The expansion of automated production places increased demands on intelligent sensory networks for collecting and processing various input signals, which necessitate higher standards for multimodal detection, sensitivity, and sensing response speed. Here, this work developed a poro-hyperelastic composites-based multimodal tactile sensor capable of triboelectric, piezoresistive, and capacitive modes across multiple strains and frequency domains. Such the multilayered flexible multimodal mechano-electronic sensor (MMES) is constructed from a carbon nanotubes porous sponge (CNPS), facilitating switching between trimodal sensing modes integrated within a single sensor structure, effectively enhancing the electromechanical robustness of the sensory system. The present MMES sensor exhibits excellent pressure sensing performances, with a wide range (0–20 kPa), fast response (less than 102 ms in piezoresistive mode and less than 62 ms in capacitive mode), high sensitivity (up to 0.12 V/kPa⁻1 in triboelectric mode), and long-term durability (exceeding 10,000 cycles). Moreover, a micro-CT generated 3D model was established using finite element analysis (FEA) to investigate porous hyperelastic behaviours of the CNPS composites, in agreement with experimental data. The results demonstrated that the MMES sensor is particularly suitable for dynamic feedback in robotic arms, allowing production lines to make accurate distinguishments and operations by sensing distinct materials and resistances encountered during assembly in real time. The outcomes offer promising applications of multimodal robotic tactile sensing for human-machine interaction.
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