6 $\mu$V. The central peak of the trident peak presents the dc-Josephson current, and the side peaks may reflect an induced unconventional Cooper pairing. Additionally, the critical currents followed inverse to temperature, which may also reflect the presence of an unconventional proximity effect. Furthermore, microwave irradiation derived a drastic change in the conductance spectra from the peak structure into oscillatory ones, a hallmark of the ac-Josephson supercurrent. The current-phase relation of the ac-Josephson effect under high power radiofrequency-irradiation was found to be 4$\pi$-periodic. The results suggest that the junction based on magnetically doped 3D TIs may realize an unconventional Cooper pairing, thus enabling access to the basic physics of Majorana bound states and unconventional superconductivity.

In-gap states of magnetic impurity in quantum spin Hall insulator proximitized to a superconductor

We study in-gap states of a single magnetic impurity embedded in a honeycomb monolayer which is deposited on superconducting substrate. The intrinsic spin–orbit coupling induces the quantum spin Hall insulating (QSHI) phase gapped around the Fermi energy. Under such circumstances we consider the emergence of Shiba-like bound states driven by the superconducting proximity effect. We investigate their topography, spin-polarization and signatures of the quantum phase transition manifested by reversal of the local currents circulating around the magnetic impurity. These phenomena might be important for more exotic in-gap quasiparticles in such complex nanostructures as magnetic nanowires or islands, where the spin–orbit interaction along with the proximity induced electron pairing give rise to topological phases hosting the protected boundary modes.

Weyl superconductor phases in a Weyl-semimetal/superconductor multilayer

Topologically nontrivial superconducting phases have been engineered in topological materials by the proximity effect in contact with conventional superconductors. In this paper, by using the method of the Kronig-Penney model, we study the superconducting proximity effect in the bulk electronic states of Weyl semimetals by considering a multilayer structure consisting of Weyl-semimetal and superconductor layers. Due to the proximity effect, two Weyl nodes are decoupled into four nodes of Majorana fermions resulting in Weyl-superconductor phases or three-dimensional extension of topological-superconductor phases. We find that mismatch of the Fermi velocity and potential barriers at the interface gap out Majorana nodes, thus turn Weyl-superconductor phases with four Majorana nodes into Weyl-superconductor phases with half of Majorana nodes and topological-superconductor phases with odd integer Chern numbers.

Identifying the graphene d-wave superconducting symmetry by an anomalous splitting zero-bias conductance peak

Not until recently, was a gate-tunable, high-temperature superconducting proximity effect in graphene demonstrated experimentally. And usually in d-wave superconductor (SC) hybrid structure, ferromagnetism and spin-triplet states could result in a splitting zero-bias conductance peak (ZBCP). Herein, we theoretically present an anomalous splitting ZBCP in a graphene-based ferromagnet/Rashba spin–orbit coupling (RSOC)/insulator/d-wave SC hybrid structure. With increasing the exchange field from h/EF = 0, the ZBCP starts to turn into a splitting one with a zero-bias conductance dip (ZBCD) sandwiched in between two subpeaks, while from h/EF = 1, the two subpeaks and ZBCD begin to gradually shrink till the ZBCP reappears. The anomalous splitting ZBCP can be modulated by the RSOC strength, magnitude of Fermi wave vector mismatch as well as insulator barrier strength. These peculiar features are ascribed to the novel spin-triplet Andreev reflection in the context of the RSOC, characteristic by the anisotropic d-wave pair symmetry combined with the relativistic nodal fermions, which in turn can be experimentally used to directly identify not only the proximity-induced ferromagnetism and RSOC but d-wave pair symmetry in graphene. These results pave the way to a new class of tunable, high-temperature superconducting spintronic devices based on large-scale graphene.

Superconductivity in an Al-twisted bilayer graphene-Al junction device

We report on realization and quantum transport study of a twisted bilayer graphene (tBLG) Josephson junction device. High-quality tBLG employed in the device fabrication is obtained via chemical vapor deposition and the device is fabricated by contacting a piece of tBLG by two closely spaced Al electrodes in an Al-tBLG-Al Josephson junction configuration. Low-temperature transport measurements show that below the critical temperature of the Al electrodes (Tc ≈ 1.1 K), the device exhibits sizable supercurrents at zero magnetic field, arising from the superconducting proximity effect with high contact transparency in the device. In the measurements of the critical supercurrent as a function of perpendicularly applied magnetic field, a standard Fraunhofer-like pattern of oscillations is observed, indicating a uniform supercurrent distribution inside the junction. Multiple Andreev reflection characteristics are also observed in the spectroscopy measurements of the device, and their magnetic field and temperature dependencies are found to be well described by the Bardeen−Cooper−Schrieffer theory.

Enhanced spin-triplet pairing in magnetic junctions with s -wave superconductors

A common path to superconducting spintronics, Majorana fermions, and topologically-protected quantum computing relies on spin-triplet superconductivity. While naturally occurring spin-triplet pairing is elusive and even common spin-triplet candidates, such as Sr$_2$RuO$_4$, support alternative explanations, proximity effects in heterostructures can overcome these limitations. It is expected that robust spin-triplet superconductivity in magnetic junctions should rely on highly spin-polarized magnets or complex magnetic multilayers. Instead, we predict that the interplay of interfacial spin-orbit coupling and the barrier strength in simple magnetic junctions, with only a small spin polarization and s-wave superconductors, can lead to nearly complete spin-triplet superconducting proximity effects. This peculiar behavior arises from an effective perfect transparency: interfacial spin-orbit coupling counteracts the native potential barrier for states of a given spin and wave vector. We show that the enhanced spin-triplet regime is characterized by a huge increase in conductance magnetoanisotropy, orders of magnitude larger than in the normal state.

Conversion of a conventional superconductor into a topological superconductor by topological proximity effect

Realization of topological superconductors (TSCs) hosting Majorana fermions is a central challenge in condensed-matter physics. One approach is to use the superconducting proximity effect (SPE) in heterostructures, where a topological insulator contacted with a superconductor hosts an effective p-wave pairing by the penetration of Cooper pairs across the interface. However, this approach suffers a difficulty in accessing the topological interface buried deep beneath the surface. Here, we propose an alternative approach to realize topological superconductivity without SPE. In a Pb(111) thin film grown on TlBiSe2, we discover that the Dirac-cone state of substrate TlBiSe2 migrates to the top surface of Pb film and obtains an energy gap below the superconducting transition temperature of Pb. This suggests that a Bardeen-Cooper-Schrieffer superconductor is converted into a TSC by the topological proximity effect. Our discovery opens a route to manipulate topological superconducting properties of materials.

Superconductivity of Topological Surface States and Strong Proximity Effect in Sn1- x Pbx Te-Pb Heterostructures.

Superconducting topological crystalline insulators are expected to form a new type of topological superconductors to host Majorana zero modes under the protection of lattice symmetries. The bulk superconductivity of topological crystalline insulators can be induced through chemical doping and the proximity effect. However, only conventional full gaps are observed, so the existence of topological superconductivity in topological crystalline insulators is still controversial. Here, the successful fabrication of atomically flat lateral and vertical Sn1- x Pbx Te-Pb heterostructures by molecular beam epitaxy is reported. The superconductivity of the Sn1- x Pbx Te-Pb heterostructures can be directly investigated by scanning tunneling spectroscopy. Unconventional peak-dip-hump gap features and fourfold symmetric quasiparticle interference patterns taken at the zero energy in the superconducting gap support the presence of the topological superconductivity in superconducting Sn1- x Pbx Te. Strong superconducting proximity effect and easy preparation of various constructions between Sn1- x Pbx Te and Pb make the heterostructures to be a promising candidate for topological superconducting devices to detect and manipulate Majorana zero modes in the future.

Enhanced Negative Nonlocal Conductance in an Interacting Quantum Dot Connected to Two Ferromagnetic Leads and One Superconducting Lead

In this paper, we investigate the electronic transport properties of a quantum dot (QD) connected to two ferromagnetic leads and one superconducting lead in the Kondo regime by means of the finite-U slave boson mean field approach and the nonequilibrium Green function technique. In this three-terminal hybrid nanodevice, we focus our attention on the joint effects of the Kondo correlation, superconducting proximity pairing, and spin polarization of leads. It is found that the superconducting proximity effect will suppress the linear local conductance (LLC) stemming from the weakened Kondo peak, and when its coupling is bigger than the tunnel-coupling of two normal leads, the linear cross conductance (LCC) becomes negative in the Kondo region. Regarding the antiparallel configuration, increasing spin polarization further suppresses LLC but enhances LCC, i.e., causing larger negative values of LCC, since it is beneficial for the emergence of cross Andreev reflection. On the contrary, for the parallel configuration, with increasing spin polarization, the LLC decreases and greatly widens with the appearance of shoulders, and eventually splits into four peaks, while the LCC decreases relatively rapidly to the normal conductance.

Dominant nonlocal superconducting proximity effect due to electron-electron interaction in a ballistic double nanowire.

Cooper pair splitting (CPS) can induce nonlocal correlation between two normal conductors that are coupled to a superconductor. CPS in a double one-dimensional electron gas is an appropriate platform for extracting a large number of entangled electron pairs and is one of the key ingredients for engineering Majorana fermions with no magnetic field. In this study, we investigated CPS by using a Josephson junction of a gate-tunable ballistic InAs double nanowire. The measured switching current into the two nanowires is significantly larger than the sum of the switching current into the respective nanowires, indicating that interwire superconductivity is dominant compared with intrawire superconductivity. From its dependence on the number of propagating channels in the nanowires, the observed CPS is assigned to one-dimensional electron-electron interaction. Our results will pave the way for the utilization of one-dimensional electron-electron interaction to reveal the physics of high-efficiency CPS and to engineer Majorana fermions in double nanowire systems via CPS.

Enhanced superconductivity in Bi2Se3/Nb heterostructures

The superconducting proximity effect in topological insulator and superconductor heterostructures has aroused intensive research interest in the past decade. While many efforts have been made to investigate the induced superconductivity in topological insulators, the exploration of the effect of topological insulators on superconductors is comparatively rare. Here, we report the observation of an enhanced superconductivity in Bi2Se3/Nb heterostructures. The superconducting transition temperature and the critical field of Bi2Se3/Nb heterostructures are higher than those of the pristine Nb thin films. Such enhanced superconductivity is due to the improved superfluid stiffness in Nb thin films by proximity to the metallic Bi2Se3 flakes. Our findings will further advance the understanding of the superconducting proximity effect in the heterostructures.

Behavior of superconductivity in a Pb/Ag heterostructure

The superconducting proximity effect is a long-standing topic of great importance in condensed matter physics. A crucial but unresolved issue is which interfacial and material details determine the efficiency of the proximity effect. In this paper, we study an epitaxially grown superconductor/normal metal (SC-NM) heterostructure (Pb/Ag) and find a spatially constant superconducting gap determined by local tunneling spectroscopy and magnetoresponse measurements, despite the highly mismatched Fermi surfaces between individual Pb and Ag epitaxial layers and the large differences in the lattice constants and electronic densities of states in the separate components. The uniform superconducting gap is in contrast to the spatially varying pair potential with a discontinuity at the interface theoretically predicted for an ideal SC-NM junction and experimentally observed previously in several lateral SC-NM junctions. We experimentally verify that the transmission of electrons across the interface in the vertical Pb/Ag heterostructure is high enough that a new band structure emerges even at the single-particle level. Our experimental results call for further theoretical work in order to develop predictive power for the proximity effect starting from realistic, materially relevant microscopic models.

Crossover between standard and inverse spin-valve effect in atomically thin superconductor/half-metal structures

Spin-singlet Cooper pairs consisting of two electrons with opposite spins cannot directly penetrate from a superconductor to a half-metal (fully spin polarized ferromagnets) which blocks the superconducting proximity effect between these materials. In this paper we demonstrate that, nevertheless, two half-metallic layers electrically coupled to the superconducting film substantially affect its critical temperature and produce the spin valve effect. Within the tight-binding model for the atomically thin multilayered spin valves we show that depending on the details of the electron energy spectra in half-metals the critical temperature as a function of the angle between the spin quantization axes in half-metals can be either monotonically increasing or decreasing. This finding highlights the crucial role of the band structure details in the proximity effect with half-metals which cannot be adequately treated in the quasiclassical theories.