In the present work, the hardness prediction of polypropylene/carbon nanotubes (PP/CNT) and low-density polyethylene/carbon nanotubes (LDPE/CNT) composite materials, processed by microwave technique, has been explored using machine learning models i.e. (Random Forest, Support Vector Regression, K-Nearest Neighbors, Linear Regression, and Neural Network). Four input vectors have been used in the construction of proposed network, such as CNT concentration, power, pressure applied, and exposure time. Hardness prediction is one output that has been evolved from the proposed work. This study presents the prediction of hardness based on machine learning models for both PP/CNT and LDPE/CNT composite materials, and the results show that the Random Forest model consistently performs better than the others models in context with performance metrics like Root Mean Square Error (RMSE), Mean Absolute Error (MAE), and Rate of determination (R2) values. Investigations have been performed on resampling strategies, showing that the jackknife approach enhances model precision and robustness in the case of LDPE/CNT composites. For PP/CNT composite material, it has been noticed that Random Forest gives the highest value of R2 (0.94), whereas Random Forest has the lowest R2 value 0.18 for LDPE/CNT composite material. Random Forest is the most reliable model for predicting the characteristics of PP/CNT composite material due to its ability to handle complex datasets. The LDPE/CNT composite material demonstrates superior prediction accuracy, with a maximum error of just 1.61%, making it a better option for high-precision applications due to enhanced mechanical interactions and improved CNT dispersion.
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