Field Of Quantum Optics Research Articles

Fluorescence by incoherently pumped polar quantum dot placed in a low-frequency monochromatic field

Abstract We studied spectral properties of high-frequency fluorescent radiation from a two-level quantum system with broken inversion spatial symmetry, which can be implemented as a model of a one-electron two-level asymmetric polar semiconductor quantum dot whose electric dipole moment operator has permanent unequal diagonal matrix elements. The case of the excitation of this system by incoherent pumping of some sort supplemented with an additional driving monochromatic field, which frequency is much lower than the optical transition frequency of the quantum dot, was considered. An analytical expression for the fluorescence spectrum as a function of the amplitude and frequency of the monochromatic driving field, as well as of the pumping intensity, was derived. We also discussed feasible practical applications of the effects under study in the field of quantum optics and optoelectronics for the generation of high-frequency radiation, possessing stationary equidistant spectrum, and for the control of the radiative properties of such nanodevices as spasers (dipole nanolasers).

Phonon-Induced Geometric Chirality.

Chiral properties have seen increasing use in recent years, leading to the emerging fields of chiral quantum optics, plasmonics, and phononics. While these fields have achieved manipulation of the chirality of light and lattice vibrations, controlling the chirality of materials on demand has yet remained elusive. Here, we demonstrate that linearly polarized phonons can be used to induce geometric chirality in achiral crystals when excited with an ultrashort laser pulse. We show that nonlinear phonon coupling quasistatically displaces the crystal structure along phonon modes that reduce the symmetry of the lattice to that of a chiral point group corresponding to a chiral crystal. By reorienting the polarization of the laser pulse, the two enantiomers can be induced selectively. Therefore, geometric chiral phonons enable the light-induced creation of chiral crystal structures and therefore the engineering of chiral electronic states and optical properties.

Nonreciprocal Photon Transport in a Chiral Optomechanical System

AbstractChiral interaction between light and quantum emitters leads to emergence development of chiral quantum optics and stimulates a wide range of practical applications in quantum regime, such as single‐photon isolation and photon unidirectional emission. Cavity optomechanics studying the interaction between optical and mechanical resonators plays an important role in the field of quantum optics. However, how to achieve the chiral interaction between light and mechanical oscillators and explore the applications of the chiral optomechanical systems are still difficult encountered in cavity optomechanics. Here, a method is proposed to achieve chiral optomechanical interaction by exploiting directional squeezed light in a multimode optomechanical system. Based on the chiral interaction between photon and phonon, the nonreciprocal photon transport at a single‐photon level can be realized. An isolation ratio of and a negligible insertion loss for the photonic isolator are obtained. This method paves the way to realize chiral optomechanical interaction for conducting chiral optomechanics and opens up the prospect of exploring and utilizing chiral photon–phonon manipulation in the quantum regime.

Large Scale Simulations of Photosynthetic Antenna Systems: Interplay of Cooperativity and Disorder.

Large-scale simulations of light-matter interaction in natural photosynthetic antenna complexes containing more than one hundred thousands of chlorophyll molecules, comparable with natural size, have been performed. Photosynthetic antenna complexes present in Green sulfur bacteria and Purple bacteria have been analyzed using a radiative non-Hermitian Hamiltonian, well-known in the field of quantum optics, instead of the widely used dipole-dipole Frenkel Hamiltonian. This approach allows us to study ensembles of emitters beyond the small volume limit (system size much smaller than the absorbed wavelength), where the Frenkel Hamiltonian fails. When analyzed on a large scale, such structures display superradiant states much brighter than their single components. An analysis of the robustness to static disorder and dynamical (thermal) noise shows that exciton coherence in the whole photosynthetic complex is larger than the coherence found in its parts. This provides evidence that the photosynthetic complex as a whole plays a predominant role in sustaining coherences in the system even at room temperature. Our results allow a better understanding of natural photosynthetic antennae and could drive experiments to verify how the response to electromagnetic radiation depends on the size of the photosynthetic antenna.

Optimal control for nonlinear time-fractional Schrödinger equation: an application to quantum optics

In this research article, a fractional optimal control problem (FOCP) is applied to a nonlinear time-fractional Schrödinger equation (NTFSE) incorporating a trapping potential. The NTFSE is an innovative mathematical advancement in the field of quantum optics, bridging fractional calculus with nonlinear quantum mechanics and addressing the intricacies of systems involving memory and nonlinearity. This exploration helps with potential technological advancements in quantum optics and related domains. Examining the FOCP within this system allows one to design quantum optical systems with enhanced performance, improved precision stability, and robustness against disturbances. In this work, the performance index for the problem is constructed, and then it is reformulated using the fractional variational principle and the Lagrange multiplier method. Additionally, the Jacobi collocation numerical method is employed to solve the FOCP and numerical simulations are demonstrated across various parameters which offer valuable insights into the implemented methodology.

Optimizing biphoton generation via reconfigurable nonlinear waveguide arrays based on scattering tensor.

Spontaneous parametric down-conversion (SPDC) plays a pivotal role in the field of quantum optics, especially in generating quantum entangled states. This study delves into utilizing the scattering tensor of nonlinear waveguide arrays to characterize the SPDC process and optimize its efficiency. By computing the pseudo-inverse of the third-order scattering tensor describing the nonlinear arrays for biphoton generation, we determine the optimal pump profile and array conditions that best approximate a desired output biphoton distribution. Counterintuitively, due to the diffraction of the pump beam, we find that the optimal biphoton correlation does not occur at positions corresponding to the maximum pumping in real space within the coupled nonlinear arrays. Our finding demonstrates that the scattering tensor method combined with universal beam-splitter meshes provides a promising route toward reconfigurable integrated quantum light sources.

Indirect measurement of atomic magneto-optical rotation via Hilbert transform

Abstract The Kramers–Kronig relations are a pivotal foundation of linear optics and atomic physics, embedding a physical connection between the real and imaginary components of any causal response function. A mathematically equivalent, but simpler, approach instead utilises the Hilbert transform. In a previous study, the Hilbert transform was applied to absorption spectra in order to infer the sole refractive index of an atomic medium in the absence of an external magnetic field. The presence of a magnetic field causes the medium to become birefringent and dichroic, and therefore it is instead characterised by two refractive indices. In this study, we apply the same Hilbert transform technique to independently measure both refractive indices of a birefringent atomic medium, leading to an indirect measurement of atomic magneto-optical rotation. Key to this measurement is the insight that inputting specific light polarisations into an atomic medium induces absorption associated with only one of the refractive indices. We show this is true in two configurations, commonly referred to in literature as the Faraday and Voigt geometries, which differ by the magnetic field orientation with respect to the light wavevector. For both cases, we measure the two refractive indices independently for a Rb thermal vapour in a 0.6 T magnetic field, finding excellent agreement with theory. This study further emphasises the application of the Hilbert transform to the field of quantum and atomic optics in the linear regime.

Characterizing Biphoton Spatial Wave Function Dynamics with Quantum Wavefront Sensing.

With an extremely high dimensionality, the spatial degree of freedom of entangled photons is a key tool for quantum foundation and applied quantum techniques. To fully utilize the feature, the essential task is to experimentally characterize the multiphoton spatial wave function including the entangled amplitude and phase information at different evolutionary stages. However, there is no effective method to measure it. Quantum state tomography is costly, and quantum holography requires additional references. Here, we introduce quantum Shack-Hartmann wavefront sensing to perform efficient and reference-free measurement of the biphoton spatial wave function. The joint probability distribution of photon pairs at the back focal plane of a microlens array is measured and used for amplitude extraction and phase reconstruction. In the experiment, we observe that the biphoton amplitude correlation becomes weak while phase correlation shows up during free-space propagation. Our work is a crucial step in quantum physical and adaptive optics and paves the way for characterizing quantum optical fields with high-order correlations or topological patterns.

Tailoring the nonclassicality of light states via mode detuning in waveguide beam splitters

The recent advent of integrated waveguide systems with reconfigurable propagation constants and coupling coefficients has opened the door to using waveguide detuning as a resource for readily tailoring the quantum properties of light states. Here we theoretically demonstrate that waveguide mode detuning can be used for molding the nonclassical properties of two interacting quantum optical fields in integrated waveguide couplers. In particular, we explore the states that are generated by conditional measurements when one of the input ports of the waveguide coupler is excited by coherent states, squeezed vacuum states, and thermal states, while the other port is excited by a single-photon Fock state. We explore the detuning range required to attain nonclassical states. Our findings could pave the way for a robust integrated-optics protocol, providing enhanced control and engineering capabilities over multiphoton quantum states.

Atom Mediated Single‐Photon Nonlinearity in a Quadratically Coupled Optomechanical System

AbstractIn this paper, conventional phonon blockade (CPNB) and conventional photon blockade (CPTB) effects, as well as unconventional phonon blockade (UPB) effects, are studied in an optomechanical system with nonlinear interaction between the cavity frequency and the square of the mechanical displacement driven by an external field, where a two‐level atom couples with the mechanical mode and a microwave driving field pumps cavity mode. The second‐order correlation function is analytically calculated, which is in good agreement with the numerical simulation given by the master equation. With energy‐level diagram, the atom‐mechanical mode coupling is found to induces the degeneracy splitting of the states and give the optimal conditions for CPNB and CPTB in this system. With the origin of UPB, the optimal conditions are derived and it is found that the realization of UPB is determined by the two couplings of the cavity and atom with respect to the mechanical mode. Moreover, some discussions on the experimental implementation in this quadratically coupled optomechanical system are presented. This study provides a possible way for realizing single‐photon nonlinearity and can extend the applications of optomechanical systems in the field of quantum optics.

Coherent control of photonic band gaps through the relative phase using modified superradiance lattice.

We report photonic band gaps based on a modified superradiance lattice having reflectivity close to 100% for both the low and high-frequency ranges. We observe that tuning the relative phase between the coupling fields provides additional control over photonic band gaps. We notice that the relative phase can control three input channels of the probe field simultaneously and efficiently. This feature of relative phase over photonic band gaps provides potential in the field of quantum optics. Further, this scheme is experimentally more viable. Rubidium atoms 87Rb can obtain low-frequency (infrared) photonic band gaps. On the other hand, rubidium atoms 85Rb and beryllium ions Be2+ can form high-frequency ultraviolet and soft X-ray photonic band gaps, achieving reflectivities of 80% and 96%, respectively. This scheme holds promise for constructing highly efficient optical switches and beam splitters.

Gap-Free Tuning of Second and Third Harmonic Generation in Mechanochemically Synthesized Nanocrystalline LiNb1−xTaxO3 (0 ≤ x ≤ 1) Studied with Nonlinear Diffuse Femtosecond-Pulse Reflectometry

The tuning of second (SHG) and third (THG) harmonic emission is studied in the model system LiNb 1−xTa xO 3 (0≤x≤1, LNT) between the established edge compositions lithium niobate (LiNbO 3, x=0, LN) and lithium tantalate (LiTaO 3, x=1, LT). Thus, the existence of optical nonlinearities of the second and third order is demonstrated in the ferroelectric solid solution system, and the question about the suitability of LNT in the field of nonlinear and quantum optics, in particular as a promising nonlinear optical material for frequency conversion with tunable composition, is addressed. For this purpose, harmonic generation is studied in nanosized crystallites of mechanochemically synthesized LNT using nonlinear diffuse reflectometry with wavelength-tunable fundamental femtosecond laser pulses from 1200 nm to 2000 nm. As a result, a gap-free harmonic emission is validated that accords with the theoretically expected energy relations, dependencies on intensity and wavelength, as well as spectral bandwidths for harmonic generation. The SHG/THG harmonic ratio ≫1 is characteristic of the ferroelectric bulk nature of the LNT nanocrystallites. We can conclude that LNT is particularly attractive for applications in nonlinear optics that benefit from the possibility of the composition-dependent control of mechanical, electrical, and/or optical properties.

Quantum Computing and Artificial Intelligence: Synergies and Challenges

Due to the explosive rise of quantum computing, there has been intense competition in business and academics in the field of quantum optics in recent decades. The current invention's overall scalability in quantum computing has surpassed many orders of magnitude, whereas ubiquitous quantum computers can support up to hundreds of quantum bits, or thousands of qubits. Strong machines continue to be developed. As a result, ethnicity has served as the inspiration for a huge number of studies and reports. This essay offers an introduction for everyone who would truly like to understand more about the ideas of quant communication and computing from a machine learning standpoint. It starts with such an educational approach and goes on to cover important turning points and the latest advancements in quantum computing. In this research, these fundamental characteristics of such a virtual network are divided into four major challenges, each of which has been thoroughly examined. correspondingly, A, B, C, and D stand for quantum physics, networking, security, and algorithms. The main issues, important areas of research, and most recent advancements are discussed as the article comes to a close.

Spatially oriented correlated emission based on selective drive of diatomic superradiance states

<sec>In recent years, the radiative properties of atomic systems have been a hot topic in the research fields of quantum optics and quantum information. With the continuous development of nanophotonics, quantum antennas have become an important model for studying atomic radiation. In order to investigate these phenomena in depth, we investigate a system composed of two two-level atoms, and study the two-photon emission phenomenon of diatomic system under conditions of driving directional tunable laser field, interatomic dipole-dipole interaction, and spontaneous emission coherence.</sec><sec>In this study, we diagonalize the atomic Hamiltonian to obtain the eigenvalues and entangled states of the system (symmetric and asymmetric states of two atoms), and use the rotating wave approximation to rotate the system into the laser frame. The evolution of the system is characterized mainly by the evolution of symmetric and asymmetric state, as well as the evolution of coherent terms. In our studies it is found that for identical atoms, certain laser directions and geometric configurations can exclusively drive the superradiant and subradiant states of atoms, which can enhance the first-order interference effect of the atoms and markedly increase the probability of two-photon emission in a specific detection direction. When the superradiant state of the atom is solely driven, there will be no coupling between the superradiant state and subradiant state, resulting in a correlation function angular distribution that is symmetric along the direction perpendicular to atomic axis. Further adjusting the laser direction causes the atomic interference patterns to shift, and the system will exhibit two-photon emission characteristics on one side or both sides.</sec><sec>For nonidentical atomic systems, due to detuning between the two atoms, the laser cannot drive the superradiant state or subradiant state individually, and the influence of changing the laser direction on the coupling strength diminishes with the increase of detuning between the atoms. When the laser is in resonance with one of the atoms, due to the atomic interactions, the other atom can achieve the strongest coherent effect without resonating with the laser. This research reveals that atomic detuning is crucial for the correlation values and angular distribution of the correlation function. By adjusting the atomic detuning and laser direction, the system can display highly directed one-sided two-photon emission characteristics. However, different dissipation rates will lead the probability of two-photon emission to decrease. Our studies can achieve highly directional two-photon emission on one side or both sides, which provides a theoretical basis for studying the two-photon emission of nanoantennas.</sec>

Cost-Effective Laboratory Matrix Projection Micro-Lithography System.

This paper presents a home-built projection lithographer designed to transfer the image from a DLP (digital light processing) projector MEMS matrix onto the microscope objective's field of view, where a photoresist-covered substrate is placed. The photoresist is exposed using blue light with a wavelength of 450 nm. To calibrate the device and adjust focal lengths, we utilize a red light that does not affect the photoresist. The substrate is located on a movable platform, allowing the exposure field to be shifted, enabling the exposure of designs with lateral sizes of 1 × 1 cm2 at a resolution of a few micrometers. Our setup showcases a 2 μm resolution for the single frame 200 × 100 μm2, and a 5 μm resolution for 1 × 1 cm2 with field stitching. The exposure speed, approximately 1 mm2/100 s, proves to be sufficient for a variety of laboratory prototyping needs. This system offers a significant advantage due to its utilization of easily accessible and budget-friendly components, thereby enhancing its accessibility for a broader user base. The exposure speed and resolution meet the requirements for laboratory prototyping in the fields of 2D materials, quantum optics, superconducting microelectronics, microfluidics, and biology.

Magic wavelengths for the 6S-7P transition of cesium atoms

For the trapped pre-cooled atoms in an optical dipole trap (ODT), the magic-wavelength ODT can eliminate the differential light shift of the transition between two atomic states, so that the transition frequency between the two states is the same as that of atoms in the free space, which is of great significance for improving the experimental repetition rate and reducing the atomic decoherence in the fields of cold atom physics, quantum optics, and precision measurement. Here we calculate the dynamic polarizabilities of cesium 6S ground state and 7P excited state by using the multi-level model for the ODT with laser wavelength from 1200 to 2000 nm. The magic wavelengths of ODT are obtained for the linearly and circularly polarized laser beams at the intersection of dynamic polarizabilities of two atomic states. Furthermore, we analyze the robustness of the magic trapping conditions and the feasibility of the experimental operation near the telecom C-band wavelength.

Phase estimation of a Mach-Zehnder interferometer via the Laguerre excitation squeezed state.

Quantum metrology has an important role in the fields of quantum optics and quantum information processing. Here we introduce a kind of non-Gaussian state, Laguerre excitation squeezed state as inputs of traditional Mach-Zehnder interferometer to examine phase estimation in realistic case. We consider the effects of both internal and external losses on phase estimation by using quantum Fisher information and parity detection. It is shown that the external loss presents a bigger effect than the internal one. The phase sensitivity and the quantum Fisher information can be improved by increasing the photon number and even surpass the ideal phase sensitivity by two-mode squeezed vacuum in a certain region of phase shift for realistic case. Our results can find significant practical applications in quantum metrology.

Unraveling time- and frequency-resolved nuclear resonant scattering spectra

A data analysis scheme for time- and frequency-resolved nuclear resonant scattering is proposed. It provides access to the resonance structure of M\"ossbauer samples and allows one to retrieve the phase-resolved nuclear resonant target response, which is of major interest in the rapidly developing field of x-ray quantum optics.

Nonequilibrium Hanbury Brown-Twiss interferometry: Theory and application to binary stars

Intensity interferometry based on Hanbury Brown and Twiss's seminal experiment for determining the radius of the star Sirius formed the basis for developing the quantum theory of light. To date, the principle of this experiment is used in various forms across different fields of quantum optics, imaging, and astronomy. Although the technique is powerful, it has not been generalized for objects at different temperatures. Here, we address this problem using a generating functional formalism by employing the $P$-function representation of quantum-thermal light. Specifically, we investigate the photon coincidences of a system of two extended objects at different temperatures using this theoretical framework. We show two unique aspects in the second-order quantum coherence function: interference oscillations and a long-baseline asymptotic value that depends on the observation frequency, temperatures, and size of both objects. We apply our approach to the case of binary stars and discuss the advantages of measuring these two features in an experiment. In addition to the estimation of the radii of each star and the distance between them, we also show that the present approach is suitable for the estimation of temperatures as well. To this end, we apply it to the practical case of binary stars Luhman 16 and Spica $\ensuremath{\alpha}$ Vir. We find that for currently available telescopes, an experimental demonstration is feasible in the near term. Our work contributes to the fundamental understanding of intensity interferometry of quantum-thermal light and can be used as a tool for studying two-body thermal emitters, from binary stars to extended objects.

Unconventional photon blockade in a non-Hermitian indirectly coupled resonator system.

Photon blockade provides an effective way to realize the single-photon source, which attracts intensive attention in the fields of quantum optics and quantum information. Here in this study, we investigate photon blockade in a non-Hermitian indirectly coupled resonator system, which consists of a dissipative cavity and a Kerr nonlinear resonator coupled to two nano-scatters. We find that by tuning the coupling phase θ between the two resonators, the quantum interference could be induced on one side near the exceptional points (EPs), resulting in the unconventional photon blockade effect. Furthermore, it is noticed that the large Kerr nonlinearity is not always beneficial for unconventional photon blockades. There is an optimal threshold for the intensity of the Kerr nonlinearity and the phase angle θ for the appearance of the unconventional photon blockade effect. We believe the current study has substantial consequences for investigating the physical characteristics close to EPs and presents a novel method for developing integrated on-chip single-photon sources.