Optical Nanocavities Research Articles

ZnO-Nanowire-Induced Nanocavities in Photonic Crystal Disks

We realize a novel type of nanowire-induced optical nanocavities based on photonic crystal disks, a design outperforming its one-dimensional and two-dimensional photonic crystal counterparts in ter...

Nanostructure-Enhanced Photoconductive Terahertz Emission and Detection.

Photoconductive antennas are commonly used for terahertz wave generation and detection. However, their relatively low radiation power and detection sensitivity often place limitations on the signal-to-noise ratio and operation bandwidth of terahertz imaging and spectroscopy systems. Several different techniques are attempted to address these limitations. The most promising ones take advantage of the unique tools provided by nanotechnology. In this review, the recent nanotechnology-enabled advances in photoconductive antennas, which use nanostructures, such as optical nanoantennas, plasmonic structures, and optical nanocavities, to increase the interaction of the optical pump beam with the photoconductive semiconductor, are discussed. All of these techniques are experimentally demonstrated to be efficient tools for enhancing the performance of photoconductive antennas for terahertz wave generation and detection.

Interaction and Coherence of a Plasmon–Exciton Polariton Condensate

Polaritons are quasiparticles arising from the strong coupling of electromagnetic waves in cavities and dipolar oscillations in a material medium. In this framework, localized surface plasmon in metallic nanoparticles defining optical nanocavities have attracted increasing interests in the past decade. This interest results from their sub-diffraction mode volume, which offers access to extremely high photonic densities by exploiting strong scattering cross sections. However, high absorption losses in metals have hindered the observation of collective coherent phenomena, such as condensation. In this work, we demonstrate the formation of a nonequilibrium room temperature plasmon–exciton–polariton condensate with a long-range spatial coherence, extending a hundred of microns, well over the excitation area, by coupling Frenkel excitons in organic molecules to a multipolar mode in a lattice of plasmonic nanoparticles. Time-resolved experiments evidence the picosecond dynamics of the condensate and a sizable blueshift, thus measuring for the first time the effect of polariton interactions in plasmonic cavities. Our results pave the way to the observation of room temperature superfluidity and novel nonlinear phenomena in plasmonic systems, challenging the common belief that absorption losses in metals prevent the realization of macroscopic quantum states.

Nanophotonics with 2D transition metal dichalcogenides [Invited

Two-dimensional semiconducting transition metal dichalcogenides (TMDCs) have recently become attractive materials for several optoelectronic applications, such as photodetection, light harvesting, phototransistors, light-emitting diodes, and lasers. Their bandgap lies in the visible and near-IR range, and they possess strong excitonic resonances, high oscillator strengths, and valley-selective response. Coupling these materials to optical nanocavities enhances the quantum yield of exciton emission, enabling advanced quantum optics and nanophotonics devices. Here, we review the state-of-the-art advances of hybrid exciton-polariton structures based on monolayer TMDCs coupled to plasmonic and dielectric nanocavities. We discuss the optical properties of 2D WS2, WSe2, MoS2 and MoSe2 materials, paying special attention to their energy bands, photoluminescence/absorption spectra, excitonic fine structure, and to the dynamics of exciton formation and valley depolarization. We also discuss light-matter interactions in such hybrid exciton-polariton structures. Finally, we focus on weak and strong coupling regimes in monolayer TMDCs-based exciton-polariton systems, envisioning research directions and future opportunities for this material platform.

Tunable Resonance Coupling in Single Si Nanoparticle-Monolayer WS2 Structures.

Two-dimensional semiconducting transition metal dichalcogenides (TMDCs) are extremely attractive materials for optoelectronic applications in the visible and near-infrared range. Coupling these materials to optical nanocavities enables advanced quantum optics and nanophotonic devices. Here, we address the issue of resonance coupling in hybrid exciton-polariton structures based on single Si nanoparticles (NPs) coupled to monolayer (1L)-WS2. We predict a strong coupling regime with a Rabi splitting energy exceeding 110 meV for a Si NP covered by 1L-WS2 at the magnetic optical Mie resonance because of the symmetry of the mode. Further, we achieve a large enhancement in the Rabi splitting energy up to 208 meV by changing the surrounding dielectric material from air to water. The prediction is based on the experimental estimation of TMDC dipole moment variation obtained from the measured photoluminescence spectra of 1L-WS2 in different solvents. An ability of such a system to tune the resonance coupling is realized experimentally for optically resonant spherical Si NPs placed on 1L-WS2. The Rabi splitting energy obtained for this scenario increases from 49.6 to 86.6 meV after replacing air by water. Our findings pave the way to develop high-efficiency optoelectronic, nanophotonic, and quantum optical devices.

Electrically tunable perfect light absorbers as color filters and modulators

Methods for spectrally controlling light absorption in optoelectronic devices have attracted considerable attention in recent years. It is now well known that a Fabry-Perot nanocavity comprising thin semiconductor and metal films can be used to absorb light at selected wavelengths. The absorption wavelength is controlled by tailoring the thickness of the nanocavity and also by nanostructure patterning. However, the realization of dynamically tuning the absorption wavelength without changing the structural geometry remains a great challenge in optoelectronic device development. Here it is shown how an ultrathin n-type doped indium antimonide integrated into a subwavelength-thick optical nanocavity can result in an electrically tunable perfect light absorber in the visible and near infrared range. These absorbers require simple thin-film fabrication processes and are cost effective for large-area devices without resorting to sophisticated nanopatterning techniques. In the visible range, a 40 nm spectral shift can be attained by applying a reasonable bias voltage to effect the color change. It is also shown that these electrically tunable absorbers may be used as optical modulators in the infrared. The predicted (up to) 95.3% change in reflectance, transforming the device from perfectly absorbing to highly reflective, should make this technology attractive to the telecommunication (switching) industry.

Quantum phase transition in a multiconnected Jaynes-Cummings lattice

The rapid progress in quantum technology enables the implementation of artificial many-body systems with correlated photons and polaritons. A multiconnected Jaynes-Cummings (MCJC) lattice can be constructed by connecting qubits and cavities alternatively. Such kind of models can be realized with superconducting qubits coupled to superconducting microwave resonators or with quantum dots coupled to optical nanocavities. We study physical properties of the one-dimensional MCJC lattice using the density-matrix renormalization group method. This model has an intrinsic symmetry between the left and right qubit-cavity couplings. The competition between these couplings may drive the ground state either to a Mott-insulating or to a superfluid phase at an integer filling. We calculate the single-particle and density-density correlation functions, the correlation lengths in the Mott-insulating phase and the Luttinger parameters in the superfluid phase, and determine accurately the critical points that separate these two phases.

Ultrasmall Mode Volumes of Multilayered Hyperbolic Metamaterial Nanocavities in the Visible Range

Designing optical nanocavities with high quality factors (Q) or small mode volume (Vm) has important applications in the field of quantum information due to the strong light-matter coupling phenomena. The multilayered hyperbolic metamaterial (HMM) nanocavities have been designed and numerically investigated to achieve the small mode volume. Unique dispersion relations of our HMM nanocavity enable propagation of large wave vectors result in strong wave confinement. The excitation of coupled localized surface plasmons, which have achieved ultrasmall mode volume below 10 –6 λ3 or high Q/Vm around 107 λ–3 causing better electric fields confinement. These properties can be demonstrated by rationally the geometrical parameters and may have potential applications in light-matter interaction.

Mixed‐Mode Electro‐Optical Operation of Ge2Sb2Te5 Nanoscale Crossbar Devices

The use of phase‐change materials for a range of exciting new optoelectronic applications from artificial retinas to ultrahigh‐resolution displays requires a thorough understanding of how these materials perform under a combination of optical and electrical stimuli. This study reports for the first time the complex link between the electronic and optical properties in real‐world crossbar nanoscale devices constructed by confining a thin layer of Ge2Sb2Te5 between transparent indium tin oxide electrodes, forming an optical nanocavity. A novel proof‐of‐concept device that can be operated by a combination of optical and electrical stimuli is presented, leading the way for the development of further applications based on mixed‐mode electro‐optical operation.

Control of Fano resonances and slow light using Bose-Einstein condensates in a nanocavity

In this study, a standing wave in an optical nanocavity with Bose-Einstein condensate (BEC) constitutes a one-dimensional optical lattice potential in the presence of a finite two bodies atomic interaction. We report that the interaction of a BEC with a standing field in an optical cavity coherently evolves to exhibit Fano resonances in the output field at the probe frequency. The behavior of the reported resonance shows an excellent compatibility with the original formulation of asymmetric resonance as discovered by Fano [U. Fano, Phys. Rev. 124, 1866 (1961)]. Based on our analytical and numerical results, we find that the Fano resonances and subsequently electromagnetically induced transparency of the probe pulse can be controlled through the intensity of the cavity standing wave field and the strength of the atom-atom interaction in the BEC. In addition, enhancement of the slow light effect by the strength of the atom-atom interaction and its robustness against the condensate fluctuations are realizable using presently available technology.

Super-wideband perfect solar light absorbers using titanium and silicon dioxide thin-film cascade optical nanocavities

Wideband perfect light absorbers covering visible and near-infrared solar optical radiations are significant for solar thermal energy systems. In this work, titanium and silicon dioxide multilayer thin film structures were investigated for perfect light absorption in wideband solar optical radiation spectral range from 400 nm to 2500 nm wavelength. Wideband solar light absorbers with different numbers of titanium and silicon dioxide layers and different layer thicknesses were designed, fabricated and characterized. It is found that the optimal wideband solar light absorber consists of only six titanium and silicon dioxide layers that form two cascade optical nanocavities, and increasing the number of optical cavities does not improve optical absorption in the solar spectrum. A super-wideband solar light absorber 97.97% total absorptance over the wavelength range from 400 nm to 1700 nm has been experimentally demonstrated.

Ultrasmall Mode Volumes in Plasmonic Cavities of Nanoparticle-On-Mirror Structures.

The mode volume and Purcell factor are two important parameters to assess the performance of optical nanocavities. Achieving small mode volumes and high Purcell factors for nanocavity structures while simplifying their fabrication has been a major task to realize high-performance and large-scale photonic devices and systems. Different optical resonators based on nanoparticle-on-mirror (NPoM) structures are systematically analyzed, which are easy to fabricate and flexible to use. Direct comparison of these optical resonators is made through finite-difference time-domain (FDTD) simulations. The achievement of ultrasmall mode volumes below 10-7 (λ/n)3 based on the NPoM structure through FDTD simulations is demonstrated by rationally selecting the structural parameters. Such NPoM structures provide a decent Purcell factor on the order of 107 , which can effectively enhance spontaneous emission and facilitate a number of photonic applications. The simulation results are confirmed by dark field scattering and second-harmonic generation measurements. This work is scientifically important and offers practical guidelines for the design of optical resonators for state-of-the-art optical and photonic devices.

Colored dual-functional photovoltaic cells

In this article, we review our recent efforts on multi-functional photovoltaic (PV) cells that can produce desired reflective, transmissive, or neutral colors, by controlling light interaction with semiconductors and electrode structures in a desired manner. The PV cells integrated with plasmonic color filtering schemes using subwavelength gratings, and other approaches exploiting photonic resonances in an optical nanocavity consisting of highly absorbing semiconductor media are described. For further enhancement of optical and electrical performance characteristics of the multi-functional PV cells, possible difficulties and the outlook for future work are discussed.

Zeroth order Fabry-Perot resonance enabled ultra-thin perfect light absorber using percolation aluminum and silicon nanofilms

We demonstrated perfect light absorption in optical nanocavities made of ultra-thin percolation aluminum and silicon films deposited on an aluminum surface. The total layer thickness of the aluminum and silicon films is one order of magnitude less than perfect absorption wavelength in the visible spectral range. The ratio of silicon cavity layer thickness to perfect absorption wavelength decreases as wavelength decreases due to the increased phase delays at silicon-aluminum boundaries at shorter wavelengths. It is explained that perfect light absorption is due to critical coupling of incident wave to the fundamental Fabry-Perot resonance mode of the structure where the round trip phase delay is zero. Simulations were performed and the results agree well with the measurement results.

High quality factor nanophotonic resonators in bulk rare-earth doped crystals.

Numerous bulk crystalline materials exhibit attractive nonlinear and luminescent properties for classical and quantum optical applications. A chip-scale platform for high quality factor optical nanocavities in these materials will enable new optoelectronic devices and quantum light-matter interfaces. In this article, photonic crystal nanobeam resonators fabricated using focused ion beam milling in bulk insulators, such as rare-earth doped yttrium orthosilicate and yttrium vanadate, are demonstrated. Operation in the visible, near infrared, and telecom wavelengths with quality factors up to 27,000 and optical mode volumes close to one cubic wavelength is measured. These devices enable new nanolasers, on-chip quantum optical memories, single photon sources, and non-linear devices at low photon numbers based on rare-earth ions. The techniques are also applicable to other luminescent centers and crystal.

Double-way spectral tunability for the control of optical nanocavity resonance.

Scanning Near-field Optical Microscopy (SNOM) has been successful in finely tuning the optical properties of photonic crystal (PC) nanocavities. The SNOM nanoprobes proposed so far allowed for either redshifting or blueshifting the resonance peak of the PC structures. In this paper, we theoretically demonstrate the possibility of a redshifting (up to +0.65 nm) and a blueshifting (up to −5 nm) the PC cavity resonance wavelength with a single perturbation element. As an example, a fiber bowtie-aperture nano-antenna (BNA) engraved at the apex of a SNOM tip is proposed to play this role. The double-way tunability is the result of a competition between an induced electric dipole (BNA at resonance) leading to a redshift and an induced magnetic dipole (the tip metalcoating) giving rise to a blueshift of the resonance wavelength. We demonstrate that the sign of the spectral shift can be simply controlled through the tip-to-cavity distance. This study opens the way to the full postproduction control of the resonance wavelength of high quality-factor optical cavities.

Tunable Optical Nanocavity of Iron-garnet with a Buried Metal Layer

We report on the fabrication and characterization of a novel magnetophotonic structure designed as iron garnet based magneto-optical nanoresonator cavity constrained by two noble metal mirrors. Since the iron garnet layer requires annealing at high temperatures, the fabrication process can be rather challenging. Special approaches for the protection of metal layers against oxidation and morphological changes along with a special plasma-assisted polishing of the iron garnet layer surface were used to achieve a 10-fold enhancement of the Faraday rotation angle (up to 10.8°/µm) within a special resonance peak of 12 nm (FWHM) linewidth at a wavelength of 772 nm, in the case of a resonator with two silver mirrors. These structures are promising for tunable nanophotonics applications, in particular, they can be used as magneto-optical (MO) metal-insulator-metal waveguides and modulators.

High quality-factor optical nanocavities in bulk single-crystal diamond.

Single-crystal diamond, with its unique optical, mechanical and thermal properties, has emerged as a promising material with applications in classical and quantum optics. However, the lack of heteroepitaxial growth and scalable fabrication techniques remains the major limiting factors preventing more wide-spread development and application of diamond photonics. In this work, we overcome this difficulty by adapting angled-etching techniques, previously developed for realization of diamond nanomechanical resonators, to fabricate racetrack resonators and photonic crystal cavities in bulk single-crystal diamond. Our devices feature large optical quality factors, in excess of 105, and operate over a wide wavelength range, spanning visible and telecom. These newly developed high-Q diamond optical nanocavities open the door for a wealth of applications, ranging from nonlinear optics and chemical sensing, to quantum information processing and cavity optomechanics.

A chemical sensor based on a photonic-crystal L3 nanocavity defined in a silicon-nitride membrane

The application of a silicon-nitride based L3 optical nanocavity as a chemical sensor is explored. It is shown that by adjusting the thickness of an ultra-thin Lumogen Red film deposited onto the nanocavity surface, the fundamental optical mode undergoes a progressive red-shift as the layer-thickness increases, with the cavity being able to detect the presence of a single molecular monolayer. The optical properties of a nanocavity whose surface is coated with a thin layer of a porphyrin-based polymer are also explored. On exposure of the cavity to an acidic-vapour, it is shown that changes in the optical properties of the porphyrin-film (thickness and refractive index) can be detected through a reversible shift in the cavity mode wavelength. Such effects are described using a finite difference time-domain model.

Ultrafast spontaneous emission of copper-doped silicon enhanced by an optical nanocavity

Dopants in silicon (Si) have attracted attention in the fields of photonics and quantum optics. However, the optical characteristics are limited by the small spontaneous emission rate of dopants in Si. This study demonstrates a large increase in the spontaneous emission rate of copper isoelectronic centres (Cu-IECs) doped into Si photonic crystal nanocavities. In a cavity with a quality factor (Q) of ~16,000, the photoluminescence (PL) lifetime of the Cu-IECs is 1.1 ns, which is 30 times shorter than the lifetime of a sample without a cavity. The PL decay rate is increased in proportion to Q/Vc (Vc is the cavity mode volume), which indicates the Purcell effect. This is the first demonstration of a cavity-enhanced ultrafast spontaneous emission from dopants in Si, and it may lead to the development of fast and efficient Si light emitters and Si quantum optical devices based on dopants with efficient optical access.