Nonlinear Refractive Index Changes Research Articles

Linear and Nonlinear Optical Properties of Symmetric and Asymmetric Double Triangular Quantum Dots Withinside the Presence of Magnetic Field

AbstractLinear and third‐order nonlinear optical absorption coefficients and relative refractive index changes in symmetric and asymmetric double triangular quantum dots are examined theoretically. The dependence of these optical properties on the magnetic field is examined. After calculating energies and wave functions within the effective mass and parabolic band approaches, analytical expressions of linear and nonlinear optical properties are obtained using the compact density matrix approach and iterative method. Numerical calculations are presented for typical GaAs/AlGaAs material. The results show that the magnetic field causes different effects on the and transitions. Moreover, the calculated results also reveal that the resonance frequency and nonlinear contribution are different in symmetric and asymmetric structures. As a result, it is concluded that the magnetic field plays a vital and important role in the electronic and optical properties of the system and can be used to tune the inter‐subband transitions and change the corresponding optical sensitivities.

Electric field-induced modulation of electronic and optical properties in doped CdTe/CdS core/shell quantum dots embedded in an oxide matrix

This work presents a theoretical analysis of a CdTe/CdS core/shell quantum dots embedded in a dielectric oxide matrix under the influence of hydrogenic impurity and the applied electric field intensity. The eigenstates and their corresponding eigenfunctions are computed by solving the Schrodinger equation using the finite element method within the effective mass approximation. The first-order linear and third-order nonlinear optical absorption coefficients as well as the refractive index changes are computed based on the compact density matrix approach. The obtained result shows that the first-order linear and third-order nonlinear optical properties are more pronounced with the electric field, surrounding oxide matrix and the donor impurity effects. However, the first-order linear and third-order nonlinear optical absorption coefficients and refractive index changes can experience a red or blue shift under the influence of electric field, oxide matrix and hydrogenic impurity. In addition, under all conditions, the height peaks of these optical properties can be raised (fall). Our findings demonstrate the critical importance of considering the roles of electric field, the presence of donor impurity, and the capped dielectric oxide matrix in the design and fabrication of core–shell-based optoelectronic devices.

The effect of hydrostatic pressure, temperature and impurity factor on linear and nonlinear optical properties of InxGa1-xAs tuned quantum dot with modified Gaussian potential under the action of a vertical magnetic field

This study presents a detailed theoretical analysis of the effects of hydrostatic pressure, temperature, impurity factors, and external electric fields on the optical properties of InxGa1-xAs tuned quantum dot. A uniform magnetic field, directed perpendicular to the quantum dot plane, is applied. The system is excited using a monochromatic electromagnetic field, considering electron intersubband transitions. Energy levels and wave functions are determined using the parabolic band approximation and effective mass approximation. The linear and nonlinear optical absorption coefficients and refractive index changes are computed using the compact-density matrix approach and the iterative method. Numerical results indicate that the peaks of the linear and nonlinear optical absorption coefficients and refractive index changes shift towards lower energies (red shift) and higher energies (blue shift) under varying hydrostatic pressure, temperature, and impurity factor strength. Additionally, the peak values of the absorption coefficients and refractive index changes increase or decrease based on these parameter variations. These results have significant implications for the design and optimization of quantum dot-based optoelectronic devices.

Optical solitons for the dispersive concatenation model with power law of self-phase modulation: undetermined coefficients

AbstractThis paper recovers 1-soliton solutions to the dispersive concatenation model that comes with power law of self-phase modulation. The method of undetermined coefficients has made this retrieval possible. The parameter constraints are listed for the existence of the solitons. While a full spectrum of solitons is enumerated and exhibited, it is proved that dark 1-solitons exist only for Kerr law of nonlinear refractive index change.

Investigation of linear and nonlinear optical properties in quantum dots: Influence of magnetic and AB flux fields

In the present work, analytical expressions for the energy eigenvalues and eigen functions are obtained by solving the radial Schrödinger equation for inverse quadratic Hellmann plus Yukawa (IQHY) potential using Nikiforov-Uvarov functional analysis method. As an application part of this work, expressions for the linear and third-order nonlinear absorption coefficients and refractive index changes are computed to study the optical properties of the spherical GaAs quantum dots. We extend the investigation of the IQHY potential by incorporating the effects of magnetic and Aharonov–Bohm (AB) flux fields. Our results reveal that the optical properties of the GaAs quantum dots are strongly influenced by variations in the dot radius, potential height and intensity of incident photons. Specifically, we observe that the introduction of magnetic and AB flux fields significantly alters the energy eigenvalues and eigenfunctions, leading to distinct optical characteristics. The results of present study are found in consistent with other theoretical studies available in the literature.

Optical and electronic properties of a two-dimensional quantum ring under rotating effects

This work presents a theoretical study on the effects of rotation on the nonrelativistic quantum motion of a charged particle confined to a 2D ring in the presence of the Aharonov–Bohm effect and a uniform magnetic field. We formulate the Schrödinger equation with minimal coupling, incorporating the gauge field for the rotating frame and the potential vector of the electromagnetic field. By solving the equation of motion, we determine the eigenvalues and eigenfunctions of the particle. We analyze the probability distribution as a function of varying rotating parameter values and observe a perceptible shift in the distribution. This shift indicates a higher probability of locating the electron at the edges of the ring. The second part of our study focuses on the investigation of rotation effects on the linear and nonlinear optical properties of the system. Specifically, we examine the linear, nonlinear, and total refractive index changes, as well as the optical absorption coefficients. Through numerical analysis, we demonstrate significant rotating effects on energy levels and optical properties. Our findings indicate that, for the considered physical parameters, the impact of rotation on the optical properties becomes prominent at values on the order of a few terahertz.

Synthesis, Surface Morphology, Gas Sensor, DSC Technique and Third-Order Behavior of Conducting Polymer.

The compound polyaniline (Poly-ANI) with different concentrations of (H2SO4) sulfuric acid has been synthesized by the chemical polymerization method. The prepared compounds have been characterized using number of techniques including FTIR, FE-SEM, EDS and DSC. Additionally, UV-Vis spectroscopy employed for studying the linear optical properties of polymer with different acid concentrations. Third order optical nonlinearity was characterized using Z-scan at 532nm. The results showed that the nonlinear refractive index has a negative sign. It was observed that the nonlinear refractive index changes in different ratios of H2SO4. The high value of nonlinear refractive index ( ) obtained along Z-axis is cm2/W, and the corresponding is 21.5 × 10-5 esu. Also, the Poly-ANI film shows the response to NH3 gas sensing in the range 20ppm-250ppm and can be used for NH3 sensing application.

Impact of intense laser Bessel beam on excitonic complexes in ellipsoidal quantum dot

This theoretical study investigates the response of a strongly oblate GaAs ellipsoidal quantum dot to an intense laser field with a Bessel intensity profile at non-resonant extreme violet and simultaneously resonant mid-infrared laser irradiation. Mainly, the linear and nonlinear optical properties of biexcitons in quantum dot are observed. Due to the complexity of the considered particle, all calculations are performed in the framework of the variational method. Biexciton variational function is constructed on the one-particle wave functions, which are correlated with each other by exponents with variational parameters. The biexciton energies for different values of applied intense laser field magnitude on the small geometrical parameter of ellipsoidal quantum dot are calculated. The nonlinear optical properties, including the oscillator strength, third-order nonlinear susceptibility, absorption coefficient, and refractive index change, are evaluated. Numerical results reveal the dependence of the exciton and biexciton energies on the intensity of the laser field and the geometrical parameters of the quantum dot. Additionally, the dependencies of the third-order susceptibility, absorption coefficient, and induced refractive index change on photon energy near the one-photon resonance and two-photon resonance are analyzed. The two-photon absorption coefficient of the biexciton in GaAs ellipsoidal quantum dot is computed, and the spectra of refractive index changes induced by biexciton transitions between ground states are analyzed for different magnitudes of the intense laser field. Biexciton recombination radiative lifetime on the small semiaxis of the ellipsoidal quantum dot for the different values of the laser field influence is estimated. Finally, the visualization of the localization region of biexciton in the ellipsoidal quantum dot is performed.

Linear and nonlinear optical absorption coefficients and refractive index changes of GaAs/GaAsSb/GaAs V-shaped quantum wells affected by intense laser fields

Linear and nonlinear optical absorption coefficients and refractive index changes of GaAs/GaAsSb/GaAs V-shaped quantum wells affected by intense laser fields

Nonlinear absorption coefficient and relative refractive index change for Konwent potential quantum well as a function of intense laser field effect

Nonlinear absorption coefficient and relative refractive index change for Konwent potential quantum well as a function of intense laser field effect

Nonlinear optical properties in GaAs/Ga0.7Al0.3As spherical quantum dots with Like-Deng-Fan-Eckart potential

The effects of several key factors on the nonlinear optical properties of spherical quantum dots (QDs) with like-Deng-Fan-Eckart potential are studied theoretically, aiming at nonlinear optical absorption coefficients (OACs) and refractive index changes (RICs). By using the Factorization method to solve the Schrödinger equation, the dependent wave functions and energy levels are determined, and the analytical expressions of OACs and RICs are obtained by making use of the iterative method and density-matrix theory. It is worth noting that the numerical results show that the radius of QDs, the depth of limiting potential and the tuned effective mass have an enormous impact on the peaks and formants of OACs and RICs.

Investigation on nonlinear optical properties of symmetric and asymmetric double V-shaped AlxGa1-xAs/GaAs potential wells with structural parameters and external electromagnetic fields

ABSTRACT Linear, nonlinear and total optical absorption coefficients and relative refractive index changes for symmetric and asymmetric double V-shaped quantum well configurations formed within AlxGa1-xAs/GaAs heterostructure have been theoretically investigated. Responses of these coefficients to well widths, barrier widths and aluminium concentrations within the barrier as well as applied external electromagnetic fields were the subject of this study. The electronic spectra of the structures are obtained as a solution to the Schrödinger equation with relevant potential and external agents in the framework of effective mass and envelope wave function approximations. The optical properties are calculated by the analytical expressions obtained by iterative solutions within the compact density matrix approach. Although increasing barrier width and aluminium concentration act similarly significant red shifting on the referred coefficients for both symmetric and asymmetric double V-shaped wells, the varying well widths act differently for each configuration. Strengthening electric and magnetic fields shift the resonance peaks to blue for both symmetric and asymmetric wells. The results show that optical properties can be controlled by structural parameters, external probes and asymmetry of double V-shaped wells.

Effects of the confinement potential parameters and optical intensity on the linear and nonlinear optical properties of spherical quantum dots

We study the linear and nonlinear optical properties of a spherical GaAs quantum dot with screened modified Kratzer potential (SMKP) by solving the time-independent Schrödinger wave equation using the diagonalization method. The obtained electronic properties of the system alongside the compact density formalism are used to evaluate the linear, third-order nonlinear and total optical absorption coefficients and change in the relative refractive index of the system. We show that the confinement potential parameters and optical intensity significantly affects the behaviour of absorption coefficients and refractive index changes. It is important to note that the findings of this study will find application in optoelectronics and related areas.

Theoretical investigation of laser field effect on nonlinear optical properties of quantum dots

In this work, we have theoretically investigated the effects of a high-frequency intense laser field on the nonlinear optical properties of a two-dimensional Gaussian quantum dot system. A non-resonant monochromatic intense laser field with circular polarization applied to the system is considered in the framework of a non-perturbative approach. The nonlinear optical properties of the system have been investigated by using the compact-density matrix approach and iterative procedure. The laser field effect on the linear and the third-order nonlinear absorption coefficients and refractive index changes have been examined. Results reveal that the optical characteristics of the two-dimensional Gaussian quantum dot system are considerably influenced by the strength of the intense laser field in addition to structure parameters.

Investigation of Biexciton Induced Linear and Nonlinear Refractive Index Changes in Ellipsoidal Quantum Dot

Investigation of Biexciton Induced Linear and Nonlinear Refractive Index Changes in Ellipsoidal Quantum Dot

Ecofriendly Perovskites with Giant Self‐Defocusing Optical Response

AbstractThe full optical control of light using sustainable green technologies is one of the incipient challenges of the Photonics community. There are, however, few optical materials able to provide a significant nonlinear refractive index change under small enough intensities (< 1 GW cm−2), and, more importantly, allowing the external control of the magnitude and sign of their nonlinear response. This manuscript demonstrates that Cs2SnI6 lead‐free nanocrystals (NCs) present an extraordinary self‐defocusing response not yet observed up to now in any material. Despite its complex structural form, these NCs are fully characterized here, both experimentally and theoretically, revealing a giant negative refractive change Δn = −0.05 under proper illumination conditions. The nonlinear response is tuned with the intensity, concentration of NCs in the solvent, and propagation distance leading to a crossover where the media transforms to self‐focusing with Δn = +0.002. These results can provide fascinating opportunities in sensing and light–matter interactions for a future ecofriendly photonic technology.

Dynamics Simulation and Experimental Investigation of Q-Switching in a Self-Mode-Locked Semiconductor Disk Laser

Q-switching in a mode-locked laser not only makes the amplitude of every single output pulse unequal, but also limits the time width and peak power of output pulses. This paper investigates the Q-switching in a self-mode-locked semiconductor disk laser numerically and experimentally. By using the delay differential equations for passively mode-locking, conditions of Q-switching in a self-mode-locked semiconductor disk laser are numerically analyzed for the first time. Meanwhile, based on the experimental results, the causes of Q-switching tendency including the change of nonlinear refractive index and the change of soft aperture, are also discussed. Some possible measures to suppress Q-switching instability, i.e., to obtain stable continuous-wave mode-locking in a self-mode-locked semiconductor disk laser are proposed.

Investigation of linear and nonlinear optical absorption coefficients and refractive index changes of a zigzag quantum well with structure parameters and applied external fields

In this study, we have investigated some linear and nonlinear optical properties of GaAs/GaAlAs zigzag quantum well structures under different electric and magnetic field intensities. We also examined the effect of adjustable structural parameters as well as width on the optical response of the system. The diagonalization method has been the tool to numerically solve the effective mass approximation Schrödinger equation obtaining the energy levels and related wave functions needed to evaluate the expressions of linear, third-order nonlinear, and total optical absorption coefficients and relative refractive index changes derived within the compact density matrix method. Results show that the optical response becomes blue-shifted with the applied electric and magnetic fields’ increment.

Anisotropic photoelectric properties in GaN/AlN quantum dots under terahertz laser polarization

The linear and nonlinear anisotropic optical absorption coefficients(OACs) and refractive index changes(RICs) of GaN/AlN cubical quantum dots(CQDs) subjected to terahertz laser field(TLF) are investigated. The results show that under the polarization of TLF, with the increase of laser dressing parameters, the peak of OACs and RICs increases nonlinearly and have a redshift. More importantly, our work indicated that with the enhancement of TLF polarization, the redistribution of electron excited state wave function will lead to the “loss” of optical properties in the specific frequency band. The redistribution of electron ground state wave function has a significant modulation effect on the magnitude of OACs(RICs) peak. • The enhancement of the refractive index changes was observed at low frequencies. • The phenomenon of wave function exchange in laser field modulation is found. • The modulation of laser field on optical coefficient cannot cover the whole frequency band.

The nonlinear optical properties of GaAs/GaAlAs triple quantum well: Role of the electromagnetic fields and structural parameters

Being relevant to the field of device applications, multiple semiconductor quantum wells are systems that exhibit remarkable optical and electronic properties. These can be properly tuned by suitably modifying the composition, structural parameters, and the application of external probes. Here, the electronic and optical properties of a GaAs/GaAlAs triple quantum well have been investigated under the influence of applied electric and magnetic fields, as well as the change of well and barrier widths. We have used the diagonalization method to numerically solve the Schrödinger equation under the effective mass approximation for obtaining the subband energy levels and related electronic wave functions. The expressions used for evaluating linear, third-order nonlinear, and total optical absorption coefficients (TOACs) and relative refractive index changes (RRICs) were previously derived within the compact density matrix method. According to our results, whilst an increment in the applied electric field causes a red shift in TOACs and RRICs, a blue shift of the optical responses occurs with increasing the applied magnetic field. Besides, a blue shift is observed as well by changing the width of the central well (LwL), whilst a red shift is noticed when changing left and right wells (LwL and LwR) and barrier (LbL and LbR) widths for zero fields. We believe that our study could make a contribution to designing new quantum-well-based optoelectronic devices.