Laser Pulse Shape Research Articles

Formation of spiraling infrared emission patterns by controlled interaction of optical filaments.

We analyzed the formation of mid-infrared conical emission patterns possessing spiral and half-ring shaped wavelength contours from a beam of a few optical filaments. The complex patterns were generated and modified experimentally by adaptive wavefront shaping of the femtosecond laser pulse. Mutual interactions between co-propagating filaments can induce curvature in their paths, and the spiral and half-ring emissions were shown to be a direct consequence of this angular deflection. Based on our experimental and computational results, the spirals form in the far-field due to self-interference of conical emission from a helically moving filament. The presented findings will advance the tailoring of spatial conical emission patterns potentially beneficial for spectroscopic applications and terahertz generation.

Electron bunch charge enhancement in laser wakefield acceleration using a flattened Gaussian laser pulse

We demonstrate the charge enhancement of the electron bunch using a flattened Gaussian laser pulse in laser wakefield accelerations. In laser wakefield accelerations, the change in laser pulse shape affects the diffraction pattern, resulting in laser intensity variation during plasma interaction. We employ a flattened Gaussian laser pulse to excite wakefields for electron acceleration. The central flattened region of the flattened Gaussian laser pulse, having the same energy as the Gaussian pulse, helps to enhance the pulse intensity via self-focusing. Thus, the evolution of flat Gaussian pulse enhances self-injection, which leads a considerable amount of electrons into the accelerating fields. A linear theoretical model is adopted to understand the wakefield generation mechanism using Gaussian and flattened Gaussian pulses. In order to broaden our understanding, quasi-three-dimensional PIC simulations are also performed. Our results show that a flattened Gaussian laser pulse with N=2 (where N is the order of the super Gaussian shape) yields a good quality electron bunch with retaining a relatively higher charge (about 300 pC) with respect to the case of a Gaussian laser pulse. We also show a twofold increase in bunch peak current when a flattened Gaussian pulse is employed. The electron bunches with high charge and high current may be promising candidates to drive next-generation compact free-electron lasers with unique X-ray properties.

Reaching 30% energy coupling efficiency for a high-density-carbon capsule in a gold rugby hohlraum on NIF

In the laser-driven indirect drive scheme for inertial confinement fusion, the energy coupling efficiency from the hohlraum to the capsule is typically ∼10% due to limited capsule sizes in order to attain quasi-round implosions with currently available laser energy in cylindrical hohlraums. Recent experiments at the National ignition Facility (NIF) showed ∼30% energy coupling efficiency to aluminum capsules by using a rugby-shaped hohlraum to accommodate larger capsules. This paper reports the first experiment at the NIF demonstrating ∼30% energy coupling to a 3 mm-diameter high-energy-density carbon capsule in a rugby hohlraum with a two-shock laser pulse shape. By comparing the measured bang time with a simulated hydrodynamic scaling, ∼430 kJ coupling is inferred with 1.36 MJ laser drive. The symmetry of the hot spot was observed to be more oblate than simulations predicted. X-ray images taken at late time show strong emission at the laser entrance hole of the rugby hohlraum, indicating a closure earlier than expected, which could contribute to the oblate hot spot shape. Implementing wavelength detuning or modifying the hohlraum shape to tune the symmetry in future experiments would allow symmetric implosions while maintaining the high energy coupling.

Control and Measurement of Quantum Light Pulses for Quantum Information Science and Technology

AbstractManipulation of quantum optical pulses, such as single photons or entangled photon pairs, enables numerous applications, from quantum communications and networking to enhanced sensing. Common methods to shape laser pulses based upon filtering or amplification cannot be employed with quantum light pulses as these approaches introduce detrimental loss and noise to the system. Here, methods to control and measure quantum light pulses based upon deterministic application of targeted phases in time and frequency domains are reviewed, along with recent demonstrations of quantum applications.

The effects of multispecies Hohlraum walls on stimulated Brillouin scattering, Hohlraum dynamics, and beam propagation

Experiments and simulations have been conducted to investigate the efficacy of Ta2O5-lined Hohlraum walls at reducing stimulated Brillouin backscattering (SBS) as well as any subsequent effects on the Hohlraum dynamics and capsule implosions in indirect drive experiments at the National Ignition Facility. Using a 1.1 MJ 400 TW, 351 nm, shaped laser pulse, we measure a 5× reduction in SBS power in the peak of the pulse from the wall on the outer 50° cone beams. The SBS spectrum indicates a reduction in the high-Z spectral signature when using multispecies wall materials. Detailed hydrodynamic simulations were performed using different heat conduction models with flux limiters. Additional simulations were performed on the plasma maps using the 3D parallel paraxial code pF3D to compare backscatter powers between the pure Au and Ta2O5-lined Hohlraums. Further analysis, using hydrodynamically equivalent plasmas, shows that the SBS reduction is clearly a result of the added ion Landau damping caused by the oxygen ions and not from differences in plasma conditions. The experimental and simulation results also show an increase in the wall plasma expansion when using the Ta2O5 liner leading to a 70% more oblate implosion.

Controlling H3+ Formation From Ethane Using Shaped Ultrafast Laser Pulses

An adaptive learning algorithm coupled with 3D momentum-based feedback is used to identify intense laser pulse shapes that control H3+ formation from ethane. Specifically, we controlled the ratio of D2H+ to D3+ produced from the D3C-CH3 isotopologue of ethane, which selects between trihydrogen cations formed from atoms on one or both sides of ethane. We are able to modify the D2H+:D3+ ratio by a factor of up to three. In addition, two-dimensional scans of linear chirp and third-order dispersion are conducted for a few fourth-order dispersion values while the D2H+ and D3+ production rates are monitored. The optimized pulse is observed to influence the yield, kinetic energy release, and angular distribution of the D2H+ ions while the D3+ ion dynamics remain relatively stable. We subsequently conducted COLTRIMS experiments on C2D6 to complement the velocity map imaging data obtained during the control experiments and measured the branching ratio of two-body double ionization. Two-body D3+ + C2D3+ is the dominant final channel containing D3+ ions, although the three-body D + D3+ + C2D2+ final state is also observed.

Narrow Bandwidth Gamma Comb from Nonlinear Compton Scattering Using the Polarization Gating Technique.

Nonlinear Compton scattering is a promising source of bright gamma rays. Using readily available intense laser pulses to scatter off the energetic electrons, on the one hand, allows us to significantly increase the total photon yield, but on the other hand, leads to a dramatic spectral broadening of the fundamental emission line as well as its harmonics due to the laser pulse shape induced ponderomotive effects. In this Letter we propose to avoid ponderomotive broadening in harmonics by using the polarization gating technique-a well-known method to construct a laser pulse with temporally varying polarization. We show that by restricting harmonic emission only to the region near the peak of the pulse, where the polarization is linear, it is possible to generate a bright narrow bandwidth comb in the gamma region.

Shock-ramp analysis test problem

Quasi-isentropic (ramp) compression is now a well-established experimental method and so are the analysis techniques to give Lagrangian sound speed, pressure, and density along the sample material's isentrope. A shock followed by ramp compression is a natural extension to investigate, for example, shock melt and refreeze on compression, or isentropes of states off the Hugoniot or principal isentrope. In practice, graded-density impactors produce initial shocks, compression by shaped laser pulses may be unable to produce a smooth pressure increase from zero, and incidental perturbations on the drive pulse may also give rise to shocks, so robust shock-ramp analysis methods will be needed. Appropriate analysis methods are needed for shock-ramp experiments, based on those for quasi-isentropic compression, and these require validation. This paper describes three different analyses of a shock-ramp test problem, including an assessment of their estimated errors. The methods tested were based on hydrodynamic characteristics or integration backward in space. All methods gave the known Lagrangian sound speed to within ∼1%, and pressure and volume to within less than 2% and 1%, demonstrating that the analysis methods of isentropic compression experiments can be confidently extended to the analysis of shock and ramp compression.

On the Usage of Tapered Undulators in the Measurement of Interference in the Intensity-Dependent Electron Mass Shift

In nonlinear Thomson scattering, the main emission line and its harmonics form a band-like structure due to the laser pulse shape induced ponderomotive broadening. We propose to use tapered undulators to mimic Thomson scattering and measure the intensity-dependent electron mass shift experimentally. We also numerically show that the effect is observable for realistic electron beams like in DESY or SKIF.

Focal spot optimization through scattering media in multiphoton lithography

Shaping the optical wavefront utilizing spatial light modulators (SLMs) is a valuable methodology for modification of a focal spot. It has numerous applications in microscopy, particularly in scattering media. Optical lithography techniques, i.e. multiphoton lithography, can also benefit from wavefront shaping. In this contribution, we present focus optimization in multiphoton lithography through a scattering medium. Beam shaping of a femtosecond-pulsed laser pulse was achieved using a liquid-crystal SLM. For the feedback system a low-cost approach, using a Raspberry Pi-camera in Bayer-mode was applied. Images of the focal spot were used as input for an evolutionary algorithm to improve focus quality.

Current Progress in Femtosecond Laser Ablation/Ionisation Time-of-Flight Mass Spectrometry

The last decade witnessed considerable progress in the development of laser ablation/ionisation time-of-flight mass spectrometry (LI-TOFMS). The improvement of both the laser ablation ion sources employing femtosecond lasers and the method of ion coupling with the mass analyser led to highly sensitive element and isotope measurements, minimisation of matrix effects, and reduction of various fractionation effects. This improvement of instrumental performance can be attributed to the progress in laser technology and accompanying commercialisation of fs-laser systems, as well as the availability of fast electronics and data acquisition systems. Application of femtosecond laser radiation to ablate the sample causes negligible thermal effects, which in turn allows for improved resolution of chemical surface imaging and depth profiling. Following in the footsteps of its predecessor ns-LIMS, fs-LIMS, which employs fs-laser ablation ion sources, has been developed in the last two decades as an important method of chemical analysis and will continue to improve its performance in subsequent decades. This review discusses the background of fs-laser ablation, overviews the most relevant instrumentation and emphasises their performance figures, and summarizes the studies on several applications, including geochemical, semiconductor, and bio-relevant materials. Improving the chemical analysis is expected by the implementation of laser pulse sequences or pulse shaping methods and shorter laser wavelengths providing current progress in mass resolution achieved in fs-LIMS. In parallel, advancing the methods of data analysis has the potential of making this technique very attractive for 3D chemical analysis with micrometre lateral and sub-micrometre vertical resolution.

Efficient generation of a high-field terahertz pulse train in bulk lithium niobate crystals by optical rectification.

We demonstrate a highly efficient method for the generation of a high-field terahertz (THz) pulse train via optical rectification (OR) in congruent lithium niobate (LN) crystals driven by temporally shaped laser pulses. A narrowband THz pulse has been successfully achieved with sub-percent level conversion efficiency and multi MV/cm peak field at 0.26 THz. For the single-cycle THz generation, we achieved a THz pulse with 373-μJ energy in a LN crystal excited by a 100-mJ laser pulse at room temperature. The conversion efficiency is further improved to 0.77 % pumped by a 20-mJ laser pulse with a smaller pump beam size (6 mm in horizontal and 15 mm in vertical). This method holds great potential for generating mJ-level narrow-band THz pulse trains, which may have a major impact in mJ-scale applications like terahertz-based accelerators and light sources.

The effect of the laser pulse shape on the wakefield generation in field-ionized plasma

In this paper, the effect of the laser pulse shape on the generation and evolution of the wakefield during the interaction of the intense laser pulse with the gas have been studied utilizing the parallel relativistic PIC simulation code. In order to reach this aim, three pulses with length 300 fs and different rise-times 30, 45, and 60 are typically selected. Our results show that, the amplitude of the laser wakefield produced in the gas in comparison with the plasma strongly depends on the laser pulse shape. The simulation results indicate that for the high-slope laser pulse time (here 30 fs), ionization and thus density fluctuations have no significant effect on the wakefield generation because of rapid increase of the laser electric field. While by increasing the laser pulse rise-time to 45 fs, the rapid wave breaking due to the change in the medium refractive index during the gas ionization, prevents from the wakefield amplitude growth, so that the wakefield with larger amplitude is emerged in the plasma. For a slow-sloping pulse (here 60 fs), the ratio of the wakefield generation in the gas to the plasma is altered for the different gas densities and laser intensities. Moreover, it is represented that the longer the laser pulse rise-time, the sooner difference between the wakefield produced in the gas and plasma is observed. In fact, the larger the rise-time, the greater the density fluctuations and, consequently, the larger the initial noise is generated to seed the Raman instability.

Pulse-length Effect on Laser Wakefield Acceleration of Electrons by Skewed Laser Pulses

Laser pulse-length-related control and optimization of electron acceleration from laser wakefield acceleration (LWFA) by a shaped laser pulse is proposed to investigate in this study. The laser pulse shape changes and becomes skewed due to the variation in refractive index during propagation in plasmas. The optimum laser pulse-length for excitation of plasma wave in linear regime $(a_{0} is $\tau _{L}=\lambda _{p} / \sqrt {2\pi c} $ , but, in nonlinear regime $(a_{0}>1)$ , is not quite certain. Here, laser strength parameter $(a_{0})$ is defined as the ratio $eE_{L}/\text {m}\omega \text {c}$ . In nonlinear case, the variation in pulse skewedness at an optimized laser pulse-length produces different evolution of the wakefield that might affect the electron beam parameters. The present investigation predicts an optimized laser pulse-length (with an optimize ratio of the leading to the trailing pulse edge duration) 35 fs and laser strength parameter $a_{0}=2$ to control the electron bunch charge, emittance, and energy wakefield. Injected bunch charge is enhanced about 20%, and beam emittance is reported to reduce about 40% by employing the skewed Gaussian laser pulse in place of Gaussian pulse for LWFA. Energy-spread of accelerated electron bunch is also reduced from 18% to 6.6% for $s_{\alpha }=0.45$ for 35-fs laser pulse. The electron bunch parameters can also be controlled and optimized using skewed laser pulse and optimized pulse-length.

Micro-optics for ultra-intense lasers

Table-top, femtosecond lasers provide the highest light intensities capable of extreme excitation of matter. A key challenge, however, is the efficient coupling of light to matter, a goal addressed by target structuring and laser pulse-shaping. Nanostructured surfaces enhance coupling but require “high contrast” (e.g., for modern ultrahigh intensity lasers, the peak to picosecond pedestal intensity ratio >1012) pulses to preserve target integrity. Here, we demonstrate a foam target that can efficiently absorb a common, low contrast 105 (in picosecond) laser at an intensity of 5 × 1018 W/cm2, giving ∼20 times enhanced relativistic hot electron flux. In addition, such foam target induced “micro-optic” function is analogous to the miniature plasma-parabolic mirror. The simplicity of the target—basically a structure with voids having a diameter of the order of a light wavelength—and the efficacy of these micro-sized voids under low contrast illumination can boost the scope of high intensity lasers for basic science and for table-top sources of high energy particles and ignition of laser fusion targets.

Quantum theory of femtosecond optomagnetic effects for rare-earth ions in DyFeO3

Our theoretical analysis shows that a femtosecond laser pulse can efficiently launch magnetization dynamics of ${\mathrm{Dy}}^{3+}$ ions in ${\mathrm{DyFeO}}_{3}$ and ${\mathrm{DyAlO}}_{3}$. Excitation of electrons from the ground state to the low-lying electronic level of ${\mathrm{Dy}}^{3+}$ ions by circularly or linearly polarized light can be seen as a result of an effective magnetic field acting on the magnetic moments of the rare-earth ions. It is shown that the launched magnetization dynamics can be expressed as a combination of coherent oscillations of mutually parallel and mutually antiparallel magnetic moments of ${\mathrm{Dy}}^{3+}$ ions, respectively. While the antiparallel magnetic moments lie in the plane perpendicular to the wave vector of light in the medium $\mathbit{k}$, the parallel magnetic moments are aligned along $\mathbit{k}$. The magnetization dynamics depend strongly on the duration and the shape of the pumping laser pulse, as well as on the anisotropy in properties of the rare-earth ion.

Laser-plasma acceleration beyond wave breaking

Laser wakefield accelerators rely on the extremely high electric fields of nonlinear plasma waves to trap and accelerate electrons to relativistic energies over short distances. When driven strongly enough, plasma waves break, trapping a large population of the background electrons that support their motion. Aside from limiting the maximum electric field, this trapping can lead to accelerated electron bunches with large energy spreads. Here, we introduce a novel regime of plasma wave excitation and wakefield acceleration that allows for arbitrarily high electric fields while avoiding the deleterious effects of unwanted trapping. The regime, enabled by spatiotemporal shaping of laser pulses, exploits the property that nonlinear plasma waves with superluminal phase velocities cannot trap charged particles and are therefore immune to wave breaking.

Using Temporally Synthesized Laser Pulses to Enhance the Conversion Efficiency of Sn Plasmas for EUV Lithography

We have studied the laser pulse shape dependence of the conversion efficiency of λ = 1.03 μm laser pulse energy into 13.5 nm extreme ultraviolet (EUV) emission from a Sn laser-produced plasma. Laser pulses of arbitrary temporal shape ranging from hundreds of picoseconds to several nanoseconds were generated using a programmable pulse synthesizer based on a diode-pumped chirped pulse amplification Yb: YAG laser. Measurements show that the conversion efficiency favors the use of nearly square pulses of duration longer than 2 ns, in agreement with hydrodynamic/atomic physics simulations. A 35% increase in conversion efficiency was obtained when Q-switched pulses were substituted by square pulses of a similar duration. Experiments conducted irradiating a Sn target with a sequence of two time-delayed 250 ps pulses showed a 30 percent increase in the EUV yield respect to a single pulse of the same total energy when the pulse separation was optimum at 2.1 ns. This suggests that re-heating of the plasma with delayed laser pulses could be used to improve the EUV yield. The spectroscopic characterization of EUV emission and in-band EUV images that characterize the source size are also presented.

Field-free alignment of triatomic molecules controlled by a slow turn-on and rapid turn-off shaped laser pulse

The field-free alignment of XCN (X = F, Cl, Br, I) molecules steered by a slow turn-on and rapid turn-off shaped laser pulse is theoretically investigated by using the density matrix theory. Based on the interactions of permanent dipole, polarizability and hyperpolarizability, the results of relatively accurate molecular alignment are obtained in an non-adiabatic regime, and the alignment differences among the molecules are compared. It is shown that the maximum degree of molecular alignment can be obviously improved when the rising time of the shaped laser pulse is adjusted. It is found that the N = 1 shaped pulse has an advantage over the Gaussian or super-Gaussian shaped pulse in enhancing the maximum degree of field-free alignment. Within a certain range, the optimal alignment can be achieved when the pulse amplitude takes a smaller value for FCN, ClCN and BrCN, while the pulse amplitude must take a larger value for ICN. Finally, we analyse the variation of molecular alignment by changing the rotational temperature and find that the large permanent dipole moment and polarizability, and the small hyperpolarizability for those molecules, are more conducive to create a high degree of molecular alignment at the same temperature. Abbreviations: PACS 33.80.-b: Photon interactions with molecules; PACS 33.15.Vb: Correlation times in molecular dynamics; PACS 33.15.Kr: Electric and magnetic moments (and derivatives), polarizability, and magnetic susceptibility

Optimization of piezotransducer dimensions for quasicollinear paratellurite AOTF

The method of quasicollinear acousto-optic tunable filters (AOTFs) piezoelectric transducer dimensions optimization is presented. The AOTFs with large interaction length apply the bulk acoustic wave (BAW) reflection from the input optical facet. Optimization is based on spectral approach to simulation of the BAW field in anisotropic media and Raman–Nath equations numerically solved for the inhomogeneous acoustic field. It was found that variation of the transducer dimensions can minimize RF power consumption of the AOTF. Comparison of the optimized transducer dimensions with those commonly used in quasicollinear paratellurite AOTFs showed that it is possible to improve the AOTF energy efficiency in about 2 times. It was shown that acoustic field simulation results obtained for one AOTF geometry can be applied to the other geometries but for equivalent frequency providing the same ultrasound beam ray spectrum width. It was also shown that when choosing the quasicollinear AOTF with reflection geometry, one should not rely only on the AO figure of merit value, since the energy efficiency of such AOTF type will be determined by the product of the AO figure of merit and the AOTF efficiency, which takes into account the change in the acoustic beam width in the reflection process. The results aim at improving the design of AOTFs for ultrashort laser pulse shaping.