Multiple Fano Resonances Research Articles

Multiple Fano Resonances in Plasmonic Heptamer Clusters Composed of Split Nanorings

Fano resonances in plasmonic nanostructures are important for plasmon line shaping. Compared to a single Fano resonance, multiple Fano resonances can modify plasmon lines at several spectral positions simultaneously, but they often suffer from weak modulation depths. In this paper, plasmonic heptamer clusters comprising split nanorings are designed to form multiple Fano resonances. Three prominent Fano resonances are observed in the spectra due to the formation of multiple narrow subradiant resonances, and the multiple Fano resonances can be switched on and off by adjusting the polarization direction. Particularly, by modifying the geometry parameters, there is a large tunability of the modulation depth of each Fano resonance. Heptamer clusters comprising split nanorings are highly suitable for plasmon line shaping, and it is expected that they are useful for multiwavelength biosensing and surface-enhanced Raman scattering.

Multiple Fano resonances in monolayer hexagonal non-close-packed metallic shells

In this study, we first numerically investigate the appearance and properties of multiple Fano resonances in two-dimensional hexagonal non-close-packed arrays of symmetric metallic shells. The coexistence of broad sphere-like plasmon modes formed from the near-field interaction between the individual sphere plasmons and substantially narrower void plasmon modes supported by the inner surface of the individual shell resonant over the same range of energies can produce such Fano resonances. In particular, void and sphere-like plasmon modes of different angular momentum could directly interact without the need of symmetry breaking in the structure. A cost-effective colloidal crystal templating method is utilized to prepare the arrays of the metallic shells with small openings. The effect of the symmetry breaking on the Fano resonances in metallic cup arrays is experimentally and numerically investigated. Further tunability on the Fano resonances is gained by changing the size of the inner dielectric core, hence changing the moment of the void plasmon modes and consequently the resonance frequency. By adopting the polymer dielectric core with gain materials, our study may offer realizable experimental opportunities towards subwavelength low threshold plasmonic lasing.

Excitation and Tuning of Higher-Order Fano Resonances in Plasmonic Oligomer Clusters

Plasmonic oligomer clusters are assemblies of closely packed metallic nanoparticles. They provide a rich set of spectral features such as Fano lineshapes and a simultaneous tunability of the supported resonances in the optical wavelength regime. In this study, we investigate numerically and experimentally clusters of plasmonic nanoparticles that exhibit multiple Fano resonances due to the interference of one broad superradiant mode and multiple narrow subradiant modes. In particular we investigate oligomers with multiple ring modes and elongated chains of nanoparticles surrounded by one ring of nanoparticles. We show that the number of nanoparticles and their respective arrangement in the cluster strongly influence the spectral position and modulation depth of the spectral signature of the supported modes. Our study opens up the pathway to "plasmonic super molecules" that show unprecedented tunability, which renders them highly suitable for applications such as multiwavelength surface-enhanced Raman scattering.

Multiple Fano resonances in metallic arrays of asymmetric dual stripes

Characteristics of Fano resonances in metallic arrays of asymmetric dual stripes are theoretically investigated. The structure consists of two perfect metal stripes with unequal sizes in a unit cell. In addition to the total reflection that usually occurs in single-stripe arrays, the dual-stripe arrays exhibit two extra pairs of reflection peaks and dips, which are identified as the Fano resonance with the reflection line shape characterized by a Fano formula. In particular, the peak-dip pair on the high-frequency side is recognized as the high-order Fano resonance, as compared to its counterpart on the low-frequency side. Features of the Fano resonances are further illustrated with the electric field and surface current patterns at the corresponding frequencies. The underlying mechanism of multiple Fano resonances in the dual-stripe arrays is also discussed.

Experimental Realization of Subradiant, Superradiant, and Fano Resonances in Ring/Disk Plasmonic Nanocavities

Subradiant and superradiant plasmon modes in concentric ring/disk nanocavities are experimentally observed. The subradiance is obtained through an overall reduction of the total dipole moment of the hybridized mode due to antisymmetric coupling of the dipole moments of the parent plasmons. Multiple Fano resonances appear within the superradiant continuum when structural symmetry is broken via a nanometric displacement of the disk, due to coupling with higher order ring modes. Both subradiant modes and Fano resonances exhibit substantial reductions in line width compared to the parent plasmon resonances, opening up possibilities in optical and near IR sensing via plasmon line shape design.

Electrically controlled Fano lines in double quantum dot system with intra-dot Coulomb interaction

Theoretical study of quantum interference processes which take place during electron transport through artificial molecule formed by double quantum dot system is presented. The non-equilibrium Green function formalism based on the equation of motion method within Hartree–Fock approximation is used to calculate the conductance spectrum. Interplay between intra-dot Coulomb correlations described by parameter U and the separation of energy levels in both dots is discussed. For small U multiple Fano resonances described by Fano parameters of opposite signs and correlated with steps in electron accumulation on the dots can be observed. Positions of Fano lines as well as their shapes can be easily controlled with use of the gate voltage.

Fano Resonances in Individual Coherent Plasmonic Nanocavities

We observe the appearance of Fano resonances in the optical response of plasmonic nanocavities due to the coherent coupling between their superradiant and subradiant plasmon modes. Two reduced-symmetry nanostructures probed via confocal spectroscopy, a dolmen-style slab arrangement and a ring/disk dimer, clearly exhibit the strong polarization and geometry dependence expected for this behavior at the individual nanostructure level, confirmed by full-field electrodynamic analysis of each structure. In each case, multiple Fano resonances occur as structure size is increased.

Multiple Fano resonance in a two-dot system

Interference effects in electron transport across a double quantum dot are studied theoretically within the framework of the Hartree–Fock approach by means of the Green function formalism based on the equation of motion method. An influence of inter–dot Coulomb repulsion of strength U on conductance spectra is analyzed and a limit of U comparable to the tunneling rate between two dots is discussed in detail. A variety of Fano features, including multiple (double or triple) Fano resonances, is found as a result of interferences between four states, molecular bonding and antibonding ones, as well as these states shifted by U. The number and intensity of Fano resonance peaks present in the conductance spectrum strongly depend on the relation between parameters which describe the inter-dot tunneling rate and inter-dot Coulomb interaction between electrons.