Laser Pulse Shape Research Articles

Ponderomotive potential effects on strong field two-photon double ionization in neon

Abstract In the context of the recently reported experiment on photoionization in neon atom, we theoretically study the photoionization of neon atom at a comparatively intense laser field. The calculated photoelectron spectrum for a Gaussian laser pulse show an asymmetric double peak line shape at a pulse duration of 14.2 fs and peak intensity of 1 × 1015 W cm−2. A systematic study clearly indicates that the ponderomotive potential of the photoelectron released during photoionization of neon is instrumental in causing the visible asymmetry. Interestingly, for similar laser parameters asymmetry in the photoelectron spectrum gets significantly reduced for a Sech2 shaped laser pulse. Time resolved photoelectron spectrum reveals that even for a Sech2 shaped laser pulse the two peak photoelectron spectrum is initially asymmetric and evolves into a symmetric line shape with increase in time. The results clearly indicate that irrespective of laser pulse shape asymmetry shows a non-linear decrease as a function of time. Our study also shows the possibility of controlling the asymmetry by varying the pulse duration. The calculations establishes a correlation between the effects of direct double ionization and ponderomotive potential on the asymmetry of the photoelectron spectrum at different pulse durations.

Temperature effect on acoustic waves reflection condition in anisotropic crystals

The reflection of acoustic waves in anisotropic media has found important applications in acousto-optics (AO). It may be realized both with changing the type of acoustic mode and without it. The latter case is applied for the realization of the quasi-collinear AO diffraction geometry for which the incident light and ultrasound wave group velocity vectors are collinear. The acoustic wave involved into the AO interaction exists due to the reflection from the AO cell input optical face. Quasi-collinear configuration of AO interaction enables achieving exceptionally high spectral resolution and diffraction efficiency, therefore, it is applied for the laser pulse shaping. However, the application of AO tunable filters for such purposes requires high acoustic power values, which induce the temperature gradients in the AO crystal. Temperature variations influence the stiffness constants of the AO crystal, impacting the characteristics of incident and reflected acoustic waves, affecting the acoustic wave reflection condition and consequently, the AO diffraction characteristics. This study presents the theoretical and experimental examination of the temperature influence on the acoustic beam reflection in anisotropic crystals on the example of tellurium dioxide crystal. This paper is supported by the Russian Science Foundation, grant 23-12-00057.

A linearized hydrodynamic code for laser ablation and its application to laser pulse shaping for direct-drive fusion

One of the most harmful processes in inertial confinement fusion is Rayleigh–Taylor instability (RTI), and an efficient way to mitigate it is pulse shaping. However, because shaped laser pulses lead to unsteady ablation, it is insufficient to evaluate RTI based solely on the instability growth rate. Here, for better prediction of RTI during linear growth, hydrodynamic equations for laser ablation (including both balance and linearized perturbation equations) are solved numerically and used to optimize the laser pulse shape for direct-drive inertial confinement fusion. For given target conditions and laser energy, simulations show that a picket pulse before the main laser pulse can reduce RTI significantly, and it is clear that the reduction comes from two aspects: (i) the lower RTI seed due to rarefaction at the descending edge of the picket in the imprint stage and (ii) the smaller growth rate due to enhanced ablation velocity at the main pulse in the acceleration stage. It is found that the perturbed laser deposition in an underdense plasma also has a profound influence on RTI seeds in the imprint stage.

Toward Stabilizing the Keyhole in Laser Spot Welding of Aluminum: Numerical Analysis.

The inherent instability of laser welding, particularly keyhole instability, poses significant challenges in industrial applications, leading to defects such as porosities that compromise weld quality. Various forces act on the keyhole and molten pool during laser welding, influencing process stability. These forces are categorized into those promoting keyhole opening and penetration (e.g., recoil pressure) and those promoting keyhole collapse (e.g., surface tension, Darcy's damping forces), increasing instability and defect likelihood. This paper provides a comprehensive instability analysis to uncover key factors affecting keyhole and process instability, presenting future avenues for improving laser welding stability. Using a novel numerical method for simulating laser spot welding on aluminum with COMSOL Multiphysics 5.6, we investigated the effect of laser pulse shaping on keyhole and process instability. Our analysis focused on keyhole morphology, fluid flow behaviour, and force analysis. The results indicated that the curvature effect, Marangoni effect, and Darcy's damping force are primary contributors to instability, with the curvature effect and Darcy's damping force being the most dominant. Additionally, erratic and high-velocity magnitudes induce intense fluid flow behaviour, exacerbating keyhole instability. Moreover, single/quadruple peak triangular and variant rectangular ramp-down pulse shapes produced the least instability, while multi-pulse rectangular shapes exhibited intense instability. It was found that combining triangular/rectangular pulse shapes can reduce force and keyhole instability by smoothing spontaneous force spikes, resulting in a more stabilized welding process. Controlling fluid flow and abrupt force changes with appropriate pulse shaping is key to defect-free welded products.

The long road to ignition: An eyewitness account

This paper reviews the many twists and turns in the long journey that culminated in ignition in late 2022 using the laser heated indirect-drive approach to imploding DT filled targets at the National Ignition Facility (NIF), located at the Lawrence Livermore National Laboratory (LLNL). We describe the early origins of the Laser Program at LLNL and key developments such as the paradigm shifting birth of high energy density physics (HEDP) studies with lasers, changes in choice of laser wavelength, and the development of key diagnostics and computer codes. Fulfilling the requirements of the multi-faceted Nova Technical Contract was a necessary condition for the approval of the NIF, but more importantly, the end of the Cold War and the cessation of nuclear testing were key catalysts in that approval, along with the ready-and-waiting field of HEDP. The inherent flexibility of the field of laser driven inertial confinement fusion played a fundamental role in achieving success at the NIF. We describe how the ultimately successful ignition target design evolved from the original “point design” target, through the lessons of experiment. All key aspects of that original design changed: The capsule's materials and size were changed; the hohlraum's materials, size, laser entrance hole size, and gas fills were also all changed, as were the laser pulse shapes that go along with all those changes. The philosophy to globally optimize performance for stability (by raising the adiabat and thus lowering the implosion convergence) was also key, as was progress in target fabrication, and in increasing NIF's energy output. The persistence of the research staff and the steadfast backing of our supporters were also necessary elements in this success. We gratefully acknowledge seven decades of researcher endeavors and four decades of the dedicated efforts of many hundreds of personnel across the globe who have participated in NIF construction, operation, target fabrication, diagnostic, and theoretical advances that have culminated in ignition.

Ultrafast artificial intelligence: machine learning with atomic-scale quantum systems

Abstract We train a model atom to recognize hand-written digits in the range 0-9, employing intense light--matter interaction as a computational resource. For training, the images of the digits are converted into shaped laser pulses (data input pulses). Simultaneously with an input pulse, another shaped pulse (program pulse), polarized in the orthogonal direction, is applied to the atom and the system evolves quantum mechanically according to the time-dependent Schr"odinger equation. The purpose of the optimal program pulse is to direct the system into specific atomic final states (classification states) that correspond to the input digits. 
A success rate of about 40\% is achieved when using a basic optimization scheme that might be limited by the computational resources for finding the optimal program pulse in a high-dimensional search space. Our key result is the capability of the laser-programmed atom to generalize, i.e.,~the classification of unseen images is improved by training. This atom-sized machine-learning image-recognition scheme operates on time scales down to tens of femtoseconds, is scalable towards larger (e.g. molecular) systems, and is readily reprogrammable towards other learning/classification tasks.

Acousto-optic femtosecond laser beam shaping for bottle-beam generation

Abstract This study explores the properties of a laser beam shaping system comprising an acousto-optic dispersive delay line (AODDL) and an acousto-optic tunable filter (AOTF) for ultrashort laser pulse shaping. The system demonstrates the AODDL’s ability to generate signals with arbitrarily positioned transmission windows and investigates the impact of spectral width on field distributions. The AOTF’s frequency scanning and simultaneous control of two and three spectral components are presented. The experimental setup utilizes femtosecond laser radiation, and the results highlight the system’s versatility for programmable spectral and spatial filtering, offering potential applications in advanced optical manipulation.

Temperature impact on acoustic wave reflection in quasi-collinear acousto-optic devices.

Quasi-collinear geometry is a special configuration of acousto-optic (AO) diffraction that applies the acoustic wave reflection from the AO cell input optical face and provides an extremely large interaction length for achieving abnormally high spectral resolution of AO tunable filters. As a result, it becomes possible to implement the multifrequency diffraction which has found important applications for laser pulse shaping. The operation of quasi-collinear AO devices in the multifrequency diffraction regimen is accompanied by the appearance of the longitudinal and transverse temperature gradients in the crystal, mainly due to the acoustic power absorption. Temperature changes the AO cell material stiffness moduli, affecting the characteristics of the incident and reflected acoustic waves (propagation velocities and walk-off angles), and the reflection condition in general. On the example of paratellurite crystal is shown that the AO cell heating near the reflecting facet leads to a deviation of the reflected acoustic beam propagation direction from that specified during the AO cell manufacturing. The deviation magnitude depends on the reflection geometry choice and, in the paratellurite, may exceed several degrees, which adversely affects the AO diffraction characteristics, reducing the AO interaction efficiency and distorting the transmission function shape. The reflected beam deviation may be compensated by means of choosing the angle between the AO cell reflecting face and the piezoelectric transducer face, taking into account the operating AO device thermal regimen.

Generation of UV Ellipsoidal Pulses by 3D Amplitude Shaping for Application in High-Brightness Photoinjectors

Photocathode laser pulse shaping is a crucial technology for enhancing the performance of X-ray free-electron lasers by optimizing the quality of electron beams generated from photocathodes within high-gradient radio frequency guns. By precisely shaping these laser pulses, it is possible to significantly reduce the transverse emittance of produced electron bunches. The optimal pulse shape is an ellipsoidal distribution, commonly referred to as the Kapchinskij–Vladimirskij profile. A pulse-shaping scheme utilizing a commercial Yb:KGW laser operating at 514 nm with a repetition rate of 1 MHz and duration of 260 fs has been developed for generating electron bunches with high peak and average power. This study presents the experimental realization of ellipsoidal pulses via three-dimensional amplitude shaping using spatial light modulators at 514 nm, followed by conversion to UV (257 nm) suitable for Cs 2Te photocathodes. The preservation of pulse shape and a high conversion efficiency during this process are investigated and our experiments pave the way for future emittance minimization for X-ray free-electron lasers.

Ultrafast reverse saturable absorption and all-optical computing with boron dipyrromethene (BODIPY) chromophore derivatives

Ultrafast reverse saturable absorption (RSA) in chromophore-based borondipyrro-methenes (BODIPYs) derivatives, 1,7-Diphenyl-3,5-bis(9,9-dimethyl-9H-fluoren-2-yl)-boron-diuoride-azadipyrromethene (ZL-61) and 1,7-Diphenyl-3,5-bis(4-(1,2,2-triphenyl-vinyl)phenyl)-boron-diuoride azadipyrromethene (ZL-22), has been theoretically analyzed with femtosecond (fs) laser pulses at 800 nm and 850 nm. The results are in good agreement with the reported experimental results. The effect of input pulse intensity, pulse width, nonlinear absorption (NLA) coefficients, sample thickness and laser pulse shaping on transmittance has been studied and optimized for high contrast and low-power operation. All-optical fs NOT and the universal NOR and NAND Boolean logic gates have been designed with ZL-61 and ZL-22. The logic gates with top-hat input pulse profile have a sharp switch ON/OFF time compared to the Gaussian input laser profile. Ultrafast operation at relatively low pump intensities opens up exciting prospects for the applicability of BODIPY derivatives for ultrafast low-power all-optical computing and information processing.

High repetition-rate dual-channel X-ray spectrometer for high-intensity laser-plasma experiments.

We describe the development and demonstration of a high-repetition-rate-capable dual-channel (DC) x-ray spectrometer designed for high-intensity laser-plasma experiments (≥1×1021 W/cm2). The spectrometer, which operates at high repetition rates, is limited only by the refresh rate of targets and the camera's frame rate. It features two channels, each equipped with a flat highly oriented pyrolytic graphite (HOPG) crystal and a unique detector plane, allowing it to resolve two distinct x-ray bands: approximately 7-10 and 10-13keV. Each detector plate carrier holds two slots for active (scintillators) or passive (imaging plates) x-ray detectors. We present the design and testing of the HR-DC-HOPG using both the COMET laser (10J, 0.5ps shot/4min) at LLNL's Jupiter Laser Facility and the SCARLET laser (10J, 30fs shot/min) at Ohio State University. The results demonstrate the spectrometer's performance across various laser energies, target materials, pulse shapes, and detector types.

Novel signatures of radiation reaction in electron–laser sidescattering

In this article we investigate novel signatures of radiation reaction via the angular deflection of an electron beam colliding at 90 degrees with an intense laser pulse. Due to the radiation reaction effect, the electrons can be deflected towards the beam axis for plane wave backgrounds, which is not possible in the absence of radiation reaction effects. The magnitude and size of the deflection angle can be controlled by tailoring the laser pulse shapes. The effect is first derived analytically using the Landau–Lifshitz equation, which allows to determine the important scaling behavior with laser intensity and particle energy. We then move on to full scale 3D Monte Carlo simulations to verify the effect is observable with present day laser technology. We investigate the opportunities for an indirect observation of laser depletion in such side scattering scenarios.

A mathematical expression to predict a laser pulse shape

A mathematical expression to predict the shape of a laser pulse is obtained. It is compatible with an experimental one published elsewhere. Comparative computations with other published trials that follow the same trend are made. As a result, our trial is recommended for forthcoming theoretical studies to be published in the field of pulsed laser heating.

Laser pulse shape transformation in hybrid LC cells containing gold nano-island films

A nano-structured surface containing an Au nano-island film is used to fabricate hybrid liquid crystal (HLC) cells. HLCs are characterized by faster response times. The dynamic holographic technique is applied to make the conversion of the laser pulse shape by using HLCs. From a comparative analysis of experimental results with theoretical modeling of a dynamic process, the time constants of the dynamic grating recording and relaxation have been determined.

Validation of implosion modeling through direct-drive shock timing experiments at the National Ignition Facility.

Precise modeling of shocks in inertial confinement fusion implosions is critical for obtaining the desired compression in experiments. Shock velocities and postshock conditions are determined by laser-energy deposition, heat conduction, and equationsof state. This paper describes experiments at the National Ignition Facility (NIF) [E. M. Campbell and W. J. Hogan, Plasma Phys. Control. Fusion 41, B39 (1999)10.1088/0741-3335/41/12B/303] where multiple shocks are launched into a cone-in-shell target made of polystyrene, using laser-pulse shapes with two or three pickets and varying on-target intensities. Shocks are diagnosed using the velocity interferometric system for any reflector (VISAR) diagnostic [P.M. Celliers et al., Rev. Sci. Instrum. 75, 4916 (2004)0034-674810.1063/1.1807008]. Simulated and inferred shock velocities agree well for the range of intensities studied in this work. These directly-driven shock-timing experiments on the NIF provide a good measure of early-time laser-energy coupling. The validated models add to the credibility of direct-drive-ignition designs at the megajoule scale.

Shaped Laser Pulses for Microsecond Time-Resolved Cryo-EM: Outrunning Crystallization during Flash Melting.

Water vitrifies if cooled at rates above 3 × 105 K/s. In contrast, when the resulting amorphous ice is flash heated, crystallization occurs even at a more than 10 times higher heating rate, as we have recently shown. This may present an issue for microsecond time-resolved cryo-electron microscopy experiments, in which vitreous ice samples are briefly melted with a laser pulse because transient crystallization could potentially alter the dynamics of the embedded proteins. Here, we demonstrate how shaped microsecond laser pulses can be used to increase the heating rate and outrun crystallization. Time-resolved electron diffraction experiments reveal that the critical heating rate for amorphous solid water (ASW) is about 108 K/s. Our experiments add to the toolbox of the emerging field of microsecond time-resolved cryo-electron microscopy by demonstrating a straightforward approach for avoiding crystallization during laser melting and for achieving significantly higher heating rates, which paves the way for nanosecond time-resolved experiments.

Nonlocal effects on the shock-augmented ignition scheme of laser inertial fusion

Shock-augmented ignition (SAI) has recently been proposed as a viable approach to optimize the shock ignition scheme of laser fusion, which may substantially reduce laser power and intensity requirements and, as a result, greatly inhibit the growth of laser-plasma instabilities. However, the nonlocal thermal transport effect, which is believed to play a significant role in shock ignition, has not been considered in evaluation of the SAI scheme yet. Here, by self-consistently including modeling of the space-time-dependent nonlocal thermal transport into the radiation hydrodynamic simulations, we revisit the whole implosion and ignition dynamics of SAI numerically and theoretically. We find that, due to the nonlocal effect, on the one hand, the time-delay window between the igniter spike and the compression pulse in the drive laser for achieving high-gain fusion is much broadened from about 0.45 to 0.7 ns, relaxing the difficulty of laser pulse shaping; on the other hand, both the coast time and the fusion burn duration are significantly reduced by, respectively, 0.22 ns and 47 ps, in favor of increasing the hot-spot pressure around the stagnation stage. Published by the American Physical Society 2024

Proton-boron fusion scheme taking into account the effects of target degeneracy

The proton-boron (p-B11) reaction is regarded as the holy grail of advanced fusion fuels, since the primary reaction produces three α particles with few neutrons and induced radioactivities from second order reactions. Compared to the deuterium-tritium reaction a much higher reaction temperature is required. Moreover, bremsstrahlung energy losses due to the high nuclear charge of boron deem it seemingly apparent than a fusion reactor based on deuterium-tritium plasma in equilibrium is to say the least very difficult. It is becoming more appealing to collide intense laser beams or accelerated proton beams with a boron target to produce p-B11 reactions. The fusion yield of p-B11 reactions is closely related to proton beam parameters and boron target conditions such as density, temperature, and ingredients. Degeneracy will increase fusion yields by reducing the stopping power of injected protons. In this work, we suggest a scheme for beam-target p-B11 fusions via injecting a MeV proton beam into a highly compressed quantum degenerated boron target. Such a boron target can be achieved via quasi-isentropic compression of solid boron by using precisely shaped laser pulses. Our results indicate that for densities ranging from 103 to 104ρs, where ρs is the density of solid boron, contributions of bound and free electrons to the stopping of protons can be completely disregarded and dramatically reduced, respectively. The result is an increase in fusion yield by orders of magnitude. Furthermore, in order to achieve multiplication factor F greater than one, with F defined as the ratio of output fusion energy to the energy of injected protons, it is found there exists a minimum possible density of boron target, which is 1.8×105ρs when the kinetic energy of injected protons is 880 keV. Published by the American Physical Society 2024

Influence of laser pulse shape and cleanliness on two-photon microscopy

Nonlinear microscopy, including two-photon microscopy, requires pulsed lasers as light source. Typically, when choosing the appropriate pulsed laser for two-photon microscopy, the pulse repetition rate, pulse width, total power output, and output beam diameter are among the critical parameters which are often emphasised. Here, we demonstrate that the pulse shape, often overlooked, can have significant impact on the two-photon microscopy excitation efficiency and the effective signal brightness. We provide metrics to ease practical selection of pulsed laser sources for two-photon microscopy.

Space-time dependent non-local thermal transport effects on laser ablation dynamics in inertial confinement fusion

In inertial confinement fusion (ICF), electron thermal transport plays a key role in laser ablation and the subsequent implosion processes, which always exhibits intractable non-local effects. Simple modifications of the local Spitzer–Härm model with either an artificially-assumed constant flux limiter or a purely time-dependent one are applied to explain some experimental data, but fail to simultaneously reproduce the space-time evolution of the whole laser ablation process. Here, by carrying out a series of one-dimensional and two-dimensional radiation hydrodynamic simulations where the space-time-dependent non-local thermal transport model proposed by Schurt, Nicolaï and Busquet (the SNB model) are self-consistently included, we systematically study the non-local effects on the whole laser ablation dynamics including those occurring at the critical surface, the conduction zone and the ablation front. Different from those obtained previously, our results show that due to the non-local heat flow redistribution and redirection, at the critical surface the thermal flux is more inhibited, in the conduction zone the lateral thermal transport is suppressed, and ahead of the ablation front the plasma is preheated. When combined together they eventually result in significant improvement of the laser absorption efficiency, extension of the conduction zone, increase of both the mass ablation rate and shock velocity. Furthermore, the dependence of these laser ablation dynamics on different drive laser intensities is investigated, which provides beneficial enlightenments on potential laser pulse shaping and/or ignition scheme optimization in ICF.