Nonresonant Regime Research Articles

Non-resonant tunnelling in short-period superlattices with optical cavities

The vertical transport in short-period InAs/AlSb and GaAs/AlAs superlattices was studied. The negative differential conductivity was observed in a miniband transport regime as a result of the overlapping of confined states in a periodic quantum well structure (Esaki-Tsu mechanism). Several maxima appeared on current–voltage characteristics of the superlattices found in the non-resonant tunnelling regime. They are shown to be due to the influence of the optical cavity on optical transitions within quantum wells (Purcell effect).

Non-resonant tunnelling in short-period superlattices with optical cavities

The vertical transport in short-period InAs/AlSb and GaAs/AlAs superlattices was studied. The negative differential conductivity was observed in a miniband transport regime as a result of the overlapping of confined states in a periodic quantum well structure (Esaki-Tsu mechanism). Several maxima appeared on current–voltage characteristics of the superlattices found in the non-resonant tunnelling regime. They are shown to be due to the influence of the optical cavity on optical transitions within quantum wells (Purcell effect).

Vibrationally induced decoherence in single-molecule junctions

We investigate the interplay of quantum interference effects and electronic-vibrational coupling in electron transport through single-molecule junctions, employing a nonequilibrium Green's function approach. Our findings show that inelastic processes lead, in general, to a quenching of quantum interference effects. This quenching is more pronounced for increasing bias voltages and levels of vibrational excitation. As a result of this vibrationally induced decoherence, vibrational signatures in the transport characteristics of a molecular contact may strongly deviate from a simple Franck-Condon picture. This includes signatures in both the resonant and the non-resonant transport regime. Moreover, it is shown that local cooling by electron-hole pair creation processes can influence the transport characteristics profoundly, giving rise to a significant temperature dependence of the electrical current.

Photon-assisted entanglement creation by minimum-error generalized quantum measurements in the strong-coupling regime

We explore possibilities of entangling two distant material qubits with the help of an optical radiation field in the regime of strong quantum electrodynamical coupling with almost resonant interaction. For this purpose the optimum generalized field measurements are determined which are capable of preparing a two-qubit Bell state by postselection with minimum error. It is demonstrated that in the strong-coupling regime some of the recently found limitations of the non-resonant weak-coupling regime can be circumvented successfully due to characteristic quantum electrodynamical quantum interference effects. In particular, in the absence of photon loss it is possible to postselect two-qubit Bell states with fidelities close to unity by a proper choice of the relevant interaction time. Even in the presence of photon loss this strong-coupling regime offers interesting perspectives for creating spatially well-separated Bell pairs with high fidelities, high success probabilities, and high repetition rates which are relevant for future realizations of quantum repeaters.

Near resonant and nonresonant third-order optical nonlinearities of colloidal InP/ZnS quantum dots

We have investigated the third-order optical nonlinearities of high-quality colloidal InP/ZnS core-shell quantum dots (QDs) using Z-scan technique with femtosecond pulses. The two-photon absorption cross-sections as high as 6.2 × 103 GM are observed at 800 nm (non-resonant regime) in InP/ZnS QDs with diameter of 2.8 nm, which is even larger than those of CdSe, CdS, and CdTe QDs at similar sizes. Furthermore, both of the 2.2 nm and 2.8 nm-sized InP/ZnS QDs exhibit strong saturable absorption in near resonant regime, which is attributed to large exciton Bohr radius in this material. These results strongly suggest the promising potential of InP/ZnS QDs for widespread applications, especially in two-photon excited bio-imaging and saturable absorbing.

Surface plasmon assisted optical nonlinearities of uniformly oriented metal nano-ellipsoids in glass

The nonlinear optical properties of nanocomposites consisting of non-spherical silver nanoparticles in glass matrix have been studied using the femtosecond Z-scan technique. The spheroidal nanoparticles were uniformly oriented along a common direction. By polarization sensitive studies, longitudinal and transverse plasmon resonances can be addressed separately. A sign reversal in optical nonlinearity from negative to positive is observed while switching the light interaction from near to non-resonant regime, which can be done by simply rotating the light polarization by 90°. Studying samples with different aspect ratio, we obtained the dispersion of third-order nonlinearity in the near-resonant regime, showing an enhancement of the nonlinear processes by more than two orders of magnitude due to the electric field enhancement at the surface plasmon resonance.

Ab initiocomplex band structure of conjugated polymers: Effects of hydrid density functional theory andGWschemes

The non-resonant tunneling regime for charge transfer across nanojunctions is critically dependent on the so-called \beta{} parameter, governing the exponential decay of the current as the length of the junction increases. For periodic materials, this parameter can be theoretically evaluated by computing the complex band structure (CBS) -- or evanescent states -- of the material forming the tunneling junction. In this work we present the calculation of the CBS for organic polymers using a variety of computational schemes, including standard local, semilocal, and hybrid-exchange density functionals, and many-body perturbation theory within the GW approximation. We compare the description of localization and \beta{} parameters among the adopted methods and with experimental data. We show that local and semilocal density functionals systematically underestimate the \beta{} parameter, while hybrid-exchange schemes partially correct for this discrepancy, resulting in a much better agreement with GW calculations and experiments. Self-consistency effects and self-energy representation issues of the GW corrections are discussed together with the use of Wannier functions to interpolate the electronic band-structure.

Time-dependent pointer states and decoherence of the quantized atom-field model in a nonresonant regime

We consider the quantized atom-field model and for the regime ; where , and respectively represent the self-Hamiltonians of the environment, the system, and the interaction between the system and the environment. Considering a single-mode quantized field we obtain the time evolution operator for the model. Using our time evolution operator we calculate the time-dependent pointer states of the system and the environment, which are characterized by their property of not entangling with states of another subsystem. We obtain a closed form expression for the off-diagonal element of the reduced density matrix of the system and study the decoherence of the central system in our model. We show that for the case where the system initially is not prepared in one of its pointer states, the off-diagonal element of the reduced density matrix of the system decays with a decoherence time that is inversely proportional to the square root of the mass of the bosonic field particles.

Comportamiento dinámico de viaductos cortos considerando la interacción vehículo-vía-estructura-suelo

The dynamic vehicle-track-bridge-soil interaction is studied on high speed lines. The analysis is carried out using a general and fully three dimensional multi-body-finite element-boundary element model, formulated in the time domain to predict vibrations due to the train passage over the bridge. The vehicle is modelled as a multi-body system, the track and the bridge are modelled using finite elements and the soil is considered as a homogeneous half-space by the boundary element method. Usually, moving force model and moving mass model are employed to study the dynamic response of bridges. In this work, the multi-body system allows one to consider the quasi-static and dynamic excitation mechanisms. Soil-structure interaction is taken into account on the dynamic structure behaviour on simply-supported short span bridges. The influence of soil-structure interaction is analysed in both resonant and non-resonant regimes.

Off-resonance and non-resonant dispersion of Kerr nonlinearity for symmetric molecules [Invited

The exact formula is derived from the "sum over states" (SOS) quantum mechanical model for the frequency dispersion of the nonlinear refractive index coefficient n₂ for centrosymmetric molecules in the off-resonance and non-resonant regimes. This expression is characterized by interference between terms from two-photon transitions from the ground state to the even-symmetry excited states and one-photon transitions between the ground state and odd-symmetry excited states. When contributions from the two-photon terms exceed those from the one-photon terms, the non-resonant intensity-dependent refractive index n₂>0, and vice versa. Examples of the frequency dispersion for the three-level SOS model are given. Comparison is made with other existing theories.

Vibration Control of a Cylindrical Shell Structure Using Macro Fiber Composite Actuators

We studied the vibration suppression of an end-capped cylindrical shell structure with surface bonded macro fiber composite actuators. The dynamic characteristics of the cylindrical shell structure were first analyzed, and then a negative velocity feedback algorithm was applied to suppress the structural vibration at resonance and nonresonance vibration frequencies. The modal mass and stiffness matrix of the smart cylindrical shell structure were extracted for the controller design. An active controller was designed to suppress vibration of the smart structure, and the control performance was evaluated in resonance and nonresonance regimes. It was found that structural vibration was reduced by adopting a proper negative velocity feedback control algorithm in both resonance and nonresonance regimes.

A thioester substrate binds to the enzyme Arthrobacter thioesterase in two ionization states: evidence from Raman difference spectroscopy

4-Hydroxybenzoyl-CoA (4-HB-CoA) thioesterase from Arthrobacter is the final enzyme catalyzing the hydrolysis of 4-HB-CoA to produce coenzyme A and 4-hydroxybenzoic acid in the bacterial 4-chlorobenzoate dehalogenation pathway. Using a mutation E73A that blocks catalysis, stable complexes of the enzyme and its substrate can be analyzed by Raman difference spectroscopy. Here we have used Raman difference spectroscopy, in the non-resonance regime, to characterize 4-HB-CoA bound in the active site of the E73A thioesterase. In addition we have characterized complexes of the wild-type enzyme complexed with the unreactive substrate analog 4-hydroxyphenacyl-CoA (4-HP-CoA). Both sets of complexes show evidence for two forms of the ligand in the active site, one population has the 4-hydroxy group protonated, 4-OH, while the second has the group as the hydroxide, 4-O(-). For bound 4-HP-CoA X-ray data show that glutamate 78 is close to the 4-OH in the complex and it is likely that this is the proton acceptor for the 4-OH proton. Although the pK(a) of the 4-OH group on the free substrate in aqueous solution is 8.6, the relative populations of ionized and neutral 4-HB-CoA bound to E73A remain invariant between pH 7.3 and pH 9.8. The invariance with pH suggests that the 4-OH and the -COO(-) of E78 constitute a tightly coupled pair where their separate pK(a)s lose their individual qualities. Narrow band profiles are seen in the C=O double bond and C-S regions suggesting that the hydrolyzable thioester group is rigidly bound in the active site in a syn gauche conformation.

A Godunov-type method for the shallow water equations with discontinuous topography in the resonant regime

We investigate the Riemann problem for the shallow water equations with variable and (possibly) discontinuous topography and provide a complete description of the properties of its solutions: existence; uniqueness in the non-resonant regime; multiple solutions in the resonant regime. This analysis leads us to a numerical algorithm that provides one with a Riemann solver. Next, we introduce a Godunov-type scheme based on this Riemann solver, which is well-balanced and of quasi-conservative form. Finally, we present numerical experiments which demonstrate the convergence of the proposed scheme even in the resonance regime, except in the limiting situation when Riemann data precisely belong to the resonance hypersurface.

Excitation Mechanisms of CdTe/ZnTe Quantum Dots under Non-Resonant and Quasi-Resonant Regime

Excitation Mechanisms of CdTe/ZnTe Quantum Dots under Non-Resonant and Quasi-Resonant Regime T. Kazimierczuka,∗, J.A. Gaj , A. Golnik, M. Goryca, M. Nawrocki, M. Koperski, T. Smolenski, J. Suffczynski, P. Wojnar and P. Kossacki Institute of Experimental Physics, Faculty of Physics, University of Warsaw, Hoza 69, 00-681 Warsaw, Poland Institute of Physics, Polish Academy of Sciences, al. Lotnikow 32/46, 02-668 Warsaw, Poland Grenoble High Magnetic Field Laboratory, CNRS, BP 166, 38042 Grenoble Cedex 9, France We discuss possible mechanisms of quantum dot population control. A set of experiments, including time-resolved photoluminescence, single photon correlations, excitation correlation, and photoluminescence excitation is used to determine the actual mechanism under non-resonant and quasi-resonant regime.

Modelling of the neoclassical toroidal plasma viscosity torque in tokamaks

Neoclassical toroidal plasma viscosity (NTV) torque induced by non-axisymmetric magnetic perturbation in the collisionless regimes in tokamaks is modelled by solving the bounce-averaged drift kinetic equation numerically. The detailed comparison between the numerical and the analytic solutions of NTV is discussed in this paper. In different asymptotic limits of the collisionless regimes, the numerical solutions are in good agreement with the analytic results. The numerical results are different from the analytic results calculated from the smoothly connected formula in the transit regimes. The pitch angle scattering is especially important in the regime. The final difference between the numerical and the analytic results can be up to a factor of 2 near the transition between the non-resonant and resonant regimes. This reveals the importance of the boundary condition of the pitch angle space. The sign of the electric field is found to be important in the calculation of the NTV torque. It shows that the effect of the resonant particles makes the NTV torque more important for the lower collisionality and lower rotation cases, which are the International Thermonuclear Experimental Reactor relevant conditions. It also shows that the electron NTV torque is important in the low collisionality case. This numerical method can be applied for modelling the NTV torque in different collisionality regimes and their transitions in tokamaks without additional approximations.

Asymptotic estimates and stability analysis of Kuramoto-Sivashinsky type models

We first show asymptotic L2 bounds for a class of equations, which includes the Burger-Sivashinsly model for odd solutions with periodic boundary conditions. We consider the conditional stability of stationary solutions of Kuramoto-Sivashinsky equation in the periodic setting. We establish rigorously the general structure of the spectrum of the linearized operator, in particular the linear instability of steady states. In addition, we show conditional asymptotic stability with asymptotic phase, under a natural spectral hypothesis for the corresponding linearized operator. For the zero solution, we have more precise results. Namely, in the non-resonant regime L ≠ nπ, we prove conditional asymptotic stability, provided one considers only mean value zero data. If, however, L = n0π (but still \({\int\nolimits_{-L}^L u_0(x) dx=0}\)), then we have conditional orbital stability. More specifically, the solutions relax to a small (but generally non-zero) function as long as the initial data are small and lie on a center-stable manifold of codimension 2(n0 − 1).

SH-wave propagation and resonance phenomena in a periodically layered composite structure with a crack

This paper presents a dynamic analysis of time-harmonic plane SH-waves propagating in periodically multilayered elastic composites with a strip-like crack. The total wave field in the multilayered elastic structure is described as a sum of incident wave field modeled by the transfer matrix method and the scattered wave field governed by an integral representation containing the crack-opening-displacement. The integral equation derived from the boundary conditions on the crack-faces is solved numerically by a Galerkin method. The paper focuses on resonant and non-resonant regimes of anti-plane wave motion in a stack of elastic layers weakened by a single strip-like crack and wave localization in the vicinity of the crack. The scattered extra displacement induced by the presence of the crack is investigated in detail for both situations of high and low contrast in material properties. Numerical results for the average crack-opening-displacement, the transmission coefficient, the stress intensity factor and the average energy flow are presented and discussed to reveal wave resonance and localization phenomena within the band-gaps and the pass-bands.

Organic-inorganic magnetic tunnel heterojunctions based on dithiapyrannylidene ultrathin films grown on Fe3O4(111)

We report on the morphology, transport, and magnetic properties of ultrathin films of 4,4′-bis(diphenyl-2,6-thiapyrannylidene) (DITPY-Ph4), a planar quinoïd organic compound with potential applications in electronics. Atomic force microscopy (AFM) shows that highly homogeneous and continuous DITPY-Ph4 ultrathin films with thicknesses as low as 2 nm can be grown on epitaxial Fe3O4(111). Current-sensing AFM performed on ultrathin layers evidences an insulating behavior with a nonresonant tunneling conduction regime. Vibrating sample magnetometry achieved on Fe3O4/DITPY-Ph4/Co organic-inorganic heterojunctions reveals the decoupling between the two magnetic electrodes and demonstrates that DITPY-Ph4 can be used to build magnetic tunnel junctions.

Nonlinear optical studies in semiconductor-doped glasses under femtosecond pulse excitation

Nonlinear optical studies in semiconductor-doped glasses (SDGs) are performed under femtosecond laser pulse excitation. Z-scan experiments with 800 nm wavelength pulses are used to excite SDG samples in the resonance and non-resonance regimes. Schott colour glass filter OG 515 shows stronger two-photon absorption than GG 420 and both the samples exhibit positive nonlinearity. However, in resonantly excited RG 850 the intensity-dependent Z-scan shows transition from saturable to reverse saturable absorption behaviour with the increase in intensity.

High Order Symmetry Structural Properties of Vibrational Resonances Using Multiple-Field Polarization Coherent Anti-Stokes Raman Spectroscopy Microscopy

Polarization-resolved coherent anti-Stokes Raman scattering (CARS) is usually applied to measure the depolarization ratio in solutions or evidence orientation effects in anisotropic media. We present an extensive approach based on multiple-field polarization-resolved CARS, in order to unravel the complexity of vibrational resonances up to the fourth-order symmetry, at the microscopic scale in nonisotropic media. The CARS polarized signals measured under a continuous variation of the incident pump and/or Stokes excitation beams are analyzed using a full tensorial picture both in the nonresonant and resonant regimes. This method evidences the strong influence of vibrational symmetries on polarized CARS, and more specifically the occurrence of Kleinman symmetry deviations at the vicinity of the Raman lines frequencies. This technique, illustrated on a cubic symmetry crystal, is general and can be applied to other medium symmetries.