Soft X-ray Source Research Articles

The 2016 January eruption of recurrent Nova LMC 1968

ABSTRACTWe present a comprehensive review of all observations of the eclipsing recurrent Nova LMC 1968 in the Large Magellanic Cloud which was previously observed in eruption in 1968, 1990, 2002, 2010, and most recently in 2016. We derive a probable recurrence time of 6.2 ± 1.2 yr and provide the ephemerides of the eclipse. In the ultraviolet–optical–IR photometry the light curve shows high variability right from the first observation around 2 d after eruption. Therefore no colour changes can be substantiated. Outburst spectra from 2016 and 1990 are very similar and are dominated by H and He lines longward of 2000 Å. Interstellar reddening is found to be E(B − V) = 0.07 ± 0.01. The super soft X-ray luminosity is lower than the Eddington luminosity and the X-ray spectra suggest the mass of the white dwarf (WD) is larger than 1.3 M⊙. Eclipses in the light curve suggest that the system is at high orbital inclination. On day 4 after the eruption a recombination wave was observed in Fe ii ultraviolet absorption lines. Narrow-line components are seen after day 6 and explained as being due to reionization of ejecta from a previous eruption. The UV spectrum varies with orbital phase, in particular a component of the He ii 1640 Å emission line, which leads us to propose that early-on the inner WD Roche lobe might be filled with a bound opaque medium prior to the re-formation of an accretion disc. Both this medium and the ejecta can cause the delay in the appearance of the soft X-ray source.

The RS CVn candidate DG Ari: orbital and long cycles revealed

DG Ari (ASAS J025521+1539.4) is a variable star that was found in the search of binary stars with periods longer than 30 days in ASAS catalogue. The source shows two periodic component in its light curve. We estimate both, the orbital period, and the long-term cycle using PDM. Additionally, we present a match with the soft X-ray source 1RXSJ025521.3+153951 located at similar position. According with these results, we discuss about its nature as a RS CVn candidate.

The complications of learning from Super Soft Source X-ray spectra

Super Soft X-ray Sources (SSS) are powered by nuclear burning on the surface of an accreting white dwarf, they are seen around 0.1–1 keV (thus in the soft X-ray regime), depending on effective temperature and the amount of intervening interstellar neutral hydrogen (NH). The most realistic model to derive physical parameters from observed SSS spectra would be an atmosphere model that simulates the radiation transport processes. However, observed SSS high-resolution grating spectra reveal highly complex details that cast doubts on the feasibility of achieving unique results from atmosphere modeling. In this article, I discuss two independent atmosphere model analyses of the same data set, leading to different results. I then show some of the details that complicate the analysis and conclude that we need to approach the interpretation of high-resolution SSS spectra differently. We need to focus more on the data than the models and to use more phenomenological approaches as is traditionally done with optical spectra.

Focus on test, measurement, and analytical equipment

Focus on test, measurement, and analytical equipment

Development of a vacuum system for a compact soft X-ray source

The results of the development and experimental investigation of vacuum system with micromembrane element for a compact soft X-ray source and their implementation are presented.

High-Power Ultrashort Pulse Lasers to Pump Plasma-Based Soft X-Ray Lasers

High-energy ultrashort pulse optical lasers operating at high repetition rate are required to drive intense compact coherent soft X-ray sources, including soft X-ray lasers, for applications in nanoscience and nanotechnology, material studies, and high field science. This paper reviews two types of high-power solid-state laser systems developed at Colorado State University to pump compact, high repetition rate, and plasma-based soft X-ray lasers. One is a flashlamp-pumped, petawatt-class Ti:sapphire chirped-pulse amplification laser that generates 0.85 PW pulses of 30 fs duration at 3.3 Hz repetition rate. Using a fraction of the output energy from this laser, we have demonstrated gain-saturated, compact, repetitive lasers down to 6.85 nm in Ni-like Gd and have observed gain in shorter wavelength transitions, down to 5.85 nm in Ni-like Dy. The second type of pump laser is an all diode-pumped chirped-pulse amplification system based on cryogenically cooled Yb:YAG active mirror amplifiers that produces 1 J pulses of picosecond duration at 500 Hz repetition rate. These compact diode-pumped laser systems have enabled new advances in high-average-power tabletop soft X-ray lasers that include 100 Hz demonstrations at wavelengths ranging from 10.9 to 18.9 nm, as well long duration operation at these high repetition rates for periods up to one hour. These and other recent results that include the operation of an 18.9 nm laser Ni-like Mo laser at 400 Hz repetition rate open a path to compact kilohertz repetition rate soft X-ray lasers.

Persistent Quasi-periodic Pulsations during a Large X-class Solar Flare

Abstract Solar flares often display pulsating and oscillatory signatures in the emission, known as quasi-periodic pulsations (QPP). QPP are typically identified during the impulsive phase of flares, yet in some cases, their presence is detected late into the decay phase. Here, we report extensive fine structure QPP that are detected throughout the large X8.2 flare from 2017 September 10. Following the analysis of the thermal pulsations observed in the Geostationary Operational Environmental Satellite/X-ray sensor and the 131 Å channel of Solar Dynamics Observatory/Atmospheric Imaging Assembly, we find a pulsation period of ∼65 s during the impulsive phase followed by lower amplitude QPP with a period of ∼150 s in the decay phase, up to three hours after the peak of the flare. We find that during the time of the impulsive QPP, the soft X-ray source observed with the Reuven Ramaty High Energy Solar Spectroscopic Imager rapidly rises at a velocity of approximately 17 km s−1 following the plasmoid/coronal mass ejection eruption. We interpret these QPP in terms of a manifestation of the reconnection dynamics in the eruptive event. During the long-duration decay phase lasting several hours, extended downward contractions of collapsing loops/plasmoids that reach the top of the flare arcade are observed in EUV. We note that the existence of persistent QPP into the decay phase of this flare are most likely related to these features. The QPP during this phase are discussed in terms of magnetohydrodynamic wave modes triggered in the post-flaring loops.

A “water window” tomography based on a laser-plasma double-stream gas-puff target soft X-ray source

A desktop laser-plasma double-stream gas-puff target soft X-ray (SXR) source, operating in the so-called “water window” spectral range (λ = 2.3–4.4 nm). was successfully employed to acquire 3D tomographic images in transmission mode, using a Fresnel zone-plate microscope. The microscope, operating at the He-like nitrogen spectral line, 2.88-nm wavelength, allows acquiring 3D SXR volumetric reconstructions with a resolution of a few microns. The development of a compact system offers the possibility to obtain 3D reconstructed images in relatively short time and in a laboratory environment, without the involvement of large “photon facilities”, such as synchrotrons or free electron lasers, however, with the modest volume resolution at this point. The possibility to obtain three-dimensional images in the SXR wavelength range using a compact, laser-plasma based system may be useful for material and life sciences, where it is required to visualize small features of the samples in 3D that are not visible with a single 2D image. Details about the equipment and the setup constructions as well as some imaged samples will be presented and discussed.

NEXAFS at nitrogen K-edge and titanium L-edge using a laser-plasma soft x-ray source based on a double-stream gas puff target

We present a possibility of reaching higher energy absorption edges of organic materials, beyond the carbon K-edge, in the near edge X-ray absorption fine structure (NEXAFS) spectroscopy technique using a compact laser-produced plasma soft X-ray (SXR) source based on a double-stream gas puff target. The source was optimized for emission in the SXR spectral range from 1.5 to 5 nm wavelength using the krypton/helium target. The emission spectrum of the source and the absorption spectrum of the investigated sample were measured simultaneously by means of a grazing incidence spectrometer, equipped with a single, large aperture diffractive element. Based on both spectra, the optical density was computed for the silicon nitride membranes in a transmission mode, to reveal the NEXAFS features near the nitrogen K-edge. Moreover, due to spectral narrowing of the SXR emission by the use of titanium filter, reaching the titanium L-edge was also possible. Multiple SXR pulse data were compared to single SXR pulse (single-shot) data as well as to the numerical simulations. In this paper, the detailed information about the source, spectroscopy system, and the results of NEXAFS measurements is presented and discussed.

Water-window soft X-ray source using cryogenic Ar laser plasma

A water-window soft X-ray source using laser plasma from a cryogenic solid Ar target has demonstrated an average output power of 0.5 W with continuously repeated pulses at 3.3 Hz. A higher output power of up to 1 W at 10 Hz can be achieved by simply improving the target system. The characteristics of the Ar ion debris from the plasma were also studied and the kinetic energies of the main ions were found to be less than 2 keV. Using the measured ion spectrum, the erosion damage sputtered by Ar ions on the silicon nitride membrane was studied and the results indicated that the damage should cause no problems in the application of a contact soft X-ray microscope. Our laser plasma X-ray source will provide a compact and convenient source suitable for the soft X-ray microscopy in place of conventional synchrotron facilities.

Atmospheric pressure plasma corona enhanced by photoionizer for degradation of VOCs

A hybrid titanium dioxide (TiO2)-integrated photoionization enhanced atmospheric pressure plasma corona system was developed for effective toluene removal. The individual and synergistic effects of a corona discharge, a photoionizer irradiation with a soft x-ray source, and a TiO2 photocatalyst on toluene removal were investigated by performing various experiments. Voltage–current characteristics revealed a lower corona inception voltage and a higher current at the same voltage caused by combining the corona discharge, the photoionizer irradiation, and the TiO2 photocatalyst. The toluene removal efficiency was significantly enhanced by combining the corona discharge, the photoionizer irradiation, and the TiO2 photocatalyst: (corona discharge + photoionizer irradiation + TiO2: ~86.0%) > (corona discharge + TiO2: ~70.8%) > (corona discharge + photoionizer irradiation: ~51.1%) > (corona discharge: ~43.8%). The toluene removal efficiency increased with an increase in the photoionizer energy. These trends were mainly due to the degree of ion generation in the system. Corona discharge generates ions inside the system, and ion concentration increases as the applied voltage is increased. The photoionizer creates positive and negative ions, which lowers the corona inception voltage and enhances the current. The TiO2 film also enhances ion production under corona discharge, and is activated by photoionizer irradiation to create additional electron–hole pairs. In addition, the rougher surface induced by the morphology change in TiO2 under corona discharge has a positive effect on toluene removal.

Bright High-Order Harmonic Generation around 30 nm Using Hundred-Terawatt-Level Laser System for Seeding Full Coherent XFEL

In the past few years, the laser wakefield acceleration (LWFA) electron is a hot topic. One of its applications is to produce soft X-ray free-electron laser (XFEL). During this process, high harmonic generation (HHG) is a potential seed. To decrease the timing jitter between LWFA and HHG, it is better for them to come from the same laser source. We have experimentally investigated bright high-order harmonic generation with a 200-terawatt (TW)/1-Hz Ti: Sapphire laser system. By using the loosely focused method and optimizing the phase-matching conditions, we have obtained bright high-order harmonics around 30 nm. Output energy of the 29th harmonic (27.6 nm) reaches as high as 100 nJ per pulse, and the harmonic beam divergence is estimated to be 0.3 mrad in a full width at half maximum (FWHM). Although the hundred-TW-level laser system has the problems of poor beam quality and shot-to-shot energy fluctuation for HHG, the generated soft X-ray (~30 nm) sources can also have good stability by carefully optimizing the laser system.

Emission of water-window soft x-rays under optically thin conditions using low-density foam targets.

The effect of optical thickness in a bismuth water-window soft x-ray source is considered by comparing the emission from laser-produced plasmas of a 7.5% atomic density foam target and a solid-density target. The number of photons recorded in the 4nm region was comparable for both targets at a plasma-initiating laser pulse duration of 6ns. From experiments at different pulse durations of 150ps and 6ns, self-absorption (opacity) effects were found to be relatively small for bismuth plasmas as compared to those of tin, based on the same emission mechanism and which are used in 13.5nm sources for extreme ultraviolet lithography.

Radiographic imaging of insects using a copper x-pinch plasma backlighting source

The use of copper x-pinch plasmas as backlighting source for radiographing insects is described. The experiments use 4x 25µm Cu wires driven by a ∼400kA, ∼350ns current pulse to produce a localized source of soft x-rays in the micrometer range. Both source size and energy range of the x-rays photons produced by the x-pinch enable the imaging of low contrast objects such as the rich inner structures of insects with excellent spatial resolution. The technique is used in three different insects: a moth, a fly and a beetle. These radiographies allow clear observation of the details of outer (e.g., wings) and internal systems of the insects. A description of the method and ways to improve the quality of the radiographs are shown and discussed.

Optical coherence tomography (OCT) with 2\u2009nm axial resolution using a compact laser plasma soft X-ray source

We present optical coherence tomography (OCT) with 2 nm axial resolution using broadband soft X-ray radiation (SXR) from a compact laser plasma light source. The laser plasma was formed by the interaction of nanosecond laser pulses with a gaseous target in a double stream gas puff target approach. The source was optimized for efficient SXR emission from the krypton/helium gas puff target in the 2 to 5 nm spectral range, encompassing the entire “water-window” spectral range from 2.3 nm to 4.4 nm wavelength. The coherence parameters of the SXR radiation allowed for the OCT measurements of a bulk multilayer structure with 10 nm period and 40% bottom layer thickness to period ratio, with an axial resolution of about 2 nm and detect multilayer interfaces up to a depth of about 100 nm. The experimental data are in agreement with OCT simulations performed on ideal multilayer structure. In the paper, detailed information about the source, its optimization, the optical system, OCT measurements and the results are presented and discussed.

Selection of target elements for laser-produced plasma soft x-ray sources.

We demonstrated the upper limitation to the number of shots, i.e., target lifetime, together with the number of photons emitted in the water-window soft x-ray spectral region from a number of targets used as sources in this spectral region, for multi-shot irradiation at the same position on the target surface. The spectra involved result from unresolved transition arrays originating from n=3-n=4 transitions in medium-Z element plasmas and from n=4-n=4 transitions originating in high-Z plasmas. The output flux was maintained for the highest number of shots in the case of the high melting point element molybdenum, and the total output in the water window was 7.7×1013 photons/sr at a laser power density of 1.2×1014 W/cm2.

Direct Determination of Absolute Absorption Cross Sections at the L-Edge of Dilute Mn Complexes in Solution Using a Transmission Flatjet.

The 3d transition metals play a pivotal role in many charge transfer processes in catalysis and biology. X-ray absorption spectroscopy at the L-edge of metal sites probes metal 2p-3d excitations, providing key access to their valence electronic structure, which is crucial for understanding these processes. We report L-edge absorption spectra of MnII(acac)2 and MnIII(acac)3 complexes in solution, utilizing a liquid flatjet for X-ray absorption spectroscopy in transmission mode. With this, we derive absolute absorption cross-sections for the L-edge transitions with peak magnitudes as large as 12 and 9 Mb for MnII(acac)2 and MnIII(acac)3, respectively. We provide insight into the electronic structure with ab initio restricted active space calculations of these L-edge transitions, reproducing the experimental spectra with excellent agreement in terms of shapes, relative energies, and relative intensities for the two complexes. Crystal field multiplet theory is used to assign spectral features in terms of the electronic structure. Comparison to charge transfer multiplet calculations reveals the importance of charge transfer in the core-excited final states. On the basis of our experimental observations, we extrapolate the feasibility of 3d transition metal L-edge absorption spectroscopy using the liquid flatjet approach in probing highly dilute biological solution samples and possible extensions to table-top soft X-ray sources.

Atomic-like high-harmonic generation from two-dimensional materials.

The generation of high-order harmonics from atomic and molecular gases enables the production of high-energy photons and ultrashort isolated pulses. Obtaining efficiently similar photon energy from solid-state systems could lead, for instance, to more compact extreme ultraviolet and soft x-ray sources. We demonstrate from ab initio simulations that it is possible to generate high-order harmonics from free-standing monolayer materials, with an energy cutoff similar to that of atomic and molecular gases. In the limit in which electrons are driven by the pump laser perpendicularly to the monolayer, they behave qualitatively the same as the electrons responsible for high-harmonic generation (HHG) in atoms, where their trajectories are described by the widely used semiclassical model, and exhibit real-space trajectories similar to those of the atomic case. Despite the similarities, the first and last steps of the well-established three-step model for atomic HHG are remarkably different in the two-dimensional materials from gases. Moreover, we show that the electron-electron interaction plays an important role in harmonic generation from monolayer materials because of strong local-field effects, which modify how the material is ionized. The recombination of the accelerated electron wave packet is also found to be modified because of the infinite extension of the material in the monolayer plane, thus leading to a more favorable wavelength scaling of the harmonic yield than in atomic HHG. Our results establish a novel and efficient way of generating high-order harmonics based on a solid-state device, with an energy cutoff and a more favorable wavelength scaling of the harmonic yield similar to those of atomic and molecular gases. Two-dimensional materials offer a unique platform where both bulk and atomic HHG can be investigated, depending on the angle of incidence. Devices based on two-dimensional materials can extend the limit of existing sources.

Nanoimaging Using Soft X-Ray and EUV Sources Based on Double Stream Gas Puff Targets

Nanoimaging Using Soft X-Ray and EUV Sources Based on Double Stream Gas Puff Targets

Higher order harmonics suppression in extreme ultraviolet and soft x-ray**Project supported by the National Key Research and Development Program of China (Grant No. 2017YFA0206004), the National Natural Science Foundation of China (Grant No. 11375160), and the National Science Instruments Major Project of China (Grant No. 2012YQ130125).

The extreme ultraviolet and soft x-ray sources are widely used in various domains. Suppressing higher order harmonics and improving spectral purity are significant. This paper describes a novel method of higher order harmonics suppression with single order diffraction gratings in extreme ultraviolet and soft x-ray. The principle of harmonic suppression with single order diffraction grating is described, and an extreme ultraviolet and soft x-ray non-harmonics grating monochromator is designed based on the single order diffraction grating. The performance is simulated by an optical design software. The emergent beams of a monochromator with different gratings are measured by a transmission grating spectrometer. The results show that the single order diffraction grating can suppress higher order harmonics effectively, and it is expected to be widely used in synchrotron radiation, diagnostics of laser induced plasma, and astrophysics.